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  • Open Access

Exploring vibronic dynamics near a sloped conical intersection with trapped Rydberg ions

Abdessamad Belfakir1 and Weibin Li2

  • 1The UM6P Vanguard Center, Mohammed VI Polytechnic University (UM6P), Rocade Rabat-Salé, Technopolis, 11103, Morocco
  • 2School of Physics and Astronomy, and Centre for the Mathematics and Theoretical Physics of Quantum Non-equilibrium Systems, University of Nottingham, Nottingham NG7 2RD, United Kingdom

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Phys. Rev. A 113, 023323 – Published 26 February, 2026

DOI: https://doi.org/10.1103/fp53-6k62

Abstract

We study spin-phonon coupled dynamics in the vicinity of a sloped conical intersection created by laser coupling the electronic (spin) and vibrational degrees of freedom of a pair of trapped Rydberg ions. We show that the shape of the potential energy surfaces can be engineered and controlled by exploiting the sideband transitions of the crystal vibration and dipole-dipole interactions between Rydberg ions in the Lamb-Dicke regime. Using the sideband transition, we realize a sloped conical intersection whose cone axis is only tilted along one spatial axis. When the phonon wave packet is located in the minimum of the lower potential surface, the spin and phonon dynamics are largely frozen owing to the geometric phase effect. When starting from the upper potential surface, the electronic and phonon states tunnel to the lower potential surface, leading to a partial revival of the initial state. In contrast, the dynamics drastically change when the initial wave packets are away from the conical intersection. The initial state is revived, and it is almost entirely irrelevant whether it is from the lower or upper potential surface. Complete Rabi oscillations of the adiabatic states are found when the wave packet is initialized on the upper potential surface. The dynamics occur on the microsecond and nanometer scales, implying that Rydberg ions provide a platform for simulating nonadiabatic processes in the vicinity of a sloped conical intersection.

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Phys. Rev. A 113, 023323– Published 26 February, 2026
  • Received 11 December 2025
  • Accepted 9 February 2026
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