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    Large spontaneous Hall effect arising from collinear antiferromagnetism in Ce2PtGe6

    Hayata Matsuda1,*, Ruo Hibino1,*, Chihiro Tabata2,3, Koji Kaneko2,3, Nonoka Higa4, Takahiro Onimaru4, Hiroto Tanaka1, Hideki Tou1, Hitoshi Sugawara1 et al.

    Junichi Hayashi5, Keiki Takeda5, and Hisashi Kotegawa1

    • *These authors contributed equally to this work.

    Phys. Rev. B 113, 195116 – Published 15 May, 2026

    DOI: https://doi.org/10.1103/4x23-wbc6

    Abstract

    The spontaneous Hall effect, corresponding to a zero-field anomalous Hall effect (AHE), is induced by symmetry breaking associated with ferromagnetism. Studies in recent years, however, have revealed that antiferromagnetic (AFM) states characterized by magnetic point groups that allow ferromagnetism can also break the relevant symmetries and induce AHE without a large net magnetization. Here, we report that the AFM system Ce2PtGe6 exhibits a pronounced spontaneous Hall effect. Single-crystal neutron scattering experiments demonstrate that Ce2PtGe6 exhibits a collinear AFM structure with a propagation vector q=0. The small net magnetization of ∼10−3 µB/Ce indicates that the observed AHE arises from symmetry breaking inherent to its AFM structure. The anomalous Hall conductivity (AHC) reaches 300 Ω−1cm−1, which exceeds the intrinsic AHC of related compounds such as Ce2CuGe6 and Ce2PdGe6. This large AHC, most likely attributed to the large spin-orbit coupling of the Pt atoms, provides a platform for understanding the interplay between the Berry curvatures and localized fmoments with an AFM configuration.

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