- Open Access
Fault-tolerant encoding of logical qudits in spin systems
Phys. Rev. A 113, 042439 – Published 16 April, 2026
DOI: https://doi.org/10.1103/n28j-r8bg
Abstract
Universal quantum computers require fault-tolerant logical qudits, as qudits naturally align with the simulation of multilevel physical systems. Here we present a general framework and working examples for encoding fault-tolerant logical qudits in finite-dimensional spin systems. We construct distance-3 codewords, distance-5 codewords, and general ()-distance codes that can be implemented using a single physical qudit or a small number of coupled qudits for higher distances while requiring a Hilbert-space dimension significantly smaller than conventional constructions based on multiple logical qubits. Logical operations and error-correction protocols can be implemented with polynomial scaling in the number of elementary operations. We further discuss schematic designs for physical implementation and required single-gate fidelities, which are compatible with current spin qudit platforms. This strategy provides a resource-efficient path toward realizing fault-tolerant logical qudits in finite multilevel physical systems.
Physics Subject Headings (PhySH)
Article Text
References (80)
- P. W. Shor, Polynomial-time algorithms for prime factorization and discrete logarithms on a quantum computer, SIAM Rev. 41, 303 (1999).
- L. M. Vandersypen, M. Steffen, G. Breyta, C. S. Yannoni, M. H. Sherwood, and I. L. Chuang, Experimental realization of Shor's quantum factoring algorithm using nuclear magnetic resonance, Nature (London) 414, 883 (2001).
- L. K. Grover, Proceedings of the 28th Annual ACM Symposium on Theory of Computing, Philadelphia, 1996 (ACM, New York, 1996), pp. 212–219.
- I. L. Chuang, N. Gershenfeld, and M. Kubinec, Experimental implementation of fast quantum searching, Phys. Rev. Lett. 80, 3408 (1998).
- D. G. Cory, A. F. Fahmy, and T. F. Havel, Ensemble quantum computing by NMR spectroscopy, Proc. Natl. Acad. Sci. USA 94, 1634 (1997).
- R. P. Feynman, Simulating physics with computers, Int. J. Theor. Phys. 21, 467 (1982).
- S. Lloyd, Universal quantum simulators, Science 273, 1073 (1996).
- A. Aspuru-Guzik, A. D. Dutoi, P. J. Love, and M. Head-Gordon, Simulated quantum computation of molecular energies, Science 309, 1704 (2005).
- C. L. Degen, F. Reinhard, and P. Cappellaro, Quantum sensing, Rev. Mod. Phys. 89, 035002 (2017).
- F. Dolde, M. W. Doherty, J. Michl, I. Jakobi, B. Naydenov, S. Pezzagna, J. Meijer, P. Neumann, F. Jelezko, N. B. Manson, and J. Wrachtrup, Nanoscale detection of a single fundamental charge in ambient conditions using the center in diamond, Phys. Rev. Lett. 112, 097603 (2014).
- J. Clarke and F. K. Wilhelm, Superconducting quantum bits, Nature (London) 453, 1031 (2008).
- C. H. Bennett and G. Brassard, Quantum cryptography: Public key distribution and coin tossing, Theor. Comput. Sci. 560, 7 (2014).
- M. Chizzini, F. Tacchino, A. Chiesa, I. Tavernelli, S. Carretta, and P. Santini, Qudit-based quantum simulation of fermionic systems, Phys. Rev. A 110, 062602 (2024).
- E. T. Campbell, Enhanced fault-tolerant quantum computing in -level systems, Phys. Rev. Lett. 113, 230501 (2014).
- M. Chizzini, L. Crippa, A. Chiesa, F. Tacchino, F. Petiziol, I. Tavernelli, P. Santini, and S. Carretta, Molecular nanomagnets with competing interactions as optimal units for qudit-based quantum computation, Phys. Rev. Res. 4, 043135 (2022).
- R. J. MacDonell, C. E. Dickerson, C. J. Birch, A. Kumar, C. L. Edmunds, M. J. Biercuk, C. Hempel, and I. Kassal, Analog quantum simulation of chemical dynamics, Chem. Sci. 12, 9794 (2021).
- F. Turro, I. A. Chernyshev, R. Bhaskar, and M. Illa, Qutrit and qubit circuits for three-flavor collective neutrino oscillations, Phys. Rev. D 111, 043038 (2025).
- N. Ticea, E. Portoles, E. Rosenberg, A. Schuckert, A. Szasz, B. Kobrin, N. Pomata, P. Praneel, C. Miao, S. Kumar, et al., Observation of disorder-induced superfluidity, arXiv:2512.21416.
- S. Lim, J. Liu, and A. Ardavan, Fault-tolerant qubit encoding using a spin-7/2 qudit, Phys. Rev. A 108, 062403 (2023).
- D. Janković, J.-G. Hartmann, M. Ruben, and P.-A. Hervieux, Noisy qudit vs multiple qubits: Conditions on gate efficiency for enhancing fidelity, npj Quantum Inf. 10, 59 (2024).
- X. Gao, P. Appel, N. Friis, M. Ringbauer, and M. Huber, On the role of entanglement in qudit-based circuit compression, Quantum 7, 1141 (2023).
- N. P. Sawaya, T. Menke, T. H. Kyaw, S. Johri, A. Aspuru-Guzik, and G. G. Guerreschi, Resource-efficient digital quantum simulation of -level systems for photonic, vibrational, and spin- Hamiltonians, npj Quantum Inf. 6, 49 (2020).
- H. Bechmann-Pasquinucci and A. Peres, Quantum cryptography with 3-state systems, Phys. Rev. Lett. 85, 3313 (2000).
- N. J. Cerf, M. Bourennane, A. Karlsson, and N. Gisin, Security of quantum key distribution using -level systems, Phys. Rev. Lett. 88, 127902 (2002).
- D. Cozzolino, B. Da Lio, D. Bacco, and L. K. Oxenløwe, High-dimensional quantum communication: Benefits, progress, and future challenges, Adv. Quantum Technol. 2, 1900038 (2019).
- J. Preskill, Quantum computing in the NISQ era and beyond, Quantum 2, 79 (2018).
- R. F. Uy and D. A. Gangloff, Qudit-based quantum error-correcting codes from irreducible representations of SU(), Phys. Rev. A 112, 042402 (2025).
- B. L. Brock, S. Singh, A. Eickbusch, V. V. Sivak, A. Z. Ding, L. Frunzio, S. M. Girvin, and M. H. Devoret, Quantum error correction of qudits beyond break-even, Nature (London) 641, 612 (2025).
- M. H. Michael, M. Silveri, R. T. Brierley, V. V. Albert, J. Salmilehto, L. Jiang, and S. M. Girvin, New class of quantum error-correcting codes for a bosonic mode, Phys. Rev. X 6, 031006 (2016).
- Y. Ouyang, Permutation-invariant qudit codes from polynomials, Linear Algebra Appl. 532, 43 (2017).
- P. Mazurek, M. Farkas, A. Grudka, M. Horodecki, and M. Studziński, Quantum error-correction codes and absolutely maximally entangled states, Phys. Rev. A 101, 042305 (2020).
- F. Schmidt and P. van Loock, Quantum error correction with higher Gottesman-Kitaev-Preskill codes: Minimal measurements and linear optics, Phys. Rev. A 105, 042427 (2022).
- S. Dutta, D. Biswas, and P. Mandayam, Noise-adapted qudit codes for amplitude-damping noise, Phys. Rev. A 111, 032438 (2025).
- E. Knill, R. Laflamme, and W. H. Zurek, Resilient quantum computation, Science 279, 342 (1998).
- R. Laflamme, C. Miquel, J. P. Paz, and W. H. Zurek, Perfect quantum error correcting code, Phys. Rev. Lett. 77, 198 (1996).
- E. Knill and R. Laflamme, Theory of quantum error-correcting codes, Phys. Rev. A 55, 900 (1997).
- Google Quantum AI, Suppressing quantum errors by scaling a surface code logical qubit, Nature (London) 614, 676 (2023).
- D. Gottesman, A. Kitaev, and J. Preskill, Encoding a qubit in an oscillator, Phys. Rev. A 64, 012310 (2001).
- L. Hu, Y. Ma, W. Cai, X. Mu, Y. Xu, W. Wang, Y. Wu, H. Wang, Y. Song, C.-L. Zou, et al., Quantum error correction and universal gate set operation on a binomial bosonic logical qubit, Nat. Phys. 15, 503 (2019).
- S. Lim, M. V. Vaganov, J. Liu, and A. Ardavan, Demonstrating experimentally the encoding and dynamics of an error-correctable logical qubit on a hyperfine-coupled nuclear spin qudit, Phys. Rev. Lett. 134, 070603 (2025).
- X. Yu, B. Wilhelm, D. Holmes, A. Vaartjes, D. Schwienbacher, M. Nurizzo, A. Kringhøj, M. R. van Blankenstein, A. M. Jakob, P. Gupta, et al., Schrödinger cat states of a nuclear spin qudit in silicon, Nat. Phys. 21, 362 (2025).
- Y. Yang, W.-T. Luo, J.-L. Zhang, S.-Z. Wang, C.-L. Zou, T. Xia, and Z.-T. Lu, Minute-scale Schrödinger-cat state of spin-5/2 atoms, Nat. Photonics 19, 89 (2025).
- J. A. Gross, Designing codes around interactions: The case of a spin, Phys. Rev. Lett. 127, 010504 (2021).
- S. Omanakuttan and J. A. Gross, Multispin clifford codes for angular momentum errors in spin systems, Phys. Rev. A 108, 022424 (2023).
- S. Omanakuttan, V. Buchemmavari, J. A. Gross, I. H. Deutsch, and M. Marvian, Fault-tolerant quantum computation using large spin-cat codes, PRX Quantum 5, 020355 (2024).
- S. Omanakuttan, A. Mitra, E. J. Meier, M. J. Martin, and I. H. Deutsch, Qudit entanglers using quantum optimal control, PRX Quantum 4, 040333 (2023).
- A. Chiesa, E. Macaluso, F. Petiziol, S. Wimberger, P. Santini, and S. Carretta, Molecular nanomagnets as qubits with embedded quantum-error correction, J. Phys. Chem. Lett. 11, 8610 (2020).
- S. J. Lockyer, A. Chiesa, G. A. Timco, E. J. McInnes, T. S. Bennett, I. J. Vitorica-Yrezebal, S. Carretta, and R. E. Winpenny, Targeting molecular quantum memory with embedded error correction, Chem. Sci. 12, 9104 (2021).
- S. Carretta, D. Zueco, A. Chiesa, Á. Gómez-León, and F. Luis, A perspective on scaling up quantum computation with molecular spins, Appl. Phys. Lett. 118, 240501 (2021).
- S. Lim and A. Ardavan, Designing quantum error correction codes for practical spin qudit systems, Phys. Rev. A 112, 022418 (2025).
- I. Fernández de Fuentes, T. Botzem, M. A. Johnson, A. Vaartjes, S. Asaad, V. Mourik, F. E. Hudson, K. M. Itoh, B. C. Johnson, A. M. Jakob, J. C. McCallum, D. N. Jamieson, A. S. Dzurak, and A. Morello, Navigating the 16-dimensional Hilbert space of a high-spin donor qudit with electric and magnetic fields, Nat. Commun. 15, 1380 (2024).
- S. Takahashi, J. van Tol, C. C. Beedle, D. N. Hendrickson, L.-C. Brunel, and M. S. Sherwin, Coherent manipulation and decoherence of S = 10 single-molecule magnets, Phys. Rev. Lett. 102, 087603 (2009).
- Z. Liu, B.-W. Dong, H.-B. Meng, M.-X. Xu, T.-S. Wang, B.-W. Wang, C.-R. Wang, S.-D. Jiang, and S. Gao, Qubit crossover in the endohedral fullerene @, Chem. Sci. 9, 457 (2018).
- V. V. Albert, J. P. Covey, and J. Preskill, Robust encoding of a qubit in a molecule, Phys. Rev. X 10, 031050 (2020).
- S. P. Jain, E. R. Hudson, W. C. Campbell, and V. V. Albert, Absorption-emission codes for atomic and molecular quantum information platforms, Phys. Rev. Lett. 133, 260601 (2024).
- M. J. Boguslawski, Z. J. Wall, S. R. Vizvary, I. D. Moore, M. Bareian, D. T. C. Allcock, D. J. Wineland, E. R. Hudson, and W. C. Campbell, Raman scattering errors in stimulated-Raman-induced logic gates in , Phys. Rev. Lett. 131, 063001 (2023).
- X. Yu, J. Mo, T. Lu, T. Y. Tan, and T. L. Nicholson, Magneto-optical trapping of a group-III atom, Phys. Rev. A 105, L061101 (2022).
- A. M. Yao and M. J. Padgett, Orbital angular momentum: Origins, behavior and applications, Adv. Opt. Photon. 3, 161 (2011).
- B. Kim, K.-M. Hu, M.-H. Sohn, Y. Kim, Y.-S. Kim, S.-W. Lee, and H.-T. Lim, Qudit-based variational quantum eigensolver using photonic orbital angular momentum states, Sci. Adv. 10, eado3472 (2024).
- Z. Leghtas, G. Kirchmair, B. Vlastakis, R. J. Schoelkopf, M. H. Devoret, and M. Mirrahimi, Hardware-efficient autonomous quantum memory protection, Phys. Rev. Lett. 111, 120501 (2013).
- N. Ofek, A. Petrenko, R. Heeres, P. Reinhold, Z. Leghtas, B. Vlastakis, Y. Liu, L. Frunzio, S. M. Girvin, L. Jiang, et al., Extending the lifetime of a quantum bit with error correction in superconducting circuits, Nature (London) 536, 441 (2016).
- Z. Ni, S. Li, X. Deng, Y. Cai, L. Zhang, W. Wang, Z.-B. Yang, H. Yu, F. Yan, S. Liu, et al., Beating the break-even point with a discrete-variable-encoded logical qubit, Nature (London) 616, 56 (2023).
- L. Li, D. J. Young, V. V. Albert, K. Noh, C.-L. Zou, and L. Jiang, Phase-engineered bosonic quantum codes, Phys. Rev. A 103, 062427 (2021).
- S. Pirandola, S. Mancini, S. L. Braunstein, and D. Vitali, Minimal qudit code for a qubit in the phase-damping channel, Phys. Rev. A 77, 032309 (2008).
- G. K. Brennen, D. P. O'Leary, and S. S. Bullock, Criteria for exact qudit universality, Phys. Rev. A 71, 052318 (2005).
- Y. Wang, Z. Hu, B. C. Sanders, and S. Kais, Qudits and high-dimensional quantum computing, Front. Phys. 8, 589504 (2020).
- M. Rubín-Osanz, L. Bersani, S. Chicco, G. Allodi, R. De Renzi, A. Mavromagoulos, M. D. Roy, S. Piligkos, E. Garlatti, and S. Carretta, Implementation of the quantum Fourier transform on a molecular qudit with full refocusing and state tomography, arXiv:2512.15611.
- S. Chicco, G. Allodi, A. Chiesa, E. Garlatti, C. D. Buch, P. Santini, R. De Renzi, S. Piligkos, and S. Carretta, Proof-of-concept quantum simulator based on molecular spin qudits, J. Am. Chem. Soc. 146, 1053 (2024).
- B. E. Kane, A silicon-based nuclear spin quantum computer, Nature (London) 393, 133 (1998).
- H. G. Stemp, M. R. van Blankenstein, S. Asaad, M. T. Mądzik, B. Joecker, H. R. Firgau, A. Laucht, F. E. Hudson, A. S. Dzurak, K. M. Itoh, et al., Scalable entanglement of nuclear spins mediated by electron exchange, Science 389, 1234 (2025).
- M. N. Leuenberger and D. Loss, Quantum computing in molecular magnets, Nature (London) 410, 789 (2001).
- M. Murugesu, S. Takahashi, A. Wilson, K. A. Abboud, W. Wernsdorfer, S. Hill, and G. Christou, Large single-molecule magnet with spin = 51/2: Magnetic and high-frequency electron paramagnetic resonance spectroscopic characterization of a giant spin state, Inorg. Chem. 47, 9459 (2008).
- J. Rahmer, L. Dunsch, H. Dorn, J. Mende, and M. Mehring, W- and X-band EPR investigation of @, Magn. Reson. Chem. 43, S192 (2005).
- E. O. Kiktenko, A. S. Nikolaeva, and A. K. Fedorov, Colloquium: Qudits for decomposing multiqubit gates and realizing quantum algorithms, Rev. Mod. Phys. 97, 021003 (2025).
- L. E. Fischer, A. Chiesa, F. Tacchino, D. J. Egger, S. Carretta, and I. Tavernelli, Universal qudit gate synthesis for transmons, PRX Quantum 4, 030327 (2023).
- P. Rambow and M. Tian, Reduction of circuit depth by mapping qubit-based quantum gates to a qudit basis, arXiv:2109.09902.
- M. Onizhuk and G. Galli, Colloquium: Decoherence of solid-state spin qubits: A computational perspective, Rev. Mod. Phys. 97, 021001 (2025).
- J. Yoneda, K. Takeda, T. Otsuka, T. Nakajima, M. R. Delbecq, G. Allison, T. Honda, T. Kodera, S. Oda, Y. Hoshi, et al., A quantum-dot spin qubit with coherence limited by charge noise and fidelity higher than 99.9%, Nat. Nanotechnol. 13, 102 (2018).
- A. Noiri, K. Takeda, T. Nakajima, T. Kobayashi, A. Sammak, G. Scappucci, and S. Tarucha, Fast universal quantum gate above the fault-tolerance threshold in silicon, Nature (London) 601, 338 (2022).
- A. deMarti iOlius, P. Fuentes, R. Orús, P. M. Crespo, and J. E. Martinez, Decoding algorithms for surface codes, Quantum 8, 1498 (2024).