Magnetic and thermodynamic studies on the distorted kagome magnet
Phys. Rev. B 112, 024418 – Published 10 July, 2025
DOI: https://doi.org/10.1103/43bm-x8cj
Abstract
We report specific heat, ac/dc magnetic susceptibility as well as static and pulsed field magnetization studies on the distorted kagome magnet down to 0.4 K and up to high magnetic fields. The low-temperature thermodynamic properties are found to be governed by an electronic quasidoublet ground state, the energy splitting of which amounts to K and exhibits a quadratic field dependence with . Fitting of the specific heat data implies that the next excited state is strongly gapped at K and threefold degenerate in zero field. Our dc and ac susceptibility studies down to 0.4 K do not detect signatures of distinct spin glass behavior. Pulsed field magnetization measurements up to 60 T confirm the Ising-like paramagnetic nature of the magnetic ground state, which is characterized by and the anisotropy energy K.