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    Magnetic field tuned magnetic order and metamagnetic criticality in nonstoichiometric CeAuBi2

    Halyna Hodovanets1,2,*, Hyunsoo Kim1,2, Tristin Metz1, Yasuyuki Nakajima1, Christopher J. Eckberg1, Kefeng Wang1, Jie Yong1, Shanta R. Saha1, David Graf3 et al.

    Nicholas P. Butch1,4, Thomas Vojta2, and Johnpierre Paglione1,5,†

    • *Contact author: halyna.hodovanets@mst.edu
    • †Contact author: paglione@umd.edu

    Phys. Rev. B 113, 054432 – Published 20 February, 2026

    DOI: https://doi.org/10.1103/1qcc-by7y

    Abstract

    We present a detailed study of magnetization, resistivity, heat capacity, and x-ray and neutron powder diffraction measurements performed on single crystals of nonstoichiometric CeAuBi2, Au deficiency 18%, a strongly correlated antiferromagnet with Néel temperature TN=13.2 K. Field-dependent magnetization measurements reveal a large magnetic anisotropy at low temperatures with an easy axis along the crystallographic c axis, in which direction a spin-flop transition exhibits strong features in magnetization, specific heat, and resistivity at Hc=75 kOe. The constructed temperature-field phase diagram connects this transition to the suppression of magnetic order, which evolves from a second-order nature into a first-order transition that bifurcates at the spin-flop transition into three transitions below 1 K. The smoothed nature of the metamagnetic transitions in nonstoichiometric CeAuBi2 is well described by an Ising model with weak quenched disorder, suggesting that the presence of Au vacancies is sufficient to smear the complex metamagnetic behavior and tune the critical behavior of magnetic order.

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