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    Nonmagnetic-magnetic transitions in rutile RuO2

    Yue-Fei Hou

    Siyuan Liu, Wanxiang Feng, Jiajun Lu, Xinfeng Chen, and Gui-Bin Liu*

    Ping Zhang†

    • *Contact author: gbliu@bit.edu.cn
    • †Contact author: zhang_ping@iapcm.ac.cn

    Phys. Rev. B 114, 194409 – Published 13 October, 2026

    DOI: https://doi.org/10.1103/57ck-wr34

    Abstract

    Rutile RuO2 has recently attracted great interest, as its magnetic ground state remains controversial. Experimental studies have reported either nonmagnetic (NM) or altermagnetic (AM) ground states in different crystalline samples of RuO2, highlighting the need for a reasonable explanation to resolve this contradiction. In this study, density functional theory calculations are performed to reveal the correlation-sensitive and strain-dependent magnetism of bulk RuO2. On one hand, multiple AM phases with different magnitudes of the spin magnetic moment are identified for RuO2 by employing Hubbard's U parameter as a perturbation probe. On the other hand, when appropriate strains that significantly change the crystal cell volume are applied, the ground state of RuO2 is suggested to undergo transitions between the NM state (with no spin splitting) and the magnetic states (with spin splitting in the band structure). These findings not only demonstrate intriguing physics in 4d-electron-correlated RuO2, but also retain its potential for spintronic applications.

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