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    Magnetic and thermodynamic studies on the distorted kagome magnet Pr3BWO9

    A. Elghandour1,2, J. Arneth1, A. Yadav3, S. Luther4, P. Khuntia3,5,*, and R. Klingeler1,†

    • *Contact author: pkhuntia@iitm.ac.in
    • †Contact author: klingeler@kip.uni-heidelberg.de

    Phys. Rev. B 112, 024418 – Published 10 July, 2025

    DOI: https://doi.org/10.1103/43bm-x8cj

    Abstract

    We report specific heat, ac/dc magnetic susceptibility as well as static and pulsed field magnetization studies on the distorted kagome magnet Pr3BWO9 down to 0.4 K and up to high magnetic fields. The low-temperature thermodynamic properties are found to be governed by an electronic quasidoublet ground state, the energy splitting of which amounts to Δ1≃18 K and exhibits a quadratic field dependence with geff=2.6. Fitting of the specific heat data implies that the next excited state is strongly gapped at Δ2=430 K and threefold degenerate in zero field. Our dc and ac susceptibility studies down to 0.4 K do not detect signatures of distinct spin glass behavior. Pulsed field magnetization measurements up to 60 T confirm the Ising-like paramagnetic nature of the magnetic ground state, which is characterized by mJ=±4 and the anisotropy energy Ea≃950 K.

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