Field-induced anisotropic magnetocaloric and magnetotransport responses in the easy-plane antiferromagnet
Phys. Rev. B 114, 274422 – Published 13 November, 2026
DOI: https://doi.org/10.1103/1t3g-x4vn
Abstract
We report a systematic study of the anisotropic magnetic, magnetocaloric, and magnetotransport properties of single crystals, which order antiferromagnetically and exhibit strong easy-plane anisotropy that constrains the Dy moments within the basal plane. Isothermal magnetization measurements reveal successive metamagnetic transitions for in-plane magnetic fields, in contrast to the weak and nearly linear hard-axis response for up to 7 T. The associated field-induced phase evolution produces a strongly anisotropic magnetic entropy change: For , the peak values of are 14.78 and for [110] and [100], respectively. Along [001], an inverse magnetocaloric response yields a minimum of . The corresponding rotating entropy changes are and for the [001]/[110] and [001]/[100] rotation pairs, respectively. Field-dependent magnetoresistance (MR) exhibits anomalies in the field ranges associated with the in-plane metamagnetic transitions, whereas the hard-axis transverse geometry exhibits a smooth positive MR reaching about at 2 K and 7 T. A joint analysis of the paramagnetic susceptibility and magnetization isotherms using a crystalline electric field (CEF) plus molecular-field model supports the contribution of single-ion CEF effects to the easy-plane anisotropy. These results reveal a correspondence between the anisotropic magnetic-state evolution, magnetic entropy changes, and magnetotransport anomalies.