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    Magnetic frustration in the Yb-based triangular lattice compound CuYbSe2

    Barkha Khattar1, Anzar Ali2, Masahiko Isobe2, and Yogesh Singh1,*

    • *Contact author: yogesh@iisermohali.ac.in

    Phys. Rev. B 112, 174405 – Published 3 November, 2025

    DOI: https://doi.org/10.1103/5h6v-nm9s

    Abstract

    The Yb-based triangular lattice delafossites AYbX2 (A=alkali metal, X=O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe2 with a perfect triangular lattice of Yb3+ moments. Magnetic susceptibility and heat capacity measurements reveal no evidence of long-range magnetic ordering down to 1.8 K in spite of a significant antiferromagnetic exchange between Yb3+ moments, suggesting a frustrated magnetic system. Electrical resistivity measurements indicate insulating behavior, consistent with the localized nature of magnetic moments. Heat capacity reveals that CuYbSe2 can be treated as an effective spin S=1/2 triangular lattice antiferromagnet below ∼50 K. Magnetic susceptibility measurements on single crystals reveal weak magnetic anisotropy. These properties position CuYbSe2 as another platform for exploring exotic magnetic ground states in triangular lattice systems.

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