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Temporal CW polarization-tomography of photon pairs from the biexciton radiative cascade: Theory and experiment

Noam Tur1, Ismail Nassar1, Ido Schwartz1, Joseph Avron1, Dan Dalacu2, Philip J. Poole2, and David Gershoni1,*

  • *Contact author: DG@physics.technion.ac.il

Phys. Rev. B 111, 235304 – Published 23 June, 2025

DOI: https://doi.org/10.1103/4z82-v82w

Abstract

We study, experimentally and theoretically, temporal correlations between the polarization of photon pairs emitted during the biexciton-exciton radiative cascade from a single semiconductor quantum dot, optically excited by a continuous-wave light source. The system is modeled by a Lindbladian coupled to two Markovian baths: One bath represents the continuous light source, and a second represents the emitted radiation. Very good agreement is obtained between the theoretical model that we constructed and a set of 36 different time-resolved, polarization correlation measurements between cascading photon pairs.

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References (43)

  1. D. V. Regelman, U. Mizrahi, D. Gershoni, E. Ehrenfreund, W. V. Schoenfeld, and P. M. Petroff, Semiconductor quantum dot: A quantum light source of multicolor photons with tunable statistics, Phys. Rev. Lett. 87, 257401 (2001).
  2. O. Benson, C. Santori, M. Pelton, and Y. Yamamoto, Regulated and entangled photons from a single quantum dot, Phys. Rev. Lett. 84, 2513 (2000).
  3. N. Akopian, N. H. Lindner, E. Poem, Y. Berlatzky, J. Avron, D. Gershoni, B. D. Gerardot, and P. M. Petroff, Entangled photon pairs from semiconductor quantum dots, Phys. Rev. Lett. 96, 130501 (2006).
  4. M. Müller, S. Bounouar, K. D. Jöns, M. Glässl, and P. Michler, On-demand generation of indistinguishable polarization-entangled photon pairs, Nat. Photon. 8, 224 (2014).
  5. M. A. Kastner, Artificial atoms, Phys. Today 46(1), 24 (1993).
  6. R. Ashoori, Electrons in artificial atoms, Nature (London) 379, 413 (1996).
  7. S. J. Freedman and J. F. Clauser, Experimental test of local hidden-variable theories, Phys. Rev. Lett. 28, 938 (1972).
  8. A. Aspect, P. Grangier, and G. Roger, Experimental tests of realistic local theories via Bell's theorem, Phys. Rev. Lett. 47, 460 (1981).
  9. D. Gammon, E. S. Snow, B. V. Shanabrook, D. S. Katzer, and D. Park, Fine structure splitting in the optical spectra of single GaAs quantum dots, Phys. Rev. Lett. 76, 3005 (1996).
  10. V. D. Kulakovskii, G. Bacher, R. Weigand, T. Kümmell, A. Forchel, E. Borovitskaya, K. Leonardi, and D. Hommel, Fine structure of biexciton emission in symmetric and asymmetric CdSe/ZnSe single quantum dots, Phys. Rev. Lett. 82, 1780 (1999).
  11. S. Gupalov, E. Ivchenko, and A. Kavokin, Fine structure of localized exciton levels in quantum wells, J. Exp. Theor. Phys. 86, 388 (1998).
  12. E. L. Ivchenko and G. Pikus, Superlattices and other Heterostructures: Symmetry and optical Phenomena, Vol. 110 (Springer Science & Business Media, New York, 2012).
  13. M. Zieliński, Y. Don, and D. Gershoni, Atomistic theory of dark excitons in self-assembled quantum dots of reduced symmetry, Phys. Rev. B. 91, 085403 (2015).
  14. R. Winik, D. Cogan, Y. Don, I. Schwartz, L. Gantz, E. R. Schmidgall, N. Livneh, R. Rapaport, E. Buks, and D. Gershoni, On-demand source of maximally entangled photon pairs using the biexciton-exciton radiative cascade, Phys. Rev. B 95, 235435 (2017).
  15. R. M. Stevenson, A. J. Hudson, A. J. Bennett, R. J. Young, C. A. Nicoll, D. A. Ritchie, and A. J. Shields, Evolution of entanglement between distinguishable light states, Phys. Rev. Lett. 101, 170501 (2008).
  16. S. Ulrich, S. Strauf, P. Michler, G. Bacher, and A. Forchel, Triggered polarization-correlated photon pairs from a single CdSe quantum dot, Appl. Phys. Lett. 83, 1848 (2003).
  17. T. Huber, A. Predojevic, M. Khoshnegar, D. Dalacu, P. J. Poole, H. Majedi, and G. Weihs, Polarization entangled photons from quantum dots embedded in nanowires, Nano Lett. 14, 7107 (2014).
  18. E. R. Schmidgall, I. Schwartz, D. Cogan, L. Gantz, T. Heindel, S. Reitzenstein, and D. Gershoni, All-optical depletion of dark excitons from a semiconductor quantum dot, Appl. Phys. Lett. 106, 193101 (2015).
  19. M. Pennacchietti, B. Cunard, S. Nahar, M. Zeeshan, S. Gangopadhyay, P. J. Poole, D. Dalacu, A. Fognini, K. D. Jöns, V. Zwiller et al., Oscillating photonic bell state from a semiconductor quantum dot for quantum key distribution, Commun. Phys. 7, 62 (2024).
  20. D. Dalacu, A. Kam, D. G. Austing, X. Wu, J. Lapointe, G. C. Aers, and P. J. Poole, Selective-area vapour–liquid–solid growth of InP nanowires, Nanotechnology 20, 395602 (2009).
  21. D. Dalacu, K. Mnaymneh, J. Lapointe, X. Wu, P. J. Poole, G. Bulgarini, V. Zwiller, and M. E. Reimer, Ultraclean emission from inasp quantum dots in defect-free Wurtzite InP nanowires, Nano Lett. 12, 5919 (2012).
  22. G. Bulgarini, M. E. Reimer, M. Bouwes Bavinck, K. D. Jöns, D. Dalacu, P. J. Poole, E. P. Bakkers, and V. Zwiller, Nanowire waveguides launching single photons in a Gaussian mode for ideal fiber coupling, Nano Lett. 14, 4102 (2014).
  23. D. Cogan, O. Kenneth, N. H. Lindner, G. Peniakov, C. Hopfmann, D. Dalacu, P. J. Poole, P. Hawrylak, and D. Gershoni, Depolarization of electronic spin qubits confined in semiconductor quantum dots, Phys. Rev. X 8, 041050 (2018).
  24. P. Laferriere, E. Yeung, M. Korkusinski, P. J. Poole, R. L. Williams, D. Dalacu, J. Manalo, M. Cygorek, A. Altintas, and P. Hawrylak, Systematic study of the emission spectra of nanowire quantum dots, Appl. Phys. Lett. 118, 161107 (2021).
  25. M. O. Scully and M. S. Zubairy, Frontmatter, in Quantum Optics (Cambridge University Press, Cambridge, 1997), pp. i–vi.
  26. G. Lindblad, On the generators of quantum dynamical semigroups, Commun. Math. Phys. 48, 119 (1976).
  27. V. Gorini, A. Frigerio, M. Verri, A. Kossakowski, and E. Sudarshan, Properties of quantum Markovian master equations, Rep. Math. Phys. 13, 149 (1978).
  28. E. B. Davies, Quantum Theory of Open Systems (Academic Press, San Diego, CA, 1976).
  29. H.-P. Breuer, F. Petruccione et al., The Theory of Open Quantum Systems (Oxford University Press on Demand, New York, 2002).
  30. R. M. Abolfath, A. Trojnar, B. Roostaei, T. Brabec, and P. Hawrylak, Dynamical magnetic and nuclear polarization in complex spin systems: Semi-magnetic II–VI quantum dots, New J. Phys. 15, 063039 (2013).
  31. Y. Benny, S. Khatsevich, Y. Kodriano, E. Poem, R. Presman, D. Galushko, P. M. Petroff, and D. Gershoni, Coherent optical writing and reading of the exciton spin state in single quantum dots, Phys. Rev. Lett. 106, 040504 (2011).
  32. E. Poem, Y. Kodriano, C. Tradonsky, N. Lindner, B. Gerardot, P. Petroff, and D. Gershoni, Accessing the dark exciton with light, Nat. Phys. 6, 993 (2010).
  33. I. Schwartz, E. R. Schmidgall, L. Gantz, D. Cogan, E. Bordo, Y. Don, M. Zielinski, and D. Gershoni, Deterministic writing and control of the dark exciton spin using single short optical pulses, Phys. Rev. X 5, 011009 (2015).
  34. E. Dekel, D. Regelman, D. Gershoni, E. Ehrenfreund, W. V. Schoenfeld, and P. M. Petroff, Cascade evolution and radiative recombination of quantum dot multiexcitons studied by time-resolved spectroscopy, Phys. Rev. B 62, 11038 (2000).
  35. Y. Benny, Y. Kodriano, E. Poem, D. Gershoni, T. A. Truong, and P. M. Petroff, Excitation spectroscopy of single quantum dots at tunable positive, neutral, and negative charge states, Phys. Rev. B 86, 085306 (2012).
  36. M. Cygorek, M. Otten, M. Korkusinski, and P. Hawrylak, Accurate and efficient description of interacting carriers in quantum nanostructures by selected configuration interaction and perturbation theory, Phys. Rev. B 101, 205308 (2020).
  37. M. Cygorek, M. Korkusinski, and P. Hawrylak, Atomistic theory of electronic and optical properties of InAsP/InP nanowire quantum dots, Phys. Rev. B 101, 075307 (2020).
  38. Y. Benny, R. Presman, Y. Kodriano, E. Poem, D. Gershoni, T. A. Truong, and P. M. Petroff, Electron-hole spin flip-flop in semiconductor quantum dots, Phys. Rev. B 89, 035316 (2014).
  39. E. R. Schmidgall, Y. Benny, I. Schwartz, R. Presman, L. Gantz, Y. Don, and D. Gershoni, Selection rules for nonradiative carrier relaxation processes in semiconductor quantum dots, Phys. Rev. B 93, 245437 (2016).
  40. E. A. Meirom, N. H. Lindner, Y. Berlatzky, E. Poem, N. Akopian, J. E. Avron, and D. Gershoni, Distilling entanglement from random cascades with partial “which path” ambiguity, Phys. Rev. A 77, 062310 (2008).
  41. E. Dekel, D. Regelman, D. Gershoni, E. Ehrenfreund, W. Schoenfeld, and P. Petroff, Radiative lifetimes of single excitons in semiconductor quantum dots—manifestation of the spatial coherence effect, Solid State Commun. 117, 395 (2001).
  42. D. Citrin, Radiative lifetimes of excitons in semiconductor quantum dots, Superlattices Microstruct. 13, 303 (1993).
  43. L. C. Andreani, F. Tassone, and F. Bassani, Radiative lifetime of free excitons in quantum wells, Solid State Commun. 77, 641 (1991).

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