Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Editors' Suggestion
  • Open Access

Thickness-dependent topological spin texture nucleation in the high-temperature two-dimensional ferromagnet Fe3GaTe2

Y. Sun1,*, M. T. Birch2,†, D. A. Mayoh3, Y. Liu1, S. Satheesh1, G. Balakrishnan3, M. Weigand4, S. Wintz4, and M. Burghard1,‡

  • *Contact author: y.sun@fkf.mpg.de
  • †Contact author: maximilian.birch@riken.jp
  • ‡Contact author: m.burghard@fkf.mpg.de

Phys. Rev. B 113, 064425 – Published 17 February, 2026

DOI: https://doi.org/10.1103/5nvm-zlgw

Abstract

Fe3GaTe2 (FGaT) has emerged as a promising two-dimensional (2D) ferromagnet with intrinsic magnetism above room temperature. Here, we investigate the thickness-dependent nucleation and stability of topological spin textures in exfoliated FGaT flakes with thicknesses ranging from 45 to 290nm using scanning transmission x-ray microscopy. The domain size exhibits a nonmonotonic dependence on thickness, deviating from classical Kittel's t1/2 scaling due to enhanced domain-wall energy in thinner samples. Magnetic phase diagrams indicate that skyrmion nucleation becomes increasingly favorable with thickness, with a significantly expanded stability region in thicker flakes. In contrast, high-order spin textures are suppressed below ∼75nm, highlighting a critical limitation for the miniaturization of 2D skyrmion-based spintronic devices. Our results emphasize the need for better stabilization strategies, such as interfacial engineering in van der Waals heterostructures, to enable robust topological textures in thin 2D magnet flakes.

View figure in article

Physics Subject Headings (PhySH)

Article Text

Supplemental Material

References (37)

  1. J.-E. Lee, S. Yan, S. Oh, J. Hwang, J. D. Denlinger, C. Hwang, H. Lei, S.-K. Mo, S. Y. Park, and H. Ryu, Electronic structure of above-room-temperature van der Waals ferromagnet Fe3GaTe2, Nano Lett. 23, 11526 (2023).
  2. C. Gong, L. Li, Z. Li, H. Ji, A. Stern, Y. Xia, T. Cao, W. Bao, C. Wang, Y. Wang, Z. Q. Qiu, R. J. Cava, S. G. Louie, J. Xia, and X. Zhang, Discovery of intrinsic ferromagnetism in two-dimensional van der Waals crystals, Nature (London) 546, 265 (2017).
  3. B. Huang, G. Clark, E. Navarro-Moratalla, D. R. Klein, R. Cheng, K. L. Seyler, D. Zhong, E. Schmidgall, M. A. McGuire, D. H. Cobden, W. Yao, D. Xiao, P. Jarillo-Herrero, and X. Xu, Layer-dependent ferromagnetism in a van der Waals crystal down to the monolayer limit, Nature (London) 546, 270 (2017).
  4. A. M. Ruiz, D. L. Esteras, D. López-Alcalá, and J. J. Baldoví, On the origin of the above-room-temperature magnetism in the 2D van der Waals ferromagnet Fe3GaTe2, Nano Lett. 24, 7886 (2024).
  5. S. Wu, Z. He, M. Gu, L. Ren, J. Li, B. Deng, D. Wang, X. Guo, W. Li, M. Chen, Y. Chen, M. Meng, Q. Ye, B. Shen, X. Chen, J. Guo, G. Xing, I. K. Sou, and S. Li, Robust ferromagnetism in wafer-scale Fe3GaTe2 above room-temperature, Nat. Commun. 15, 10765 (2024).
  6. X. Guo, J. Li, W. Li, M. Chen, Q. Ye, S. Wu, and S. Li, Ferromagnetic enhancement of Fe3GaTe2/PtTe2 induced by interfacial spin–orbit coupling, Appl. Phys. Lett. 126, 102402 (2025).
  7. S. Jin, Y. Liu, Z. Deng, T. Wang, S. Xu, Y. Chen, X. Jiang, C. Liang, J. Hong, S.-W. Cheong, and X. Wang, Strain gradient induced skyrmion in a van der Waals magnet by wrinkling, Adv. Mater. 37, 2501935 (2025).
  8. J. Han, B. Marfoua, and J. Hong, Strain-dependent magnetic properties of two-dimensional Fe3GaTe2, J. Magnet. 29, 166 (2024).
  9. H. Pan, A. K. Singh, C. Zhang, X. Hu, J. Shi, L. An, N. Wang, R. Duan, Z. Liu, S. S. P. Parkin, P. Deb, and W. Gao, Room-temperature tunable tunneling magnetoresistance in Fe3GaTe2/WSe2/Fe3GaTe2 van der Waals heterostructures, InfoMat 6, e12504 (2024).
  10. R. Saha, H. L. Meyerheim, B. Göbel, I. Mertig, and S. S. P. Parkin, High-temperature Néel skyrmions in Fe3GaTe2 stabilized by Fe intercalation into the van der Waals gap, npj Spintron. 2, 21 (2024).
  11. X. Lv, H. Lv, Y. Huang, R. Zhang, G. Qin, Y. Dong, M. Liu, K. Pei, G. Cao, J. Zhang, Y. Lai, and R. Che, Distinct skyrmion phases at room temperature in two-dimensional ferromagnet Fe3GaTe2, Nat. Commun. 15, 3278 (2024).
  12. B. Ding, X. Li, Z. Li, X. Xi, Y. Yao, and W. Wang, Tuning the density of zero-field skyrmions and imaging the spin configuration in a two-dimensional Fe3GeTe2 magnet, NPG Asia Mater. 14, 74 (2022).
  13. Z. Li, H. Zhang, G. Li, J. Guo, Q. Wang, Y. Deng, Y. Hu, X. Hu, C. Liu, M. Qin, X. Shen, R. Yu, X. Gao, Z. Liao, J. Liu, Z. Hou, Y. Zhu, and X. Fu, Room-temperature sub-100 nm Néel-type skyrmions in non-stoichiometric van der Waals ferromagnet Fe3−xGaTe2 with ultrafast laser writability, Nat. Commun. 15, 1017 (2024).
  14. S. Xia, Y. Luo, I. A. Malik, X. Zhou, K. Han, Y. Sun, H. Lin, H. Shi, Y. Cheng, V. L. Zhang, Y. Du, S. Liu, C. Zhu, and T. Yu, Spontaneous enhancement of Dzyaloshinskii-Moriya Interaction via field-cooling-induced interface engineering in 2D van der Waals ferromagnetic ternary tellurides, arXiv:2505.06924v2.
  15. H. Zhang, Y.-T. Shao, X. Chen, B. Zhang, T. Wang, F. Meng, K. Xu, P. Meisenheimer, X. Chen, X. Huang, P. Behera, S. Husain, T. Zhu, H. Pan, Y. Jia, N. Settineri, N. Giles-Donovan, Z. He, A. Scholl, A. N'Diaye, et al., Spin disorder control of topological spin texture, Nat. Commun. 15, 3828 (2024).
  16. J. Jiang, Y. Wu, L. Kong, Y. Zhang, S. Qiu, H. Zhang, Y. Ke, S. Wang, M. Tian, and J. Tang, Stable Néel-twisted Skyrmion bags in a van der Waals magnet Fe3−xGaTe2 at room temperature, Nano Lett. 25, 3282 (2025).
  17. S. Jin, Y. Wang, H. Zheng, S. Dong, K. Han, Z. Wang, G. Wang, X. Jiang, X. Wang, J. Hong, H. Huang, Y. Zhang, T.-L. Xia, and X. Wang, Thickness- and field-dependent magnetic domain evolution in van der Waals Fe3GaTe2, Nano Lett. 24, 5467 (2024).
  18. See Supplemental Material at http://link.aps.org/supplemental/10.1103/5nvm-zlgw for the discussion of surface oxidation based on x-ray absorption spectra; SQUID measurements; domain-size calculations; contrast normalization; and additional data sets of the field sweep STXM images, which includes Refs. [32, 37].
  19. M. Weigand, S. Wintz, J. Gräfe, M. Noske, H. Stoll, B. Van Waeyenberge, and G. Schütz, TimeMaxyne: A shot-noise limited, time-resolved pump-and-probe acquisition system capable of 50 GHz frequencies for synchrotron-based X-ray microscopy, Crystals 12, 1029 (2022).
  20. C. Zhang, Z. Jiang, J. Jiang, W. He, J. Zhang, F. Hu, S. Zhao, D. Yang, Y. Liu, Y. Peng, H. Yang, and H. Yang, Above-room-temperature chiral skyrmion lattice and Dzyaloshinskii-Moriya interaction in a van der Waals ferromagnet Fe3−xGaTe2, Nat. Commun. 15, 4472 (2024).
  21. M. Wang, B. Lei, K. Zhu, Y. Deng, M. Tian, Z. Xiang, T. Wu, and X. Chen, Hard ferromagnetism in van der Waals Fe3GaTe2 nanoflake down to monolayer, npj 2D Mater. Appl. 8, 22 (2024).
  22. J.-j. Guo, Q.-l. Xia, X.-g. Wang, Y.-z. Nie, R. Xiong, and G.-h. Guo, Temperature and thickness dependent magnetization reversal in 2D layered ferromagnetic material Fe3GeTe2, J. Magn. Magn. Mater. 527, 167719 (2021).
  23. Z. Fei, B. Huang, P. Malinowski, W. Wang, T. Song, J. Sanchez, W. Yao, D. Xiao, X. Zhu, A. F. May, W. Wu, D. H. Cobden, J.-H. Chu, and X. Xu, Two-dimensional itinerant ferromagnetism in atomically thin Fe3GeTe2, Nat. Mater. 17, 778 (2018).
  24. Y. Liu and C. Petrovic, Three-dimensional magnetic critical behavior in CrI3, Phys. Rev. B 97, 014420 (2018).
  25. H. Wu, C. Hu, Y. Xie, B. G. Jang, J. Huang, Y. Guo, S. Wu, C. Hu, Z. Yue, Y. Shi, R. Basak, Z. Ren, T. Yilmaz, E. Vescovo, C. Jozwiak, A. Bostwick, E. Rotenberg, A. Fedorov, J. D. Denlinger, C. Klewe, et al., Spectral evidence for local-moment ferromagnetism in the van der Waals metals Fe3GaTe2 and Fe3GeTe2, Phys. Rev. B 109, 104410 (2024).
  26. L. Powalla, M. T. Birch, K. Litzius, S. Wintz, S. Satheesh, M. Weigand, E. Goering, G. Schütz, and M. Burghard, Skyrmion and skyrmionium formation in the two-dimensional magnet Cr2Ge2Te6, Phys. Rev. B 108, 214417 (2023).
  27. J. B. Staunton, L. Szunyogh, A. Buruzs, B. L. Gyorffy, S. Ostanin, and L. Udvardi, Temperature dependence of magnetic anisotropy: An ab initio approach, Phys. Rev. B 74, 144411 (2006).
  28. L. Deng, X. Yin, J. Tong, Y. Wu, F. Tian, and X. Zhang, Writing and reading magnetization states via strain in Fe3GaTe2/h-BN/MnBi2Te4 junction, J. Appl. Phys. 135, 174303 (2024).
  29. C. Kittel, Theory of the structure of ferromagnetic domains in films and small particles, Phys. Rev. 70, 965 (1946).
  30. F. Virot, L. Favre, R. Hayn, and M. D. Kuz'min, Theory of magnetic domains in uniaxial thin films, J. Phys. D 45, 405003 (2012).
  31. C. M. Teodorescu, Kittel's model for ferromagnetic domains, revised and completed, including the derivation of the magnetic hysteresis, Results Phys. 46, 106287 (2023).
  32. M. T. Birch, L. Powalla, S. Wintz, O. Hovorka, K. Litzius, J. C. Loudon, L. A. Turnbull, V. Nehruji, K. Son, C. Bubeck, T. G. Rauch, M. Weigand, E. Goering, M. Burghard, and G. Schütz, History-dependent domain and skyrmion formation in 2D van der Waals magnet Fe3GeTe2, Nat. Commun. 13, 3035 (2022).
  33. J. Lee, J. Yun, Y. Lee, B. Tak Kang, J. Sung Kim, N. Haberkorn, and J. Kim, Magnetic domain study in Fe3GaTe2 ferromagnet with strong perpendicular anisotropy using magnetic force microscopy, J. Appl. Phys. 136, 123905 (2024).
  34. L. Powalla, M. T. Birch, K. Litzius, S. Wintz, F. S. Yasin, L. A. Turnbull, F. Schulz, D. A. Mayoh, G. Balakrishnan, M. Weigand, X. Yu, K. Kern, G. Schütz, and M. Burghard, Seeding and emergence of composite skyrmions in a van der Waals magnet, Adv. Mater. 35, 2208930 (2023).
  35. Y. Sun, M. T. Birch, S. Finizio, L. Powalla, S. Satheesh, T. Priessnitz, E. Göring, E. Knöckl, C. Kastl, A. Holleitner, K. Kern, M. Weigand, S. Wintz, and M. Burghard, Localized spin textures stabilized by geometry-induced strain in 2D magnet Fe3GeTe2, Adv. Mater. 37, 2506279 (2025).
  36. G. Ma, R. Du, F. Lian, S. Bao, Z. Guo, X. Cai, J. Xiao, Y. Han, D. Zhang, S. Jiang, J. Huang, X. Wu, A. S. Mayorov, J. Wen, L. Wang, and G. Yu, Tailoring coercive fields and the Curie temperature via proximity coupling in WSe2/Fe3GeTe2 van der Waals heterostructures, 2D Mater. 11, 035020 (2024).
  37. D. S. Kim, J. Y. Kee, J.-E. Lee, Y. Liu, Y. Kim, N. Kim, C. Hwang, W. Kim, C. Petrovic, D. R. Lee, C. Jang, H. Ryu, and J. W. Choi, Surface oxidation in a van der Waals ferromagnet Fe3−xGeTe2, Curr. Appl. Phys. 30, 40 (2021).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation