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    Adiabatic transverse thermoelectric conversion enhanced by heat current manipulation in artificially tilted multilayers

    Fuyuki Ando1,*, Takamasa Hirai1, Hiroto Adachi2, and Ken-ichi Uchida1,3

    • 1Research Center for Magnetic and Spintronic Materials, National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki, 305-0047, Japan
    • 2Research Institute for Interdisciplinary Science, Okayama University, 3-1-1 Tsushimanaka, Kita-ku, Okayama, Okayama, 700-8530, Japan
    • 3Department of Advanced Materials Science, Graduate School of Frontier Sciences, The University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba, 277-8561, Japan

    • *Contact author: ando.fuyuki@nims.go.jp

    Phys. Rev. Applied 23, 064061 – Published 26 June, 2025

    DOI: https://doi.org/10.1103/gqvy-p5p1

    Abstract

    We phenomenologically formulate and experimentally observe an adiabatic transverse thermoelectric conversion enhanced by a heat current reorientation in artificially tilted multilayers (ATMLs). By alternately stacking two materials with different thermal conductivities and rotating the multilayered structure with respect to a longitudinal temperature gradient, we induce off-diagonal components in the thermal conductivity tensor. This off-diagonal thermal conduction (ODTC) generates a finite transverse temperature gradient and Seebeck effect–induced thermopower in the adiabatic condition, which is superposed on the isothermal transverse thermopower driven by the off-diagonal Seebeck effect. In this study, we calculate and observe the two-dimensional temperature distribution and the resultant transverse thermoelectric conversion in ATMLs comprising thermoelectric Co2MnGa Heusler alloys and Bi2−aSbaTe3 compounds. By our changing the tilt angle from 0° to 90°, the transverse temperature gradient obviously appeared in the middle angles and the transverse thermopower increases up to −121.9 µV/K in the Co2MnGa/Bi0.2Sb1.8Te3-based ATML at a tilt angle of 45° whereas the isothermal contribution is estimated to be −82.6 µV/K from the analytical calculation. This hybrid action derived from ODTC results in a significant increase of the maximum reduced conversion efficiency from 3.1% to 8.1% in calculations and from 2.3% to 4.4% in experiments.

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