Ground states of the Shastry-Sutherland lattice materials and
Phys. Rev. B 113, 064405 – Published 4 February, 2026
DOI: https://doi.org/10.1103/5xff-rcvq
Abstract
The recent realization that the rare-earth melilites host the Shastry-Sutherland lattice within planes of ions has sparked a number of studies. This family of materials lacks appreciable site mixing and conductivity, making them promising candidates for the Shastry-Sutherland model. Herein, we present the magnetic ground states of two of these rare-earth melilites: RE = Gd and Dy. We find, through measurements of magnetic susceptibility, magnetization, and specific heat capacity (RE = Dy only), that these two melilites are antiferromagnets ( K). , in accordance with its electronic configuration, has isotropic single-ion anisotropy but shows a quadratic contribution to its magnetization. has Ising-like single-ion anisotropy and is likely an effective spin- system. Both materials exhibit metamagnetic transitions. We identify this transition in , occurring at 86(1) mT for mK, to likely be a spin-flip transition.