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    Quantum nanophotonic interface for tin-vacancy centers in thin-film diamond

    Hope Lee1,*, Hannah C. Kleidermacher1,*, Abigail J.M. Stein1,*, Hyunseok Oh2, Lillian B. Hughes Wyatt3, Casey K. Kim3, Luca Basso4, Andrew M. Mounce4, Yongqiang Wang5 et al.

    Shei S. Su4, Michael Titze4,6, Ania C. Bleszynski Jayich2, and Jelena Vučković1,†

    • *These authors contributed equally to this work.
    • †Contact author: jela@stanford.edu

    Phys. Rev. Applied 25, 044074 – Published 27 April, 2026

    DOI: https://doi.org/10.1103/vwt7-b64x

    Abstract

    The negatively charged tin-vacancy center in diamond (SnV−) is an excellent solid-state qubit with optically addressable transitions and a long electron spin-coherence time at elevated temperatures (approximately 1.7 K). However, implementing scalable quantum nodes with high-fidelity optical readout of the electron spin state requires efficient photon emission and collection from the system. In this manuscript, we report a quantum photonic interface for SnV− centers based on one-dimensional photonic crystal cavities fabricated in diamond thin films. Furthermore, we provide a rigorous description of the spontaneous emission dynamics of our system, taking into account individual contributions from both the C and D transitions of the emitter. This allows for the determination of Purcell factors per transition and, by extension, the C/D branching ratio SnV− zero-phonon line. We observe quality factors of up to approximately 6000 across this sample, and we measure up to a 12-fold lifetime reduction, which translates into a Purcell factor of FC=26.2±1.5 for a targeted C transition. By considering the cavity-mode polarization alignment with the C- and D-transition dipole moments, we validate the C/D branching ratio to be ηBR=0.75±0.01, in line with previous theoretical and experimental findings.

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