Coherent suppression and dephasing-induced reentrance of high harmonics in gapped Dirac materials
Phys. Rev. B 113, 045418 – Published 15 January, 2026
DOI: https://doi.org/10.1103/4gwm-9lpy
Abstract
High-harmonic generation in solids by intense laser pulses provides a fascinating platform for studying material properties and ultrafast electron dynamics, where its coherent character is a central aspect. Using the semiconductor Bloch equations, we uncover a mechanism suppressing the high-harmonic spectrum arising from the coherent superposition of intraband vs. interband contributions. We provide evidence for the generality of this phenomenon by extensive numerical simulations exploring the parameter space in gapped systems with both linear dispersion, such as for massive Dirac fermions, and with quadratic dispersion, as, e.g., for bilayer graphene. Moreover, we demonstrate that, upon increasing dephasing, destructive interference between intraband and interband contributions is lifted. This leads to reentrant behavior of suppressed high harmonics, i.e., a crossover from the characteristic spectral shoulder to a slowly decaying signal involving much higher harmonics. We supplement our numerical observations with analytical results for the one-dimensional case.