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    Magneto-optical spectroscopy based on pump-probe strobe light

    Shihao Zhou1, Yujie Zhu2, Chunli Tang3,4, Rui Sun5, Junming Wu1, Yuzan Xiong1,6, Ingrid E. Russell1, Yi Li7, Dali Sun5 et al.

    Frank Tsui1, Binbin Yang6, Valentine Novosad7, Jia-Mian Hu2, Wencan Jin4,3, and Wei Zhang1,*

    • *Contact author: zhwei@unc.edu

    Phys. Rev. Applied 24, 054061 – Published 20 November, 2025

    DOI: https://doi.org/10.1103/dj9z-347y

    Abstract

    We demonstrate a pump-probe strobe light spectroscopy for sensitive detection of magneto-optical dynamics in the context of hybrid magnonics. The technique uses a combinatorial microwave-optical pump-probe scheme, leveraging both the high-energy resolution of microwaves and high-efficiency detection using optical photons. In contrast with conventional stroboscopy using continuous-wave light, we apply microwave and optical pulses with varying pulse widths, and demonstrate magneto-optical detection of magnetization dynamics in Y3Fe5O12 films. The detected magneto-optical signals depend strongly on the characteristics of both the microwave and the optical pulses, as well as their relative time delays. We show that good magneto-optical sensitivity and coherent stroboscopic character are maintained, even at a microwave pump pulse of 1.5 ns and an optical probe pulse of 80 ps, under a 7 MHz clock rate, corresponding to a pump-probe footprint of approximately 1% in one detection cycle. Our results show that time-dependent strobe light measurement of magnetization dynamics can be achieved in the gigahertz frequency range under a pump-probe detection scheme.

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