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    Visualizing the polarization of collective magnetic excitations in the chiral helimagnet CrNb3S6 by microwave circular dichroism spectroscopy

    Tomonori Arakawa1,*, Hiroki Shoji2, Yusuke Shimamoto2, Yusuke Kousaka2, Jun-ichiro Ohe3, Seitaro Kon1, and Yoshihiko Togawa2,4

    • *Contact author: tomonori-arakawa@aist.go.jp

    Phys. Rev. Applied 24, 044017 – Published 7 October, 2025

    DOI: https://doi.org/10.1103/vl98-dfpb

    Abstract

    Exotic and controllable collective magnetic excitations in a chiral helimagnet CrNb3S6 make it an ideal candidate for exploring emergent electromagnetic phenomena and developing magnon-based devices. Here, we experimentally investigate the polarization properties of the magnetic excitations in a CrNb3S6 single crystal using circular polarization resolved spectroscopy. An external magnetic field controlled the magnetic structure from a chiral soliton lattice (CSL), consisting of chiral soliton kinks and ferromagnetic domains, to the forced ferromagnet (FFM) phase, and conventional and circular dichroism microwave spectra are observed over a wide frequency range. The observed magnetic excitations, including a CSL phonon mode, Kittel-like mode, and band structures likely due to the excitation of magnetostatic waves, are well characterized by distinct polarization properties. These results visualize the local spin dynamics in the CSL and the influence of the Dzyaloshinskii–Moriya interaction in the FFM phase, aiding the fundamental understanding of the spin dynamics in chiral helimagnets.

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