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Higher Chern bands in helical homotrilayer transition metal dichalcogenides

Jungho Daniel Choi1,2,*, Nicolás Morales-Durán1, Yves H. Kwan3, Andrew J. Millis1,4, Nicolas Regnault1,5,6, and Daniele Guerci7,†

  • *Contact author: jchoi-visitor@flatironinstitute.org
  • †Contact author: dguerci@mit.edu

Phys. Rev. B 112, 205122 – Published 19 November, 2025

DOI: https://doi.org/10.1103/6jf2-7mst

Abstract

We propose helically twisted homotrilayer transition metal dichalcogenides as a platform for realizing correlated topological phases of matter with higher and tunable Chern numbers. We show that a clear separation of scales emerges for small twist angles, allowing us to derive a low-energy continuum model that captures the physics within moiré-scale domains. We identify regimes of twist angle and displacement field for which the highest-lying hole band is isolated from other bands and is topological with K-valley Chern number C=−2. We demonstrate that varying the displacement field can induce a transition from C=−2 to −1, as well as from a topologically trivial band to a C=−1 band. We derive an effective tight-binding description for a high-symmetry stacking domain which is valid for a wide range of twist angles, and we show that the C=−2 band can remain stable at filling fraction ν=−1 in the presence of interactions in Hartree-Fock calculations.

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