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Enhancement of vacuum-ultraviolet dispersive-wave emission using gas-filled tapered hollow-core fibers

Yinuo Zhao1,2,3,4,*, Donghan Liu1,2,3,4,*, Baoqi Shi5,6,*, Zhiyuan Huang1,3,4,†, Tiandao Chen1, Jinyu Pan1, Zhengzheng Liu1, Xinglin Zeng3,4, Wenbin He3,4 et al.

Jiapeng Huang3,4, Jinxin Zhan3,4, Xin Jiang3,4, Yuxin Leng1, Junqiu Liu5,6,‡, and Meng Pang1,3,4,§

  • 1State Key Laboratory of Ultra-intense Laser Science and Technology, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, 201800 Shanghai, China
  • 2Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, 100049 Beijing, China
  • 3Russell Centre for Advanced Lightwave Science, Shanghai Institute of Optics and Fine Mechanics and Hangzhou Institute of Optics and Fine Mechanics, Hangzhou, 311421 Zhejiang, China
  • 4Zhejiang Key Laboratory of Microstructured Specialty Optical Fiber, Hangzhou Institute of Optics and Fine Mechanics, Hangzhou, 311400 Zhejiang, China
  • 5International Quantum Academy and Shenzhen Futian SUSTech Institute for Quantum Technology and Engineering, Shenzhen, 518048 Guangdong, China
  • 6Hefei National Laboratory, University of Science and Technology of China, Hefei, 230088 Anhui, China

  • *These authors contributed equally to this work.
  • †Contact author: huangzhiyuan@siom.ac.cn
  • ‡Contact author: liujq@iqasz.cn
  • §Contact author: pangmeng@siom.ac.cn

Phys. Rev. Applied 25, L041001 – Published 1 April, 2026

DOI: https://doi.org/10.1103/ym25-kz9p

Abstract

The recent breakthroughs in laser-driving the 229Th nuclear transition have created an urgent demand for scalable vacuum-ultraviolet (VUV) sources capable of supporting high power spectral density at the critical 148.38 nm isomer energy. However, generating sufficient photon flux to overcome the low nuclear excitation probability remains a challenge for compact setups. While resonant dispersive-wave emission in gas-filled hollow-core fibers offers a promising route, standard capillaries face a fundamental trade-off: maximizing input coupling requires large core diameters, whereas efficient nonlinear VUV conversion demands high intensities and small cores. Here we resolve this conflict using a gas-filled tapered capillary fiber. This architecture uses a longitudinally decreasing core diameter to combine a large input aperture with adiabatic field concentration, thereby continuously enhancing the nonlinear interaction. Experimentally, we demonstrate a widely tunable source (135–240 nm) that achieves a twofold efficiency increase specifically at a wavelength of 148.38 nm compared with uniform geometries. By providing a scalable route to high-flux VUV generation, this work establishes a critical tabletop tool for advancing solid-state nuclear clocks and time-resolved spectroscopy.

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