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    Net magnetization and inhomogeneous magnetic order in the high-Tc nickelate superconductor Sm1−x−yEuxCayNiO2

    Alexander J. Grutter1,*,†, Nurul Fitriyah2,3,*, Brian B. Maranville1, Saurav Prakash2, Andreas Suter4, Jochen Stahn4, Gianluca Janka4, Xing Gao2, King Yau Yip2 et al.

    Zaher Salman4, Thomas Prokscha4, Julie A. Borchers1, and A. Ariando2,‡

    • *These authors contributed equally to this work.
    • †Contact author: alexander.grutter@nist.gov
    • ‡Contact author: ariando@nus.edu.sg

    Phys. Rev. B 114, 194505 – Published 9 October, 2026

    DOI: https://doi.org/10.1103/6285-5rms

    Abstract

    High-temperature and high-magnetic-field-induced reentrant superconductivity has been discovered in the infinite-layer nickelate Sm1−x−yEuxCayNiO2 (SECNO). Infinite-layer nickelates are the closest known analogs of high-Tc cuprate superconductors, yet they host distinct magnetic ground states. Using low-energy muon spin relaxation and polarized neutron reflectometry, we reveal the magnetic order in SECNO. Magnetic freezing occurs at a significantly higher temperature than in other nickelate compounds, and a net magnetization of 55±10kAm−1 emerges and remains largely unchanged across the superconducting transition. The magnitude and temperature dependence of this net magnetization are inconsistent with a paramagnetic response, and instead point towards an as-yet unidentified magnetic ordering of Eu moments. These observations suggest a close connection between the magnetic state and the unique superconducting physics exhibited by SECNO, providing a potential mechanism for Jaccarino-Peter screening in high magnetic fields.

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