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Field-induced multi-Q⃗ states in a pyrochlore Heisenberg magnet

Cecilie Glittum1,2,3 and Olav F. Syljuåsen4

Phys. Rev. B 111, 214444 – Published 30 June, 2025

DOI: https://doi.org/10.1103/5rsg-2klm

Abstract

We construct exact ground states of the J1−J3b classical Heisenberg model on the pyrochlore lattice in the presence of a magnetic field. They are noncoplanar multi-Q⃗ spin configurations with a large magnetic unit cell that generalize the previously found coplanar sublattice pairing states. Using linear spin-wave theory, we show that entropy favors these multi-Q⃗ states at low temperatures in high magnetic fields. This is confirmed by Monte Carlo simulations, and a phase diagram is constructed. We also calculate the zero-temperature dynamical structure factor. Besides the usual Goldstone modes associated with the ordering Q⃗s, we find high intensity gapless modes at momenta where there are no Bragg peaks.

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