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    Antiferromagnetic structure of KV2Se2O: A neutron diffraction study

    Yili Sun1,2,*, Yu Huang1,2,*, Jingwen Cheng1,2, Shanshan Zhang1,2, Zezhong Li1,2, Huiqian Luo1, Xiaobai Ma3,4, Wenyun Yang5, Jinbo Yang5 et al.

    Dongfeng Chen3,4, Kai Sun3,4, Matthias Gutmann6, Silvia C. Capelli6, Feiran Shen7,8, Jiazheng Hao7,8, Lunhua He1,7,8,†, Genfu Chen1,2,‡, and Shiliang Li1,2,§

    • *These authors contributed equally to this work.
    • †Contact author: lhhe@iphy.ac.cn
    • ‡Contact author: gfchen@iphy.ac.cn
    • §Contact author: slli@iphy.ac.cn

    Phys. Rev. B 112, 184416 – Published 12 November, 2025

    DOI: https://doi.org/10.1103/27n8-5q4l

    Abstract

    Altermagnetism has been proposed as a distinct class of antiferromagnets exhibiting momentum-dependent spin splitting band structures without requiring spin-orbit coupling. Recently, KV2Se2O has been identified as a metallic room-temperature altermagnet with d-wave spin-momentum locking. Here, we investigate the magnetic structure of KV2Se2O in both polycrystalline and single-crystal samples using neutron diffraction techniques. The system exhibits G-type antiferromagnetic structure with a Néel temperature TN≈ 400 K. Notably, substantial broadening of magnetic peaks was observed along L at low temperatures in single crystals, consistent with the coexistence of G-type AFM order and a c-axis spin density wave. These results demonstrate that bulk KV2Se2O cannot host altermagnetism.

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