Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Optimal and efficient inference tools for field tracking with precessing spins

Klaudia Dilcher1,*, Piotr Bania2,3,†, Diana Méndez-Avalos4, Aleksandra Sierant4, Morgan W. Mitchell4,5, and Jan Kołodyński3,1,‡

  • *Contact author: k.dilcher@cent.edu.pl
  • †Contact author: pba@agh.edu.pl
  • ‡Contact author: jankolo@ifpan.edu.pl

Phys. Rev. Applied 26, 024062 – Published 25 August, 2026

DOI: https://doi.org/10.1103/jfhj-kr1j

Abstract

Precise, real-time monitoring of magnetic field evolution is significant in applications including magnetic navigation and searches for physics beyond the standard model. One main field-monitoring technique, the spin-precession magnetometer (SPM), observes electron, nucleus, color center, or muon spins as they precess in response to their local magnetic field. Here, we study Bayesian signal-recovery methods for SPMs in the free-induction decay mode. In particular, we study tracking of field changes well within the coherence time of the spin system and thus well beyond the response bandwidth, as in [R. Jiménez-Martínez et al. Phys. Rev. Lett. 120, 040503 (2018)]. We derive the Bayesian Cramér-Rao bound that dictates the ultimate precision in estimating the Larmor frequency, which we show is attained by the computationally expensive prediction error method. Relative to this benchmark, we show that the extended Kalman filter (EKF) and cubature Kalman filter offer near-optimal tracking that is also computationally efficient, with the use of the latter giving better results only for a large spin number. Focusing thus on the EKF, we show that it is sufficient to accurately track fluctuating and unknown transient signals. Our methods can be easily adapted to other types of sensors undergoing nonlinear dissipative dynamics and experiencing intrinsic Gaussian-like stochastic noises.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (87)

  1. D. F. Jackson Kimball, D. Budker, T. E. Chupp, A. A. Geraci, S. Kolkowitz, J. T. Singh, and A. O. Sushkov, Probing fundamental physics with spin-based quantum sensors, Phys. Rev. A 108, 010101 (2023).
  2. N. Aslam, H. Zhou, E. K. Urbach, M. J. Turner, R. L. Walsworth, M. D. Lukin, and H. Park, Quantum sensors for biomedical applications, Nat. Rev. Phys. 5, 157 (2023).
  3. D. Vasyukov, Y. Anahory, L. Embon, D. Halbertal, J. Cuppens, L. Neeman, A. Finkler, Y. Segev, Y. Myasoedov, M. L. Rappaport et al., A scanning superconducting quantum interference device with single electron spin sensitivity, Nat. Nanotechnol. 8, 639 (2013).
  4. I. K. Kominis, T. W. Kornack, J. C. Allred, and M. V. Romalis, A subfemtotesla multichannel atomic magnetometer, Nature (London) 422, 596 (2003).
  5. D. Budker and M. Romalis, Optical magnetometry, Nat. Phys. 3, 227 (2007).
  6. J. M. Taylor, P. Cappellaro, L. Childress, L. Jiang, D. Budker, P. R. Hemmer, A. Yacoby, R. Walsworth, and M. D. Lukin, High-sensitivity diamond magnetometer with nanoscale resolution, Nat. Phys. 4, 810 (2008).
  7. F. Casola, T. van der Sar, and A. Yacoby, Probing condensed matter physics with magnetometry based on nitrogen-vacancy centres in diamond, Nat. Rev. Mater. 3, 1 (2018).
  8. H. B. Dang, A. C. Maloof, and M. V. Romalis, Ultrahigh sensitivity magnetic field and magnetization measurements with an atomic magnetometer, Appl. Phys. Lett. 97, 151110 (2010).
  9. D. Budker and D. F. J. Kimball, Optical Magnetometry (Cambridge University Press, Cambridge, England, 2013).
  10. A. J. Canciani and C. J. Brennan, An analysis of the benefits and difficulties of aerial magnetic vector navigation, IEEE Trans. Aerosp. Electron. Syst. 56, 4161 (2020).
  11. A. J. Canciani, Magnetic navigation on an F-16 aircraft using online calibration, IEEE Trans. Aerosp. Electron. Syst. 58, 420 (2022).
  12. I. M. Savukov and M. V. Romalis, NMR detection with an atomic magnetometer, Phys. Rev. Lett. 94, 123001 (2005).
  13. I. M. Savukov, V. S. Zotev, P. L. Volegov, M. A. Espy, A. N. Matlashov, J. J. Gomez, R. H. Kraus Jr., MRI with an atomic magnetometer suitable for practical imaging applications, J. Magn. Reson. 199, 188 (2009).
  14. M. V. Romalis and H. B. Dang, Atomic magnetometers for materials characterization, Mater. Today 14, 258 (2011).
  15. M. J. Brookes, J. Leggett, M. Rea, R. M. Hill, N. Holmes, E. Boto, and R. Bowtell, Magnetoencephalography with optically pumped magnetometers (OPM-MEG): The next generation of functional neuroimaging, Trends Neurosci. 45, 621 (2022).
  16. K. Jensen, M. A. Skarsfeldt, H. Staerkind, J. Arnbak, M. V. Balabas, S.-P. Olesen, B. H. Bentzen, and E. S. Polzik, Magnetocardiography on an isolated animal heart with a room-temperature optically pumped magnetometer, Sci. Rep. 8, 16218 (2018).
  17. Y. J. Kim, I. Savukov, and S. Newman, Magnetocardiography with a 16-channel fiber-coupled single-cell Rb optically pumped magnetometer, Appl. Phys. Lett. 114, 143702 (2019).
  18. L. Ljung and T. Söderström, Theory and Practice of Recursive Identification, 3rd ed. (MIT Press, Cambridge, Mass., 1987), Vol. 4.
  19. S. Särkkä, Bayesian Filtering and Smoothing, Institute of Mathematical Statistics Textbooks (Cambridge University Press, Cambridge, 2014).
  20. H. L. van Trees, Detection, Estimation and Modulation Theory (Wiley, New York, 1968), Vol. I.
  21. Bayesian Bounds for Parameter Estimation and Nonlinear Filtering/Tracking, edited by H. L. van Trees and K. L. Bell (Wiley-IEEE Press, Piscataway, NJ, 2007).
  22. R. Jiménez-Martínez, J. Kołodyński, C. Troullinou, V. G. Lucivero, J. Kong, and M. W. Mitchell, Signal tracking beyond the time resolution of an atomic sensor by Kalman filtering, Phys. Rev. Lett. 120, 040503 (2018).
  23. C. Gemmel, W. Heil, S. Karpuk, K. Lenz, C. Ludwig, Y. Sobolev, K. Tullney, M. Burghoff, W. Kilian, S. Knappe-Grüneberg et al., Ultra-sensitive magnetometry based on free precession of nuclear spins, Eur. Phys. J. D 57, 303 (2010).
  24. Z. D. Grujić, P. A. Koss, G. Bison, and A. Weis, A sensitive and accurate atomic magnetometer based on free spin precession, Eur. Phys. J. D 69, 135 (2015).
  25. D. Hunter, S. Piccolomo, J. D. Pritchard, N. L. Brockie, T. E. Dyer, and E. Riis, Free-induction-decay magnetometer based on a microfabricated Cs vapor cell, Phys. Rev. Appl. 10, 014002 (2018).
  26. K. Yi, Y. Liu, B. Wang, W. Xiao, D. Sheng, X. Peng, and H. Guo, Free-induction-decay He4 magnetometer using a multipass cell, Phys. Rev. Appl. 22, 014084 (2024).
  27. J. Kong, Y. Feng, Y. Wang, Q. Wang, and X.-M. Lu, Optimized spin estimation in atomic sensors via Kalman filter and smoother, Phys. Rev. Appl. 24, 064001 (2025).
  28. V. G. Lucivero, R. Jiménez-Martínez, J. Kong, and M. W. Mitchell, Squeezed-light spin noise spectroscopy, Phys. Rev. A 93, 053802 (2016).
  29. C. Troullinou, V. G. Lucivero, and M. W. Mitchell, Quantum-enhanced magnetometry at optimal number density, Phys. Rev. Lett. 131, 133602 (2023).
  30. R. D. Gill and B. Y. Levit, Applications of the van Trees inequality: A Bayesian Cramér-Rao bound, Bernoulli 1(1/2), 59 (1995).
  31. K. J. Astrom, Maximum likelihood and prediction error methods, IFAC Proc. 12, 551 (1979).
  32. R. E. Kalman, A new approach to linear filtering and prediction problems, J. Basic Eng-t. Asme. 82, 35 (1960).
  33. R. E. Kalman and R. S. Bucy, New results in linear filtering and prediction theory, J. Basic Eng-t. Asme. 83, 95 (1961).
  34. G. L. Smith, S. F. Schmidt, and L. A. McGee, Application of statistical filter theory to the optimal estimation of position and velocity on board a circumlunar vehicle, Tech. Rep. NASA-TR-R-135, 1962.
  35. C. Hide, T. Moore, and M. Smith, Adaptive Kalman filtering for low-cost INS/GPS, J. Navigation 56, 143 (2003).
  36. K. Jo, Y. Jo, J. K. Suhr, H. G. Jung, and M. Sunwoo, Precise localization of an autonomous car based on probabilistic noise models of road surface marker features using multiple cameras, IEEE Trans. Intell. Transp. Syst. 16, 3377 (2015).
  37. M. S. Grewal and A. P. Andrews, Applications of Kalman Filtering in aerospace 1960 to the present (Historical perspectives), IEEE Control Syst. Mag. 30, 69 (2010).
  38. I. Arasaratnam and S. Haykin, Cubature Kalman filters, IEEE Trans. Automat. Contr. 54, 1254 (2009).
  39. C. W. Gardiner, Handbook of Stochastic Methods for Physics, Chemistry and the Natural Sciences, Springer Series in Synergetics, Vol. 13, 3rd ed. (Springer-Verlag, Berlin, 2004), p. xviii+415.
  40. K. Dilcher, Kalman filtering for atomic sensors, https://github.com/QI2-lab/kalman-filtering-for-atomic-sensors (2024).
  41. A. Fabricant, I. Novikova, and G. Bison, How to build a magnetometer with thermal atomic vapor: A tutorial, New J. Phys. 25, 025001 (2023).
  42. C. Troullinou, R. Jiménez-Martínez, J. Kong, V. G. Lucivero, and M. W. Mitchell, Squeezed-light enhancement and backaction evasion in a high sensitivity optically pumped magnetometer, Phys. Rev. Lett. 127, 193601 (2021).
  43. D. Manzano, A short introduction to the lindblad master equation, AIP Adv. 10, 025106 (2020).
  44. L. Pezzè, A. Smerzi, M. K. Oberthaler, R. Schmied, and P. Treutlein, Quantum metrology with nonclassical states of atomic ensembles, Rev. Mod. Phys. 90, 035005 (2018).
  45. K. Mouloudakis, G. Vasilakis, V. G. Lucivero, J. Kong, I. K. Kominis, and M. W. Mitchell, Effects of spin-exchange collisions on the fluctuation spectra of hot alkali-metal vapors, Phys. Rev. A 106, 023112 (2022).
  46. I. M. Savukov and M. V. Romalis, Effects of spin-exchange collisions in a high-density alkali-metal vapor in low magnetic fields, Phys. Rev. A 71, 023405 (2005).
  47. J. Delpy, S. Liu, P. Neveu, C. Roussy, T. Jolicoeur, F. Bretenaker, and F. Goldfarb, Creation and dynamics of spin fluctuations in a noisy magnetic field, New J. Phys. 25, 093055 (2023).
  48. W. Happer and B. S. Mathur, Effective operator formalism in optical pumping, Phys. Rev. 163, 12 (1967).
  49. L. Magrini, P. Rosenzweig, C. Bach, A. Deutschmann-Olek, S. G. Hofer, S. Hong, N. Kiesel, A. Kugi, and M. Aspelmeyer, Real-time optimal quantum control of mechanical motion at room temperature, Nature (London) 595, 373 (2021).
  50. M. Koźbiał, L. Elson, L. M. Rushton, A. Akbar, A. Meraki, K. Jensen, and J. Kołodyński, Spin noise spectroscopy of an alignment-based atomic magnetometer, Phys. Rev. A 110, 013125 (2024).
  51. S. Särkkä and A. Solin, Applied Stochastic Differential Equations, Institute of Mathematical Statistics Textbooks (Cambridge University Press, United Kingdom, 2019).
  52. P. E. Kloeden and E. Platen, Numerical Solution of Stochastic Differential Equations, Stochastic Modelling and Applied Probability, Vol. 23 (Springer, New York, 1992).
  53. A. Rößler, Runge–Kutta methods for the strong approximation of solutions of stochastic differential equations, SIAM J. Numer. Anal. 48, 922 (2010).
  54. M. D. Kuznetsov and D. F. Kuznetsov, Implementation of strong numerical methods of orders 0.5, 1.0, 1.5, 2.0, 2.5, and 3.0 for Itô Sdes with multidimensional non-commutative noise based on the unified Taylor–Itô and Taylor–Stratonovich expansions and multiple Fourier–Legendre series, Electron. J. Differ. Equations Control Processes 93 (2021), https://diffjournal.spbu.ru/EN/numbers/2021.1/article.1.5.html.
  55. S. M. Kay, Fundamentals of Statistical Signal Processing: Estimation Theory (Prentice Hall, Englewood Cliffs, NJ, 1993).
  56. C. Fritsche, E. Özkan, L. Svensson, and F. Gustafsson, A fresh look at Bayesian Cramér-Rao bounds for discrete-time nonlinear filtering, in 17th International Conference on Information Fusion (FUSION) (IEEE, New York, 2014), pp. 1–8.
  57. L. Ljung, System Identification: Theory for the User, Prentice Hall Information and System Sciences Series (Prentice Hall PTR, 1999).
  58. T. Söderström and P. Stoica, System identification, Prentice-Hall International Series in Systems and Control Engineering (Prentice Hall, Englewood Cliffs, NJ, 1989).
  59. P. Bania and J. Baranowski, Field Kalman filter and its approximation, in 2016 IEEE 55th Conference on Decision and Control (CDC) (IEEE, New York, 2016), pp. 2875–2880, https://ieeexplore.ieee.org/document/7798697.
  60. P. Bania and J. Baranowski, Bayesian estimator of a faulty state: Logarithmic odds approach, in 2017 22nd International Conference on Methods and Models in Automation and Robotics (MMAR) (IEEE, New York, 2017), pp. 253–257, https://ieeexplore.ieee.org/abstract/document/8046834.
  61. J. Nocedal and S. J. Wright, Numerical Optimization, 2nd ed. (Springer, New York, NY, USA, 2006).
  62. A. W. van der Vaart, Asymptotic Statistics (Cambridge University Press, Cambridge, England, 1998).
  63. S. J. Julier and J. K. Uhlmann, Unscented filtering and nonlinear estimation, Proc. IEEE 92, 401 (2004).
  64. S. Särkkä and A. Solin, On continuous-discrete cubature Kalman filtering, IFAC Proc. 45, 1221 (2012).
  65. D. Rife and R. Boorstyn, Single tone parameter estimation from discrete-time observations, IEEE Trans. Inf. Theory 20, 591 (1974).
  66. M. Lipka, A. Sierant, C. Troullinou, and M. W. Mitchell, Multiparameter quantum sensing and magnetic communication with a hybrid dc and rf optically pumped magnetometer, Phys. Rev. Appl. 21, 034054 (2024).
  67. Y. Wang, X. Jin, Y. Ming, J. Miao, X.-M. Lu, M. W. Mitchell, and J. Kong, Adaptive real-time magnetic field tracking beyond prior waveform constraints, arXiv:2605.17784.
  68. J. Amoros-Binefa, M. W. Mitchell, and J. Kolodynski, Tracking time-varying signals with quantum-enhanced atomic magnetometers, arXiv:2503.14793.
  69. J. Kong, R. Jiménez-Martínez, C. Troullinou, V. G. Lucivero, G. Tóth, and M. W. Mitchell, Measurement-induced, spatially-extended entanglement in a hot, strongly-interacting atomic system, Nat. Commun. 11, 1 (2020).
  70. K. Mouloudakis, J. Kong, A. Sierant, E. Arkin, M. Hernández Ruiz, R. Jiménez-Martínez, and M. W. Mitchell, Anomalous noise spectra in a spin-exchange-relaxation-free alkali-metal vapor, Phys. Rev. A 109, L040802 (2024).
  71. V. B. Braginsky and F. Y. Khalili, Quantum nondemolition measurements: The route from toys to tools, Rev. Mod. Phys. 68, 1 (1996).
  72. M. Tsang and C. M. Caves, Evading quantum mechanics: Engineering a classical subsystem within a quantum environment, Phys. Rev. X 2, 031016 (2012).
  73. A. Kuzmich, N. P. Bigelow, and L. Mandel, Atomic quantum non-demolition measurements and squeezing, Europhys. Lett. 42, 481 (1998).
  74. A. Kuzmich, L. Mandel, and N. P. Bigelow, Generation of spin squeezing via continuous quantum nondemolition measurement, Phys. Rev. Lett. 85, 1594 (2000).
  75. J. Amorós-Binefa and J. Kołodyński, Noisy atomic magnetometry with Kalman filtering and measurement-based feedback, PRX Quantum 6, 030331 (2025).
  76. Z. Q. Zhang, Y. Zhang, H. Z. Guo, C. Shan, G. Chen, and K. Mølmer, Stochastic collective density-matrix approach for conditional spin squeezing, Phys. Rev. A 111, 053715 (2025).
  77. M. P. Ledbetter, V. M. Acosta, S. M. Rochester, D. Budker, S. Pustelny, and V. V. Yashchuk, Detection of radio-frequency magnetic fields using nonlinear magneto-optical rotation, Phys. Rev. A 75, 023405 (2007).
  78. G. Bevilacqua, E. Breschi, and A. Weis, Steady-state solutions for atomic multipole moments in an arbitrarily oriented static magnetic field, Phys. Rev. A 89, 033406 (2014).
  79. S. Liu, P. Neveu, J. Delpy, E. Wu, F. Bretenaker, and F. Goldfarb, Spin-noise spectroscopy of a spin-one system, Phys. Rev. A 107, 023527 (2023).
  80. A. Akbar, M. Koźbiał, L. Elson, A. Meraki, J. Kołodyński, and K. Jensen, Optimized detection modality for radio-frequency sensing with a double-resonance alignment magnetometer, Phys. Rev. Appl. 22, 054033 (2024).
  81. A. Sierant, D. Méndez-Avalos, S. T. Giraldo, and M. W. Mitchell, Quantum noise in a squeezed-light-enhanced multiparameter quantum sensor, arXiv:2506.08190.
  82. S. J. Seltzer and M. V. Romalis, Unshielded three-axis vector operation of a spin-exchange-relaxation-free atomic magnetometer, Appl. Phys. Lett. 85, 4804 (2004).
  83. B. Patton, E. Zhivun, D. C. Hovde, and D. C. Budker, All-optical vector atomic magnetometer, Phys. Rev. Lett. 113, 013001 (2014).
  84. S. J. Ingleby, C. O’Dwyer, P. F. Griffin, A. S. Arnold, and E. Riis, Vector magnetometry exploiting phase-geometry effects in a double-resonance alignment magnetometer, Phys. Rev. Appl. 10, 034035 (2018).
  85. C. R. Lee and Z. Salcic, High-performance FPGA-based implementation of Kalman filter, Microprocess. Microsy. 21, 257 (1997).
  86. V. Bonato, R. Peron, D. F. Wolf, J. A. M. de Holanda, E. Marques, and J. M. P. Cardoso, An FPGA implementation for a Kalman filter with application to mobile robotics, in 2007 International Symposium on Industrial Embedded Systems (IEEE, New York, 2007), pp. 148–155, https://ieeexplore.ieee.org/document/4297329.
  87. Y.-X. Yao and S. M. Pandit, Cramér-Rao lower bounds for a damped sinusoidal process, IEEE Trans. Signal Process. 43, 878 (1995).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation