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    Strain-induced magnetic order in RuO2 from first-principles calculations

    Wending Liu1,*, Xiaoyu Feng1,2,*, Jun Zhao1, Peng Zhang3, Dangwei Guo1, Desheng Xue1, Mingsu Si4, ZhenHua Li5,6,7,8, Fangjun Guo9 et al.

    Xiaolong Fan1,†

    • 1The Key Laboratory of Magnetism and Magnetic Functional Materials of Ministry of Education, Lanzhou University, Lanzhou 730000, China
    • 2State Key Laboratory for Artificial Microstructure & Mesoscopic Physics and Frontiers Science Center for Nano-Optoelectronics, School of Physics, Peking University, Beijing 100871, China
    • 3Xi'an Microelectronics Technology Research Institute, Xian 710025, China
    • 4School of Materials and Energy, Lanzhou University, Lanzhou 730000, China
    • 5Lanzhou Center for Theoretical Physics, Lanzhou University, Lanzhou 730000, China
    • 6Key Laboratory of Theoretical Physics of Gansu Province, Lanzhou University, Lanzhou 730000, China
    • 7Key Laboratory of Quantum Theory and Applications of MoE, Lanzhou University, Lanzhou 730000, China
    • 8Gansu Provincial Research Center for Basic Disciplines of Quantum Physics, Lanzhou University, Lanzhou 730000, China
    • 9Lanzhou Institute of Physics, Lanzhou 730000, China

    • *These authors contributed equally to this work.
    • †Contact author: fanxiaolong@lzu.edu.cn

    Phys. Rev. B 114, 144417 – Published 16 September, 2026

    DOI: https://doi.org/10.1103/4gky-vck5

    Abstract

    RuO2, proposed as a potential altermagnet, is expected to serve as a new-generation spintronic material enabling precise control of spin transport. However, the existence of magnetic order in RuO2 has recently been widely questioned. Here, based on first-principles calculations, we systematically investigate the magnetic order in RuO2 under epitaxial strain. We find that a modest global strain can drive RuO2 from a nonmagnetic state to an antiferromagnetic state. Furthermore, near the strain-induced magnetic critical point, a modest local distortion can stabilize a spin-density-wave state over the antiferromagnetic state, with an energy difference on the order of 10−100µeV and a characteristic wavelength of about 7–10 nm. Our study provides a unified microscopic picture for the experimental controversy regarding altermagnetism in RuO2, and highlights the key roles of global strain and local distortion in tuning RuO2 magnetism and spin transport.

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