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    Off-diagonal dipolar interactions in the mixed Ising-XY magnet LiHoxEr1−xF4

    Tomer Dollberg and Moshe Schechter

    Phys. Rev. B 114, 084430 – Published 27 August, 2026

    DOI: https://doi.org/10.1103/4j7m-kx4d

    Abstract

    We theoretically investigate the influence of off-diagonal dipolar interactions in the mixed-anisotropy magnet LiHoxEr1−xF4. Motivated by experimental observations showing an unexpectedly rapid suppression of the ferromagnetic transition temperature Tc upon substitution of Ho by Er ions, we use Monte Carlo simulations incorporating off-diagonal dipolar terms to elucidate the underlying physical mechanism. Our results reveal that, unlike in the diluted magnet LiHoxY1−xF4, where dilution weakens the effect of these interactions, substitution by planar Er ions amplifies it. This leads to a pronounced reduction of Tc, closely matching experimental data, thereby providing a natural explanation for discrepancies with mean-field predictions. The findings underscore the essential role of off-diagonal dipolar interactions in determining the magnetic properties of mixed-anisotropy dipolar systems.

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