- Open Access
Detecting high-dimensional time-bin entanglement in fiber-loop systems
Phys. Rev. A 112, 012410 – Published 11 July, 2025
DOI: https://doi.org/10.1103/bn8s-bqnp
Abstract
Many quantum communication protocols rely on the distribution of entanglement between the different participating parties. One example is quantum key distribution (QKD), an application that has matured to commercial use in recent years. However, difficulties remain, especially with noise resilience and channel capacity in long-distance communication. One way to overcome these problems is to use high-dimensional entanglement, which has been shown to be more robust to noise and enables higher secret-key rates. It is therefore important to have access to certifiable high-dimensional entanglement sources to confidently implement these advanced QKD protocols. Here we develop a method for certifying high-dimensional time-bin entanglement in fiber-loop systems. In these systems, entanglement creation and detection can utilize the same physical components, and the number of time bins, and thus the entanglement dimension, can be adapted without making physical changes to the setup. Our certification method builds on previous proposals for the certification of angular-momentum entanglement in photon pairs. In particular, measurements in only two experimentally accessible bases are sufficient to obtain a lower bound on the entanglement dimension for both two- and multiphoton quantum states. Numerical simulations show that the method is robust against typical experimental noise effects and works well even with limited measurement statistics, thus establishing time-bin encoded photons as a promising platform for high-dimensional quantum-communication protocols.
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References (83)
- J. L. O'Brien, A. Furusawa, and J. Vučković, Photonic quantum technologies, Nat. Photon. 3, 687 (2009).
- F. Flamini, N. Spagnolo, and F. Sciarrino, Photonic quantum information processing: A review, Rep. Prog. Phys. 82, 016001 (2019).
- S. Slussarenko and G. J. Pryde, Photonic quantum information processing: A concise review, Appl. Phys. Rev. 6, 041303 (2019).
- E. Pelucchi, G. Fagas, I. Aharonovich, D. Englund, E. Figueroa, Q. Gong, H. Hannes, J. Liu, C.-Y. Lu, N. Matsuda, J.-W. Pan, F. Schreck, F. Sciarrino, C. Silberhorn, J. Wang, and K. D. Jöns, The potential and global outlook of integrated photonics for quantum technologies, Nat. Rev. Phys. 4, 194 (2022).
- A. Aspuru-Guzik and P. Walther, Photonic quantum simulators, Nat. Phys. 8, 285 (2012).
- M. J. Hartmann, Quantum simulation with interacting photons, J. Opt. 18, 104005 (2016).
- S. Pirandola, J. Eisert, C. Weedbrook, A. Furusawa, and S. L. Braunstein, Advances in quantum teleportation, Nat. Photon. 9, 641 (2015).
- D. Llewellyn, Y. Ding, I. I. Faruque, S. Paesani, D. Bacco, R. Santagati, Y.-J. Qian, Y. Li, Y.-F. Xiao, M. Huber, M. Malik, G. F. Sinclair, X. Zhou, K. Rottwitt, J. L. O'Brien, J. G. Rarity, Q. Gong, L. K. Oxenlowe, J. Wang, and M. G. Thompson, Chip-to-chip quantum teleportation and multi-photon entanglement in silicon, Nat. Phys. 16, 148 (2020).
- E. Knill, R. Laflamme, and G. J. Milburn, A scheme for efficient quantum computation with linear optics, Nature 409, 46 (2001).
- M. A. Nielsen, Optical quantum computation using cluster states, Phys. Rev. Lett. 93, 040503 (2004).
- H.-S. Zhong, H. Wang, Y.-H. Deng, M.-C. Chen, L.-C. Peng, Y.-H. Luo, J. Qin, D. Wu, X. Ding, Y. Hu, P. Hu, X.-Y. Yang, W.-J. Zhang, H. Li, Y. Li, X. Jiang, L. Gan, G. Yang, L. You, Z. Wang et al., Quantum computational advantage using photons, Science 370, 1460 (2020).
- J. E. Bourassa, R. N. Alexander, M. Vasmer, A. Patil, I. Tzitrin, T. Matsuura, D. Su, B. Q. Baragiola, S. Guha, G. Dauphinais, K. K. Sabapathy, N. C. Menicucci, and I. Dhand, Blueprint for a scalable photonic fault-tolerant quantum computer, Quantum 5, 392 (2021).
- L. S. Madsen, F. Laudenbach, M. F. Askarani, F. Rortais, T. Vincent, J. F. F. Bulmer, F. M. Miatto, L. Neuhaus, L. G. Helt, M. J. Collins, A. E. Lita, T. Gerrits, S. W. Nam, V. D. Vaidya, M. Menotti, I. Dhand, Z. Vernon, N. Quesada, and J. Lavoie, Quantum computational advantage with a programmable photonic processor, Nature 606, 75 (2022).
- C. Couteau, S. Barz, T. Durt, T. Gerrits, J. Huwer, R. Prevedel, J. Rarity, A. Shields, and G. Weihs, Applications of single photons to quantum communication and computing, Nat. Rev. Phys. 5, 326 (2023).
- C. H. Bennett and G. Brassard, Quantum cryptography: Public key distribution and coin tossing, Theor. Comput. Sci. 560, 7 (2014).
- N. Gisin, G. Ribordy, W. Tittel, and H. Zbinden, Quantum cryptography, Rev. Mod. Phys. 74, 145 (2002).
- N. Gisin and R. Thew, Quantum communication, Nat. Photon. 1, 165 (2007).
- N. Gisin and R. Thew, Quantum communication technology, Electron. Lett. 46, 965 (2010).
- H.-K. Lo, M. Curty, and K. Tamaki, Secure quantum key distribution, Nat. Photon. 8, 595 (2014).
- S. Pirandola, U. L. Andersen, L. Banchi, M. Berta, D. Bunandar, R. Colbeck, D. Englund, T. Gehring, C. Lupo, C. Ottaviani, J. L. Pereira, M. Razavi, J. S. Shaari, M. Tomamichel, V. C. Usenko, G. Vallone, P. Villoresi, and P. Wallden, Advances in quantum cryptography, Adv. Opt. Photon. 12, 1012 (2020).
- W. Luo, L. Cao, Y. Shi, L. Wan, H. Zhang, S. Li, G. Chen, Y. Li, S. Li, Y. Wang, S. Sun, M. F. Karim, H. Cai, L. C. Kwek, and A. Q. Liu, Recent progress in quantum photonic chips for quantum communication and internet, Light Sci. Appl. 12, 175 (2023).
- R. C. Johnson, Quantum-key encryption system ships, EE Times (2003), https://www.eetimes.com/quantum-key-encryption-system-ships/.
- A. Acín, N. Brunner, N. Gisin, S. Massar, S. Pironio, and V. Scarani, Device-independent security of quantum cryptography against collective attacks, Phys. Rev. Lett. 98, 230501 (2007).
- R. Schwonnek, K. T. Goh, I. W. Primaatmaja, E. Y.-Z. Tan, R. Wolf, V. Scarani, and C. C.-W. Lim, Device-independent quantum key distribution with random key basis, Nat. Commun. 12, 2880 (2021).
- V. Zapatero, T. van Leent, R. Arnon-Friedman, W.-Z. Liu, Q. Zhang, H. Weinfurter, and M. Curty, Advances in device-independent quantum key distribution, npj Quantum Inf. 9, 10 (2023).
- P. Brown, H. Fawzi, and O. Fawzi, Computing conditional entropies for quantum correlations, Nat. Commun. 12, 575 (2021).
- E. Woodhead, A. Acín, and S. Pironio, Device-independent quantum key distribution with asymmetric CHSH inequalities, Quantum 5, 443 (2021).
- V. Zapatero and M. Curty, Long-distance device-independent quantum key distribution, Sci. Rep. 9, 17749 (2019).
- I. Esmaeil Zadeh, J. Chang, J. W. N. Los, S. Gyger, A. W. Elshaari, S. Steinhauer, S. N. Dorenbos, and V. Zwiller, Superconducting nanowire single-photon detectors: A perspective on evolution, state-of-the-art, future developments, and applications, Appl. Phys. Lett. 118, 190502 (2021).
- S. Massar, Nonlocality, closing the detection loophole, and communication complexity, Phys. Rev. A 65, 032121 (2002).
- N. Miklin, A. Chaturvedi, M. Bourennane, M. Pawłowski, and A. Cabello, Exponentially decreasing critical detection efficiency for any Bell inequality, Phys. Rev. Lett. 129, 230403 (2022).
- J. Rivera-Dean, A. Steffinlongo, N. Parker-Sánchez, A. Acín, and E. Oudot, Device-independent quantum key distribution beyond qubits, New J. Phys. 27, 054512 (2025).
- D. Kaszlikowski, P. Gnaciñski, M. Żukowski, W. Miklaszewski, and A. Zeilinger, Violations of local realism by two entangled -dimensional systems are stronger than for two qubits, Phys. Rev. Lett. 85, 4418 (2000).
- D. Collins, N. Gisin, N. Linden, S. Massar, and S. Popescu, Bell inequalities for arbitrarily high-dimensional systems, Phys. Rev. Lett. 88, 040404 (2002).
- T. Durt, N. J. Cerf, N. Gisin, and M. Żukowski, Security of quantum key distribution with entangled qutrits, Phys. Rev. A 67, 012311 (2003).
- T. Durt, D. Kaszlikowski, J.-L. Chen, and L. C. Kwek, Security of quantum key distributions with entangled qudits, Phys. Rev. A 69, 032313 (2004).
- J. Brendel, N. Gisin, W. Tittel, and H. Zbinden, Pulsed energy-time entangled twin-photon source for quantum communication, Phys. Rev. Lett. 82, 2594 (1999).
- A. Schreiber, K. N. Cassemiro, V. Potoček, A. Gábris, P. J. Mosley, E. Andersson, I. Jex, and C. Silberhorn, Photons walking the line: A quantum walk with adjustable coin operations, Phys. Rev. Lett. 104, 050502 (2010).
- T. Nitsche, F. Elster, J. Novotný, A. Gábris, I. Jex, S. Barkhofen, and C. Silberhorn, Quantum walks with dynamical control: Graph engineering, initial state preparation and state transfer, New J. Phys. 18, 063017 (2016).
- Y. He, X. Ding, Z.-E. Su, H.-L. Huang, J. Qin, C. Wang, S. Unsleber, C. Chen, H. Wang, Y.-M. He, X.-L. Wang, W.-J. Zhang, S.-J. Chen, C. Schneider, M. Kamp, L.-X. You, Z. Wang, S. Höfling, C.-Y. Lu, and J.-W. Pan, Time-bin-encoded boson sampling with a single-photon device, Phys. Rev. Lett. 118, 190501 (2017).
- A. Regensburger, C. Bersch, B. Hinrichs, G. Onishchukov, A. Schreiber, C. Silberhorn, and U. Peschel, Photon propagation in a discrete fiber network: An interplay of coherence and losses, Phys. Rev. Lett. 107, 233902 (2011).
- A. Schreiber, A. Gábris, P. P. Rohde, K. Laiho, M. Štefaňák, V. Potoček, C. Hamilton, I. Jex, and C. Silberhorn, A 2D quantum walk simulation of two-particle dynamics, Science 336, 55 (2012).
- K. R. Motes, A. Gilchrist, J. P. Dowling, and P. P. Rohde, Scalable boson sampling with time-bin encoding using a loop-based architecture, Phys. Rev. Lett. 113, 120501 (2014).
- J. Boutari, A. Feizpour, S. Barz, C. D. Franco, M. S. Kim, W. S. Kolthammer, and I. A. Walmsley, Large scale quantum walks by means of optical fiber cavities, J. Opt. 18, 094007 (2016).
- I. Dhand, M. Engelkemeier, L. Sansoni, S. Barkhofen, C. Silberhorn, and M. B. Plenio, Proposal for quantum simulation via all-optically-generated tensor network states, Phys. Rev. Lett. 120, 130501 (2018).
- M. Lubasch, A. A. Valido, J. J. Renema, W. S. Kolthammer, D. Jaksch, M. S. Kim, I. Walmsley, and R. García-Patrón, Tensor network states in time-bin quantum optics, Phys. Rev. A 97, 062304 (2018).
- T. Nitsche, T. Geib, C. Stahl, L. Lorz, C. Cedzich, S. Barkhofen, R. F. Werner, and C. Silberhorn, Eigenvalue measurement of topologically protected edge states in split-step quantum walks, New J. Phys. 21, 043031 (2019).
- I. Marcikic, H. de Riedmatten, W. Tittel, H. Zbinden, M. Legré, and N. Gisin, Distribution of time-bin entangled qubits over 50 km of optical fiber, Phys. Rev. Lett. 93, 180502 (2004).
- L. Yu, C. M. Natarajan, T. Horikiri, C. Langrock, J. S. Pelc, M. G. Tanner, E. Abe, S. Maier, C. Schneider, S. Höfling, M. Kamp, R. H. Hadfield, M. M. Fejer, and Y. Yamamoto, Two-photon interference at telecom wavelengths for time-bin-encoded single photons from quantum-dot spin qubits, Nat. Commun. 6, 8955 (2015).
- A. Boaron, B. Korzh, R. Houlmann, G. Boso, D. Rusca, S. Gray, M.-J. Li, D. Nolan, A. Martin, and H. Zbinden, Simple 2.5 GHz time-bin quantum key distribution, Appl. Phys. Lett. 112, 171108 (2018).
- A. Boaron, G. Boso, D. Rusca, C. Vulliez, C. Autebert, M. Caloz, M. Perrenoud, G. Gras, F. Bussières, M.-J. Li, D. Nolan, A. Martin, and H. Zbinden, Secure quantum key distribution over 421 km of optical fiber, Phys. Rev. Lett. 121, 190502 (2018).
- N. T. Islam, C. C. W. Lim, C. Cahall, B. Qi, J. Kim, and D. J. Gauthier, Scalable high-rate, high-dimensional time-bin encoding quantum key distribution, Quantum Sci. Technol. 4, 035008 (2019).
- F. Bouchard, K. Bonsma-Fisher, K. Heshami, P. J. Bustard, D. England, and B. Sussman, Measuring ultrafast time-bin qudits, Phys. Rev. A 107, 022618 (2023).
- F. Bouchard, K. Fenwick, K. Bonsma-Fisher, D. England, P. J. Bustard, K. Heshami, and B. Sussman, Programmable photonic quantum circuits with ultrafast time-bin encoding, Phys. Rev. Lett. 133, 090601 (2024).
- E. Fitzke, L. Bialowons, T. Dolejsky, M. Tippmann, O. Nikiforov, T. Walther, F. Wissel, and M. Gunkel, Scalable network for simultaneous pairwise quantum key distribution via entanglement-based time-bin coding, PRX Quantum 3, 020341 (2022).
- G. B. Xavier, N. Walenta, G. V. d. Faria, G. P. Temporão, N. Gisin, H. Zbinden, and J. P. v. d. Weid, Experimental polarization encoded quantum key distribution over optical fibres with real-time continuous birefringence compensation, New J. Phys. 11, 045015 (2009).
- C. Antonelli, M. Shtaif, and M. Brodsky, Sudden death of entanglement induced by polarization mode dispersion, Phys. Rev. Lett. 106, 080404 (2011).
- M. Brodsky, E. C. George, C. Antonelli, and M. Shtaif, Loss of polarization entanglement in a fiber-optic system with polarization mode dispersion in one optical path, Opt. Lett. 36, 43 (2011).
- Y.-Y. Ding, H. Chen, S. Wang, D.-Y. He, Z.-Q. Yin, W. Chen, Z. Zhou, G.-C. Guo, and Z.-F. Han, Polarization variations in installed fibers and their influence on quantum key distribution systems, Opt. Express 25, 27923 (2017).
- A. N. Craddock, A. Lazenby, G. B. Portmann, R. Sekelsky, M. Flament, and M. Namazi, Automated distribution of polarization-entangled photons using deployed New York City fibers, PRX Quantum 5, 030330 (2024).
- J. M. Donohue, M. Agnew, J. Lavoie, and K. J. Resch, Coherent Ultrafast measurement of time-bin encoded photons, Phys. Rev. Lett. 111, 153602 (2013).
- M. Monika, F. Nosrati, A. George, S. Sciara, R. Fazili, A. L. Marques Muniz, A. Bisianov, R. Lo Franco, W. J. Munro, M. Chemnitz, U. Peschel, and R. Morandotti, Quantum state processing through controllable synthetic temporal photonic lattices, Nat. Photon. 19, 95 (2025).
- A. Martin, T. Guerreiro, A. Tiranov, S. Designolle, F. Fröwis, N. Brunner, M. Huber, and N. Gisin, Quantifying photonic high-dimensional entanglement, Phys. Rev. Lett. 118, 110501 (2017).
- N. T. Islam, C. C. W. Lim, C. Cahall, J. Kim, and D. J. Gauthier, Provably secure and high-rate quantum key distribution with time-bin qudits, Sci. Adv. 3, e1701491 (2017).
- A. Sanpera, D. Bruß, and M. Lewenstein, Schmidt-number witnesses and bound entanglement, Phys. Rev. A 63, 050301(R) (2001).
- G. Sentís, C. Eltschka, O. Gühne, M. Huber, and J. Siewert, Quantifying entanglement of maximal dimension in bipartite mixed states, Phys. Rev. Lett. 117, 190502 (2016).
- P. Erker, M. Krenn, and M. Huber, Quantifying high dimensional entanglement with two mutually unbiased bases, Quantum 1, 22 (2017).
- J. Bavaresco, N. H. Valencia, C. Klöckl, M. Pivoluska, P. Erker, N. Friis, M. Malik, and M. Huber, Measurements in two bases are sufficient for certifying high-dimensional entanglement, Nat. Phys. 14, 1032 (2018).
- N. Euler and M. Gärttner, Detecting high-dimensional entanglement in cold-atom quantum simulators, PRX Quantum 4, 040338 (2023).
- R. Fickler, R. Lapkiewicz, M. Huber, M. P. J. Lavery, M. J. Padgett, and A. Zeilinger, Interface between path and orbital angular momentum entanglement for high-dimensional photonic quantum information, Nat. Commun. 5, 4502 (2014).
- L. Édouard, Récréations Mathématiques (Gauthier-Villars, Paris, 1883), pp. 176–180.
- Z. Baranyai, On the factorization of the complete uniform hypergraph, in Proceedings of the conference “Colloquium on Infinite and Finite Sets”, Keszthely, Hungary, edited by A. Hajnal, R. Rado, and V. T. Sós (North-Holland Pub. Co, Amsterdam, 1975), pp. 91–108.
- M. A. Nielsen, Conditions for a class of entanglement transformations, Phys. Rev. Lett. 83, 436 (1999).
- H. Takesue and Y. Noguchi, Implementation of quantum state tomography for time-bin entangled photon pairs, Opt. Express 17, 10976 (2009).
- S. Liu, Q. He, M. Huber, O. Gühne, and G. Vitagliano, Characterizing entanglement dimensionality from randomized measurements, PRX Quantum 4, 020324 (2023).
- N. Wyderka and A. Ketterer, Probing the geometry of correlation matrices with randomized measurements, PRX Quantum 4, 020325 (2023).
- O. Lib, S. Liu, R. Shekel, Q. He, M. Huber, Y. Bromberg, and G. Vitagliano, Experimental certification of high-dimensional entanglement withrandomized measurements, Phys. Rev. Lett. 134, 210202 (2025).
- M. I. Estrada-Delgado and Z. Blanco-Garcia, Simulations of quantum walks on beam splitter arrays modeled as higher-order rotations, Eur. Phys. J. Plus 139, 261 (2024).
- K. L. Fenwick, F. Bouchard, G. S. Thekkadath, D. England, P. J. Bustard, K. Heshami, and B. Sussman, Photonic quantum walk with ultrafast time-bin encoding, Optica 11, 1017 (2024).
- S. J. U. White, E. Polino, F. Ghafari, D. J. Joch, L. Villegas-Aguilar, L. K. Shalm, V. B. Verma, M. Huber, and N. Tischler, A robust approach for time-bin encoded photonic quantum information protocols, Phys. Rev. Lett. 134, 180802 (2025).
- N. Euler, NiklasEuler/Detecting-high-dimensional-time-bin- entanglement-in-fiber-loop-systems (2025), https://doi.org/10.5281/zenodo.15528297.
- N. Euler, NiklasEuler/TimeBinEncoding.jl (2025), https://doi.org/10.5281/zenodo.15041186.
- C. K. Hong, Z. Y. Ou, and L. Mandel, Measurement of subpicosecond time intervals between two photons by interference, Phys. Rev. Lett. 59, 2044 (1987).