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  • Letter
  • Open Access

Enhanced multichannel dual-comb spectroscopy of complex systems

Razmik Aramyan*, Oleg Tretiak, and Sushree S. Sahoo

Dmitry Budker

  • *Contact author: aramyanr@uni-mainz.de

Phys. Rev. Applied 24, L021002 – Published 22 August, 2025

DOI: https://doi.org/10.1103/7ktx-4h8m

Abstract

A multichannel dual-comb spectroscopy (DCS) approach for high-resolution, broadband spectral measurements is presented, demonstrating its effectiveness in studying complex atomic systems. By implementing a photodetector array, we enhance DCS capabilities, addressing the fundamental trade-off between signal-to-noise ratio and spectral coverage. To resolve ambiguities in frequency conversion, we introduced a relative offset in beat-note frequency, ensuring accurate spectral reconstruction. As a proof of concept, the absorption spectrum of samarium (Sm) vapor is investigated over a 52-nm range, and several previously unreported absorption lines are detected. This is a step toward “Spectroscopy 2.0,” enabling massively parallel spectroscopic measurements (including those at >100 T magnetic fields) crucial for atomic physics and fundamental interactions research.

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References (19)

  1. M. Safronova et al., Search for new physics with atoms and molecules, Rev. Mod. Phys. 90, 025008 (2018).
  2. A. Kramida et al., (2024). NIST Atomic Spectra Database (version 5.12), [Online]. Available: https://physics.nist.gov/asd. National Institute of Standards and Technology, Gaithersburg, MD. https://doi.org/10.18434/T4W30F.
  3. R. Battesti et al., High magnetic fields for fundamental physics, Phys. Rep. 765766, 1 (2018).
  4. T. W. Hänsch, Nobel lecture: Passion for precision, Rev. Mod. Phys. 78, 1297 (2006).
  5. S. Schiller, Spectrometry with frequency combs, Opt. Lett. 27, 766 (2002).
  6. N. Picqué and T. W. Hänsch, Frequency comb spectroscopy, Nat. Photonics 13, 146 (2019).
  7. I. Coddington, N. Newbury, and W. Swann, Dual-comb spectroscopy, Optica 3, 414 (2016).
  8. E. Baumann et al., Spectroscopy of the methane ν3 band with an accurate midinfrared coherent dual-comb spectrometer, Phys. Rev. A 84, 062513 (2011).
  9. Z. Wei et al., The development and application of dual-comb spectroscopy in analytical chemistry, Chin. Chem. Lett. 34, 107254 (2023).
  10. N. R. Newbury et al., Sensitivity of coherent dual-comb spectroscopy, Opt. Express 18, 7929 (2010).
  11. Y. Sugiyama et al., Precision dual-comb spectroscopy using wavelength-converted frequency combs with low repetition rates, Sci. Rep. 13, 2549 (2023).
  12. O. Tretiak et al., Improved bounds on ultralight scalar dark matter in the radio-frequency range, Phys. Rev. Lett. 129, 031301 (2022).
  13. See Supplemental Material at http://link.aps.org/supplemental/10.1103/7ktx-4h8m for high-resolution plots of the spectrum.
  14. C. Ferrara et al., Experimental atomic data of spectral lines - I. Cs, Ba, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, Lu, Hf, Re, and Os in the 370–1000 nm interval, Mon. Not. R. Astron. Soc. 527, 4440 (2023).
  15. W. Martin et al., Atomic Energy Levels - The Rare-Earth Elements: The Spectra of Lanthanum, Cerium, Praseodymium, Neodymium, Promethium, Samarium, Europium, Gadolinium, Terbium, Dysprosium, Holmium, Erbium, Thulium, Ytterbium, and Lutetium, Nat. Stand. Ref. Data Ser., Nat. Bur. Stand. (U.S.) 60, 422 (1978).
  16. W. F. Meggers et al., Tables of Spectral-Line Intensities: Part 1- Arranged by Elements, Nat. Bur. Stand. (U.S.), Monogr. 145, 403 (1975).
  17. L. Barkov et al., Study of the 4f66s27F→4f66s25D forbidden transitions of atomic samarium, Opt. Spectrosc. (USSR) 66, 288 (1989).
  18. B. Hervieu et al., Cryogenic design of the 43 T LNCMI Grenoble hybrid magnet, Phys. Procedia 67, 692 (2015).
  19. J. Beard et al., Design and tests of the 100-T triple coil at LNCMI, IEEE Trans. Appl. Supercond. 28, 1 (2018).

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