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    Effects of crystal field and momentum-based frustrated exchange interactions on multiorbital square skyrmion lattice

    Yan S. Zha* and Satoru Hayami†

    • *Contact author: yzha@phys.sci.hokudai.ac.jp
    • †Contact author: hayami@phys.sci.hokudai.ac.jp

    Phys. Rev. B 113, 174415 – Published 15 May, 2026

    DOI: https://doi.org/10.1103/4sqm-xhw9

    Abstract

    Motivated by recent theoretical predictions of a square-shaped skyrmion lattice (S-SkL) in centrosymmetric tetragonal Ce-based magnets [Y. Zha and S. Hayami, Phys. Rev. B 111, 165155 (2025)], we perform a comprehensive theoretical investigation into the role of multiorbital effects and momentum-based frustrated exchange interactions in stabilizing such topologically nontrivial magnetic textures. By employing self-consistent mean-field calculations over a broad range of model parameters, we demonstrate that the cooperative interplay among interorbital coupling, frustrated exchange interactions at higher-harmonic wave vectors, and crystal-field-induced anisotropy is crucial for the stabilization of the S-SkL. Furthermore, the competition between the easy-plane intraorbital anisotropy and the easy-axis interorbital anisotropy leads to a significant enhancement of the S-SkL stability region. We also identify a rich variety of multi-Q states, including a topologically nontrivial S-SkL state with a slight breaking of fourfold rotational symmetry (S−SkL′), magnetic bubble lattices (MBLs), and double-Q phases with a local/net scalar chirality. Our findings elucidate the microscopic mechanism responsible for the emergence of S-SkLs in prototypical Ce-based magnets and provide a route toward realizing skyrmion lattices in a broader class of f-electron materials beyond conventional Gd- and Eu-based systems lacking orbital angular momentum.

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