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    Field-induced anisotropic magnetocaloric and magnetotransport responses in the easy-plane antiferromagnet DyAgSb2

    Zilu Xia1,2,*, Haifeng Chen1,3,*, Wenbin Shi3, Zeyang Chen1, Fanchen Chang1, Wei Zhou1, Yong Fang1, Bin Qian1, Jinlei Yao3,† et al.

    Jingguo Hu2,‡ and Zhida Han1,§

    • 1Jiangsu Laboratory of Advanced Functional Materials, School of Physics and Electronic Engineering, Suzhou University of Technology, Changshu 215500, China
    • 2College of Physics Science and Technology, Yangzhou University, Yangzhou 225002, China
    • 3Key Laboratory of Efficient Low-Carbon Energy Conversion and Utilization of Jiangsu Provincial Higher Education Institutions, School of Physical Science and Technology, Suzhou University of Science and Technology, Suzhou 215009, China

    • *These authors contributed equally to this work.
    • †Contact author: jlyao@usts.edu.cn
    • ‡Contact author: jghu@yzu.edu.cn
    • §Contact author: han@cslg.edu.cn

    Phys. Rev. B 114, 274422 – Published 13 November, 2026

    DOI: https://doi.org/10.1103/1t3g-x4vn

    Abstract

    We report a systematic study of the anisotropic magnetic, magnetocaloric, and magnetotransport properties of DyAgSb2 single crystals, which order antiferromagnetically and exhibit strong easy-plane anisotropy that constrains the Dy moments within the basal plane. Isothermal magnetization measurements reveal successive metamagnetic transitions for in-plane magnetic fields, in contrast to the weak and nearly linear hard-axis response for μ0H//[001] up to 7 T. The associated field-induced phase evolution produces a strongly anisotropic magnetic entropy change: For Δμ0H=7T, the peak values of −ΔSM are 14.78 and 12.74Jkg−1K−1 for [110] and [100], respectively. Along [001], an inverse magnetocaloric response yields a minimum of −ΔSM=−5.17Jkg−1K−1. The corresponding rotating entropy changes are 15.2Jkg−1K−1 and 13.96Jkg−1K−1 for the [001]/[110] and [001]/[100] rotation pairs, respectively. Field-dependent magnetoresistance (MR) exhibits anomalies in the field ranges associated with the in-plane metamagnetic transitions, whereas the hard-axis transverse geometry exhibits a smooth positive MR reaching about 3×102% at 2 K and 7 T. A joint analysis of the paramagnetic susceptibility and magnetization isotherms using a crystalline electric field (CEF) plus molecular-field model supports the contribution of single-ion CEF effects to the easy-plane anisotropy. These results reveal a correspondence between the anisotropic magnetic-state evolution, magnetic entropy changes, and magnetotransport anomalies.

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