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    Phase fluctuation dominated superconducting transition in ultrathin Pb films: Berezinskii-Kosterlitz-Thouless transition and incoherent Cooper pairs

    Jinyue Wang1,2, Ningning Liu1,2, Xutao Wang1,2, Yanfu Wu1,2, Wenxuan Zhang1,2, Zhan Wang1,2, Dandan Guan1,2,3, Shiyong Wang1,2,3, Hao Zheng1,2,3 et al.

    Yaoyi Li1,2,3, Hao Yang1,2,3, Xiaoxue Liu1,2,3, Liang Liu1,2,3, Canhua Liu1,2,3,*, and Jinfeng Jia1,2,3,4,5

    • *Contact author: canhualiu@sjtu.edu.cn

    Phys. Rev. B 113, 024510 – Published 20 January, 2026

    DOI: https://doi.org/10.1103/18wq-6jdk

    Abstract

    We present a comprehensive study of phase fluctuation effects in ultrathin Pb films using combined scanning tunneling microscopy and two-coil mutual inductance measurements. In atomically thin films (two to four monolayers), we observe a pronounced separation between the Cooper pair formation temperature (TΔ) and the macroscopic superconducting transition temperature (Tc), signaling the emergence of incoherent Cooper pairs and a pseudogap regime above Tc. The superfluid stiffness Jn(T) exhibits distinct scaling behaviors: a Berezinskii-Kosterlitz-Thouless (BKT)-like transition with renormalized vortex dynamics in 2-ML films, and a crossover from quantum to classical phase fluctuations in 4-ML films. Thicker films (7 to 11 ML) adhere to conventional Bardeen-Cooper-Schrieffer theory, demonstrating negligible phase fluctuations despite their subcoherence-length thickness. Our results establish the dominance of phase fluctuations in low-dimensional superconductors and provide a clean experimental platform to explore BKT and incoherent pairing physics in highly crystalline systems.

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