Phase fluctuation dominated superconducting transition in ultrathin Pb films: Berezinskii-Kosterlitz-Thouless transition and incoherent Cooper pairs
Phys. Rev. B 113, 024510 – Published 20 January, 2026
DOI: https://doi.org/10.1103/18wq-6jdk
Abstract
We present a comprehensive study of phase fluctuation effects in ultrathin Pb films using combined scanning tunneling microscopy and two-coil mutual inductance measurements. In atomically thin films (two to four monolayers), we observe a pronounced separation between the Cooper pair formation temperature () and the macroscopic superconducting transition temperature (), signaling the emergence of incoherent Cooper pairs and a pseudogap regime above . The superfluid stiffness () exhibits distinct scaling behaviors: a Berezinskii-Kosterlitz-Thouless (BKT)-like transition with renormalized vortex dynamics in 2-ML films, and a crossover from quantum to classical phase fluctuations in 4-ML films. Thicker films (7 to 11 ML) adhere to conventional Bardeen-Cooper-Schrieffer theory, demonstrating negligible phase fluctuations despite their subcoherence-length thickness. Our results establish the dominance of phase fluctuations in low-dimensional superconductors and provide a clean experimental platform to explore BKT and incoherent pairing physics in highly crystalline systems.