Magnetic frustration in the Yb-based triangular lattice compound
Phys. Rev. B 112, 174405 – Published 3 November, 2025
DOI: https://doi.org/10.1103/5h6v-nm9s
Abstract
The Yb-based triangular lattice delafossites ( metal, , S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of with a perfect triangular lattice of moments. Magnetic susceptibility and heat capacity measurements reveal no evidence of long-range magnetic ordering down to 1.8 K in spite of a significant antiferromagnetic exchange between moments, suggesting a frustrated magnetic system. Electrical resistivity measurements indicate insulating behavior, consistent with the localized nature of magnetic moments. Heat capacity reveals that can be treated as an effective spin triangular lattice antiferromagnet below K. Magnetic susceptibility measurements on single crystals reveal weak magnetic anisotropy. These properties position as another platform for exploring exotic magnetic ground states in triangular lattice systems.