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    Reversible and Irreversible Voltage Manipulation of Interfacial Magnetic Anisotropy in Pt/Co/Oxide Multilayers

    Aymen Fassatoui1, Jose Peña Garcia1, Laurent Ranno1, Jan Vogel1, Anne Bernand-Mantel2, Hélène Béa3, Sergio Pizzini4, and Stefania Pizzini1,*

    • 1University Grenoble Alpes, CNRS, Institut Néel, Grenoble, France
    • 2Laboratoire de Physique et Chimie des Nano-Objets, Université de Toulouse, Toulouse, France
    • 3University Grenoble Alpes, CEA, CNRS, Grenoble INP, IRIG-SPINTEC, Grenoble, France
    • 4Department of Materials Science, University of Milano-Bicocca, Via Cozzi 53 Milano, Italy

    • *stefania.pizzini@neel.cnrs.fr

    Phys. Rev. Applied 14, 064041 – Published 14 December, 2020

    DOI: https://doi.org/10.1103/PhysRevApplied.14.064041

    Abstract

    The perpendicular magnetic anisotropy at the Co-oxide interface in Pt/Co/MOx (MOx=MgOx, AlOx, TbOx) is modified by an electric field using a 10-nm-thick ZrO2 as a solid electrolyte. The large voltage-driven modification of the interfacial magnetic anisotropy and the nonvolatility of the effect is explained in terms of the migration of oxygen ions toward or away from the Co/MOx interface. While the effect is reversible in Pt/Co/AlOx and Pt/Co/TbOx, where the Co layer can be oxidized or reduced, in Pt/Co/MgOx the effect is found to be irreversible. We propose that these differences may be related to the different nature of the ionic conduction within the MOx layers.

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