Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Seedless nonresonant gas-flow velocimetry with single-shot coherent Rayleigh-Brillouin scattering

Alexandros Gerakis*

Junhwi Bak† and Robert Randolph

Mikhail N. Shneider

  • Department of Mechanical & Aerospace Engineering, Princeton University, 08544 Princeton, New Jersey, USA

  • *Contact author: alexandros.gerakis@list.lu
  • †Present address: Hexium, Inc., Austin, Texas, USA.

Phys. Rev. Applied 24, 064035 – Published 10 December, 2025

DOI: https://doi.org/10.1103/ktvb-mw8z

Abstract

We demonstrate neutral gas-flow velocimetry by exploiting the optical dipole forces exerted by precisely tailored high-intensity laser fields on polarizable particles, in the form of single-shot coherent Rayleigh-Brillouin scattering (CRBS). This enables mapping of the velocity distribution function of the particles in a single laser shot of approximately 200 ns duration, allowing us to perform spectroscopic measurements in the time, rather than the frequency, domain. Importantly, CRBS results in a coherent signal beam, which renders the technique ideal for measurements in optically noisy environments. By correlating the time shift of the resulting spectrum to the Doppler shift caused by the bulk motion of particles, we perform neutral gas-flow velocimetry without the need to seed the flow, nondestructively, for a variety of gases, atomic or molecular. We demonstrate gas-flow velocimetry at flow velocities as low as 1ms−1, with similar velocity resolution, while temperature and gas density can also be estimated from the same single-shot spectra. To prove the effectiveness of the measurement technique, we benchmark it against Pitot tube measurements, which show excellent agreement.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (67)

  1. R. J. Goldstein, K. Y. Lau, and C. C. Leung, Velocity and turbulence measurements in combustion systems, Exp. Fluids 1, 93 (1983).
  2. P. O. Ayegba and L. C. Edomwonyi-Otu, Turbulence statistics and flow structure in fluid flow using particle image velocimetry technique: A review, Eng. Rep. 2, e12138 (2020).
  3. A. S. Monin, On the nature of turbulence, Sov. Phys. Usp. 21, 429 (1978).
  4. P. M. Danehy, R. A. Burns, D. T. Reese, J. E. Retter, and S. P. Kearney, Fleet velocimetry for aerodynamics, Annu. Rev. Fluid Mech. 54, 525 (2022).
  5. M. Raffel, A. Bauknecht, M. Ramasamy, G. K. Yamauchi, J. T. Heineck, and L. N. Jenkins, Contributions of particle image velocimetry to helicopter aerodynamics, AIAA J. 55, 2859 (2017).
  6. R. J. Bomphrey, Advances in animal flight aerodynamics through flow measurement, Evol. Biol. 39, 1 (2012).
  7. A. V. Bilsky, O. A. Gobyzov, and D. M. Markovich, Evolution and recent trends of particle image velocimetry for an aerodynamic experiment (review), Thermophys. Aeromech. 27, 1 (2020).
  8. M. I. Hasan and J. L. Walsh, Influence of gas flow velocity on the transport of chemical species in an atmospheric pressure air plasma discharge, Appl. Phys. Lett. 110, 134102 (2017).
  9. M. Whitby and N. Quirke, Fluid flow in carbon nanotubes and nanopipes, Nat. Nanotechnol. 2, 87 (2007).
  10. K. J. Loh and F. Azhari, Recent advances in skin-inspired sensors enabled by nanotechnology, JOM 64, 793 (2012).
  11. M. Yadav, X. Dai, and J. R. Roth, in IEEE Conference Record – Abstracts. 2005 IEEE International Conference on Plasma Science (IEEE, Piscataway, NJ, 2005), p. 177.
  12. J. Turner V and M. Wosnik, Velocity data in a fully developed experimental wind turbine array boundary layer, Wind Energy 25, 1495 (2022).
  13. R. B. Spelay, K. F. Adane, R. S. Sanders, R. J. Sumner, and R. G. Gillies, The effect of low Reynolds number flows on Pitot tube measurements, Flow. Meas. Instrum. 45, 247 (2015).
  14. G. Comte-Bellot, Hot-wire anemometry, Annu. Rev. Fluid Mech. 8, 209 (1976).
  15. P. C. Stainback and K. A. Nagabushana, Review: Hot-wire anemometry in transonic and subsonic slip flows, J. Fluids Eng. 119, 14 (1997).
  16. F. Motallebi, A review of the hot-wire technique in 2-D compressible flows, Prog. Aerosp. Sci. 30, 267 (1994).
  17. I. Grant, Particle image velocimetry: A review, Proc. Inst. Mech. Eng., Part C: J. Mech. Eng. Sci. 211, 55 (1997).
  18. J. Westerweel, G. E. Elsinga, and R. J. Adrian, Particle image velocimetry for complex and turbulent flows, Annu. Rev. Fluid Mech. 45, 409 (2013).
  19. S. Scharnowski and C. J. Kähler, Particle image velocimetry—Classical operating rules from today’s perspective, Opt. Lasers Eng. 135, 106185 (2020).
  20. S. Fu, P. H. Biwole, and C. Mathis, Particle tracking velocimetry for indoor airflow field: A review, Build. Environ. 87, 34 (2015).
  21. D. Dabiri and C. Pecora, Particle Tracking Velocimetry (IOP Publishing, Bristol, United Kingdom, 2019), pp. 2053–2563.
  22. H. G. Maas, A. Gruen, and D. Papantoniou, Particle tracking velocimetry in three-dimensional flows, Exp. Fluids 15, 133 (1993).
  23. M. G. R. Guastamacchia, R. Xue, K. Madi, W. T. E. Pitkeathly, P. D. Lee, S. E. D. Webb, S. H. Cartmell, and P. A. Dalgarno, Instantaneous 4D micro-particle image velocimetry (μPIV) via multifocal microscopy (MUM), Sci. Rep. 12, 18458 (2022).
  24. H. Chen and L. P. Dasi, An in-vitro study of the flow past a transcatheter aortic valve using time-resolved 3D particle tracking, Ann. Biomed. Eng. 51, 1449 (2023).
  25. W. H. Stevenson, Laser Doppler velocimetry: A status report, Proc. IEEE 70, 652 (1982).
  26. V. Rajan, B. Varghese, T. G. van Leeuwen, and W. Steenbergen, Review of methodological developments in laser Doppler flowmetry, Lasers Med. Sci. 24, 269 (2009).
  27. J. W. Czarske, Laser Doppler velocimetry using powerful solid-state light sources, Meas. Sci. Technol. 17, R71 (2006).
  28. J. W. Gregory, K. Asai, M. Kameda, T. Liu, and J. P. Sullivan, A review of pressure-sensitive paint for high-speed and unsteady aerodynamics, Proc. Inst. Mech. Eng., Part G: J. Aerosp. Eng. 222, 249 (2008).
  29. B. McLachlan and J. Bell, Pressure-sensitive paint in aerodynamic testing, Exp. Therm Fluid Sci. 10, 470 (1995). experimental methods in Thermal and Fluid Science
  30. J. W. Gregory, H. Sakaue, T. Liu, and J. P. Sullivan, Fast pressure-sensitive paint for flow and acoustic diagnostics, Annu. Rev. Fluid Mech. 46, 303 (2014).
  31. A. Gerakis, M. N. Shneider, and B. C. Stratton, Remote-sensing gas measurements with coherent Rayleigh-Brillouin scattering, Appl. Phys. Lett. 109, 31112 (2016).
  32. A. Gerakis, M. N. Shneider, and P. F. Barker, Single-shot coherent Rayleigh–Brillouin scattering using a chirped optical lattice, Opt. Lett. 38, 4449 (2013).
  33. J. Bak, R. Randolph, and A. Gerakis, Torr-level, seedless, non-resonant velocity distribution function measurement with a dual-color, single-shot coherent Rayleigh–Brillouin scattering scheme, J. Phys. D: Appl. Phys. 56, 074001 (2023).
  34. A. S. Meijer, A. S. de Wijn, M. F. E. Peters, N. J. Dam, and W. van de Water, Coherent Rayleigh–Brillouin scattering measurements of bulk viscosity of polar and nonpolar gases, and kinetic theory, J. Chem. Phys. 133, 164315 (2010).
  35. R. K. Hanson, J. M. Seitzman, and P. H. Paul, Planar laser-fluorescence imaging of combustion gases, Appl. Phys. B 50, 441 (1990).
  36. M. P. Lee, B. K. McMillin, and R. K. Hanson, Temperature measurements in gases by use of planar laser-induced fluorescence imaging of NO, Appl. Opt. 32, 5379 (1993).
  37. J. Crimaldi, Planar laser induced fluorescence in aqueous flows, Exp. Fluids 44, 851 (2008).
  38. N. Jiang, J. Bruzzese, R. Patton, J. Sutton, R. Yentsch, D. Gaitonde, W. Lempert, J. Miller, T. Meyer, R. Parker, et al., NO PLIF imaging in the CUBRC 48-inch shock tunnel, Exp. Fluids 53, 1637 (2012).
  39. P. M. Danehy, S. O’Byrne, A. Frank, P. Houwing, J. S. Fox, and D. R. Smith, Flow-tagging velocimetry for hypersonic flows using fluorescence of nitric oxide, AIAA J. 41, 263 (2003).
  40. A. Dogariu, L. E. Dogariu, M. S. Smith, J. Lafferty, and R. B. Miles, in AIAA Scitech 2019 Forum (AIAA, Reston, VA, 2019), p. 1089.
  41. D. Pulford, D. Newman, A. Houwing, and R. Sandeman, The application of coherent anti-Stokes Raman scattering to temperature measurements in a pulsed high enthalpy supersonic flow, Shock Waves 4, 119 (1994).
  42. M. W. Smith, O. Jarrett, R. R. Antcliff, G. B. Northam, A. D. Cutler, and D. J. Taylor, Coherent anti-Stokes Raman spectroscopy temperature measurements in a hydrogen-fueled supersonic combustor, J. Propul. Power 9, 163 (1993).
  43. A. D. Cutler, P. M. Danehy, R. R. Springer, S. O’Byrne, D. P. Capriotti, and R. DeLoach, Coherent anti-Stokes Raman spectroscopic thermometry in a supersonic combustor, AIAA J. 41, 2451 (2003).
  44. R. D. Hancock, F. R. Schauer, R. P. Lucht, and R. L. Farrow, Dual-pump coherent anti-Stokes Raman scattering measurements of nitrogen and oxygen in a laminar jet diffusion flame, Appl. Opt. 36, 3217 (1997).
  45. N. J. DeLuca, R. B. Miles, N. Jiang, W. D. Kulatilaka, A. K. Patnaik, and J. R. Gord, Fleet velocimetry for combustion and flow diagnostics, Appl. Opt. 56, 8632 (2017).
  46. L. E. Dogariu, A. Dogariu, R. B. Miles, M. S. Smith, and E. C. Marineau, in 2018 AIAA Aerospace Sciences Meeting (AIAA, Reston, VA, 2018), p. 1769.
  47. J. A. Wehrmeyer, L. A. Ribarov, D. A. Oguss, and R. W. Pitz, Flame flow tagging velocimetry with 193 nm H2O photodissociation, Appl. Opt. 38, 6912 (1999).
  48. T. Sakurai, T. Handa, S. Koike, K. Mii, and A. Nakano, Study on the particle traceability in transonic and supersonic flows using molecular tagging velocimetry, J. Visualization 18, 511 (2015).
  49. D. Zahradka, N. Parziale, M. Smith, and E. Marineau, Krypton tagging velocimetry in a turbulent Mach 2.7 boundary layer, Exp. Fluids 57, 62 (2016).
  50. M. A. Mustafa, D. Shekhtman, and N. J. Parziale, Single-laser krypton tagging velocimetry investigation of supersonic air and N2 boundary-layer flows over a hollow cylinder in a shock tube, Phys. Rev. Appl. 11, 064013 (2019).
  51. N. J. Parziale, M. S. Smith, and E. C. Marineau, Krypton tagging velocimetry of an underexpanded jet, Appl. Opt. 54, 5094 (2015).
  52. A. G. Hsu, R. Srinivasan, R. D. Bowersox, and S. W. North, Molecular tagging using vibrationally excited nitric oxide in an underexpanded jet flowfield, AIAA J. 47, 2597 (2009).
  53. R. Sánchez-González, R. D. W. Bowersox, and S. W. North, Vibrationally excited NO tagging by NO(A2Σ+) fluorescence and quenching for simultaneous velocimetry and thermometry in gaseous flows, Opt. Lett. 39, 2771 (2014).
  54. R. G. Seasholtz, A. E. Buggele, and M. F. Reeder, Flow measurements based on Rayleigh scattering and Fabry-Perot interferometer, Opt. Lasers Eng. 27, 543 (1997).
  55. R. Seasholtz and L. Greer III, in 36th AIAA Aerospace Sciences Meeting and Exhibit (AIAA, Reston, VA, 1998), p. 206.
  56. J. Estevadeordal, N. Jiang, A. D. Cutler, J. J. Felver, M. N. Slipchenko, P. M. Danehy, J. R. Gord, and S. Roy, High-repetition-rate interferometric Rayleigh scattering for flow-velocity measurements, Appl. Phys. B 124, 41 (2018).
  57. J. Forkey, N. Finkelstein, W. Lempert, and R. Miles, Demonstration and characterization of filtered Rayleigh scattering for planar velocity measurements, AIAA J. 34, 442 (1996).
  58. R. B. Miles, W. R. Lempert, and J. N. Forkey, Laser Rayleigh scattering, Meas. Sci. Technol. 12, R33 (2001).
  59. J. George, T. P. Jenkins, and R. B. Miles, in 30th AIAA Aerodynamic Measurement Technology and Ground Testing Conference (AIAA, Reston, VA, 2014), p. 2231.
  60. J. Bak, R. Randolph, A. Gerakis, and M. N. Shneider, in AIAA Scitech 2021 Forum (AIAA, Reston, VA).
  61. J. Bak, R. Randolph, and A. Gerakis, Dual color, frequency, pulse duration and shape agile laser system for particle spectroscopy and manipulation, Opt. Express 30, 41709 (2022).
  62. K. König, F. Bauerfeld, D. Sauer, H. Schuck, A. Uchugonova, E. Lei, M. Stark, T. Velten, R. Bückle, and R. LeHarzic, in Nano Biophotonics: Science and Technology, edited by H. Masuhara, S. Kawata, and F. Tokunaga (Elsevier, Amsterdam, the Netherlands, 2007), Vol. 3, pp. 287–296.
  63. A. Gerakis, Single shot CRBS neutral gas flow velocimetry, https://www.youtube.com/watch?v=zyowmHsZpuU (2023), accessed on 2023/07/29.
  64. H. C. Man, J. Duan, and T. M. Yue, Dynamic characteristics of gas jets from subsonic and supersonic nozzles for high pressure gas laser cutting, Opt. Laser Technol. 30, 497 (1998).
  65. H. Hoghooghi, M. N. Ahmadabadi, and M. D. Manshadi, Optimization of a subsonic wind tunnel nozzle with low contraction ratio via ball-spine inverse design method, J. Mech. Sci. Technol. 30, 2059 (2016).
  66. I. Care and F. Fourneaux, Investigation of the pressure response of different Pitot tubes, Flow Meas. Instrum. 72, 101714 (2020).
  67. R. Klopfenstein, Jr., Air velocity and flow measurement using a Pitot tube, ISA Trans. 37, 257 (1998).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation