- Open Access
Excitonic charge density waves in moiré ladders
APS Open Sci. 1, 000003 – Published 29 April, 2026
DOI: https://doi.org/10.1103/clc3-57sk
Abstract
An incommensurate charge density wave (CDW) is a periodic modulation of charge that breaks translational symmetry incongruently with the underlying lattice. Its low-energy excitations, the phasons, are collective, gapless phase fluctuations. We study a half-filled, four-band ladder model where a shift between the legs leads to a supercell of composite cells. The moiré potential narrows minibands near the Fermi level, resulting in additional peaks in the density of states, whose separation is controlled by . The inclusion of short-range Coulomb interactions leads to an excitonic incommensurate CDW state. We identify the oscillations in its amplitude with a gapped Higgs collective mode and a lowest-energy Goldstone mode, realized by long-lived neutral phasons whose propagation velocity is governed by the shift and the interleg tunneling amplitude. Our results show that even the slightest interlayer mismatches can strongly modify both charge-ordering patterns and low-energy bosonic excitations in layered materials, and suggest that the enigmatic CDW phase in the quasi-one-dimensional compound is excitonic in nature.
Physics Subject Headings (PhySH)
See Also
Sliding phasons in moiré ladders
Article Text
References (50)
- G. Abbas, Y. Li, H. Wang, W.-X. Zhang, C. Wang, and H. Zhang, Recent advances in twisted structures of flatland materials and crafting moiré superlattices, Adv. Funct. Mater. 30, 2000878 (2020).
- P.-Y. Chen, X.-Q. Zhang, Y.-Y. Lai, E.-C. Lin, C.-A. Chen, S.-Y. Guan, J.-J. Chen, Z.-H. Yang, Y.-W. Tseng, S. Gwo, et al., Tunable moiré superlattice of artificially twisted monolayers, Adv. Mater. 31, 1901077 (2019).
- Y. Gao, X. Lin, T. Smart, P. Ci, K. Watanabe, T. Taniguchi, R. Jeanloz, J. Ni, and J. Wu, Band engineering of large-twist-angle graphene/-BN moiré superlattices with pressure, Phys. Rev. Lett. 125, 226403 (2020).
- F. Escudero, A. Sinner, Z. Zhan, P. A. Pantaleón, and F. Guinea, Designing moiré patterns by strain, Phys. Rev. Res. 6, 023203 (2024).
- T. Rakib, P. Pochet, E. Ertekin, and H. T. Johnson, Moiré engineering in van der Waals heterostructures, J. Appl. Phys. 132, 120901 (2022).
- Q. Gao and E. Khalaf, Symmetry origin of lattice vibration modes in twisted multilayer graphene: Phasons versus moiré phonons, Phys. Rev. B 106, 075420 (2022).
- P. Mellado and M. Sturla, Quantum fluctuations in the van der Waals material , Phys. Rev. B 110, 134438 (2024).
- W. McMillan, Landau theory of charge-density waves in transition-metal dichalcogenides, Phys. Rev. B 12, 1187 (1975).
- S. Takada, K. Y. M. Wong, and T. Holstein, Damping of charge-density-wave motion, Phys. Rev. B 32, 4639 (1985).
- G. Grüner, The dynamics of charge-density waves, Rev. Mod. Phys. 60, 1129 (1988).
- J. R. Tucker, W. G. Lyons, and G. Gammie, Theory of charge-density-wave dynamics, Phys. Rev. B 38, 1148 (1988).
- L. P. Gor'kov and G. Grüner, Charge Density Waves in Solids (Elsevier, Amsterdam, 2012), Vol. 25.
- K. Rossnagel, On the origin of charge-density waves in select layered transition-metal dichalcogenides, J. Phys.: Condens. Matter 23, 213001 (2011).
- X. Zhu, Y. Cao, J. Zhang, E. Plummer, and J. Guo, Classification of charge density waves based on their nature, Proc. Natl. Acad. Sci. USA 112, 2367 (2015).
- M. Imada and D. J. Scalapino, Competition between the charge-density-wave and singlet-superconducting phases in a quasi-one-dimensional system, Phys. Rev. B 34, 3480 (1986).
- A. Banerjee, Y. Feng, D. M. Silevitch, J. Wang, J. C. Lang, H.-H. Kuo, I. R. Fisher, and T. F. Rosenbaum, Charge transfer and multiple density waves in the rare earth tellurides, Phys. Rev. B 87, 155131 (2013).
- A. Melikyan and Z. Tešanović, Model of phase fluctuations in a lattice -wave superconductor: Application to the Cooper-pair charge-density wave in underdoped cuprates, Phys. Rev. B 71, 214511 (2005).
- P. B. Lee and H. Fukuyama, Dynamics of the charge-density wave. II. Long-range Coulomb effects in an array of chains, Phys. Rev. B 17, 542 (1978).
- K. Efetov and A. Larkin, Charge-density wave in a random potential, Sov. Phys. JETP 45, 2350 (1977).
- P. B. Littlewood and C. M. Varma, Amplitude collective modes in superconductors and their coupling to charge-density waves, Phys. Rev. B 26, 4883 (1982).
- A. Wegner, J. Zhao, J. Li, J. Yang, A. A. Anikin, G. Karapetrov, K. Esfarjani, D. Louca, and U. Chatterjee, Evidence for pseudo–Jahn-Teller distortions in the charge density wave phase of , Phys. Rev. B 101, 195145 (2020).
- F. Guo, M. Puppin, L. Hellbrück, A. Magrez, E. B. Guedes, I. Sokolović, and J. H. Dil, Real- and reciprocal space characterization of the three-dimensional charge density wave in quasi-one-dimensional CuTe, Phys. Rev. B 110, 115112 (2024).
- D. F. Urban, C. A. Stafford, and H. Grabert, Scaling theory of the Peierls charge density wave in metal nanowires, Phys. Rev. B 75, 205428 (2007).
- J. E. Hirsch, Effect of coulomb interactions on the Peierls instability, Phys. Rev. Lett. 51, 296 (1983).
- M. Boriack and A. Overhauser, The dynamic Peierls instability, Phys. Rev. B 15, 2847 (1977).
- Q. Gao, Y.-h. Chan, P. Jiao, H. Chen, S. Yin, K. Tangprapha, Y. Yang, X. Li, Z. Liu, D. Shen, et al., Observation of possible excitonic charge density waves and metal–insulator transitions in atomically thin semimetals, Nat. Phys. 20, 597 (2024).
- M. D. Johannes and I. I. Mazin, Fermi surface nesting and the origin of charge density waves in metals, Phys. Rev. B 77, 165135 (2008).
- P. Hofmann, M. M. Ugeda, A. Tamtögl, A. Ruckhofer, W. E. Ernst, G. Benedek, A. J. Martínez-Galera, A. Stróżecka, J. M. Gómez-Rodríguez, E. Rienks, et al., Strong-coupling charge density wave in a one-dimensional topological metal, Phys. Rev. B 99, 035438 (2019).
- C.-S. Lian, C. Si, and W. Duan, Unveiling charge-density wave, superconductivity, and their competitive nature in two-dimensional , Nano Lett. 18, 2924 (2018).
- H. Ryu, Y. Chen, H. Kim, H.-Z. Tsai, S. Tang, J. Jiang, F. Liou, S. Kahn, C. Jia, A. A. Omrani, et al., Persistent charge-density-wave order in single-layer , Nano Lett. 18, 689 (2018).
- U. Ralević, N. Lazarević, A. Baum, H.-M. Eiter, R. Hackl, P. Giraldo-Gallo, I. R. Fisher, C. Petrovic, R. Gajić, and Z. V. Popović, Charge density wave modulation and gap measurements in , Phys. Rev. B 94, 165132 (2016).
- S. Kwon, H. Jung, S. Lee, G. Y. Cho, K. Kong, C. Won, S.-W. Cheong, and H. W. Yeom, Dual Higgs modes entangled into a soliton lattice in CuTe, Nat. Commun. 15, 984 (2024).
- D. S. Fisher, Sliding charge-density waves as a dynamic critical phenomenon, Phys. Rev. B 31, 1396 (1985).
- S. Brazovskii and T. Nattermann, Pinning and sliding of driven elastic systems: from domain walls to charge density waves, Adv. Phys. 53, 177 (2004).
- J. Birkbeck, J. Xiao, A. Inbar, T. Taniguchi, K. Watanabe, E. Berg, L. Glazman, F. Guinea, F. von Oppen, and S. Ilani, Quantum twisting microscopy of phonons in twisted bilayer graphene, Nature (London) 641, 345 (2025).
- H. Ochoa, Moiré-pattern fluctuations and electron-phason coupling in twisted bilayer graphene, Phys. Rev. B 100, 155426 (2019).
- H. Miao, R. Fumagalli, M. Rossi, J. Lorenzana, G. Seibold, F. Yakhou-Harris, K. Kummer, N. B. Brookes, G. Gu, L. Braicovich, G. Ghiringhelli, and M. P. M. Dean, Formation of incommensurate charge density waves in cuprates, Phys. Rev. X 9, 031042 (2019).
- J. A. Wilson, Charge density waves: sliding and related phenomena in and other transition-metal chalcogenides, Philos. Trans. R. Soc. A 314, 159 (1985).
- R. M. Fleming and C. C. Grimes, Sliding-mode Conductivity in : Observation of a threshold electric field and conduction noise, Phys. Rev. Lett. 42, 1423 (1979).
- S. Shapiro, P. Vorderwisch, K. Habicht, K. Hradil, and H. Schneider, Observation of phasons in the magnetic shape memory alloy , Europhys. Lett. 77, 56004 (2007).
- H. Fukuyama and M. Ogata, Theory of phason drag effect on thermoelectricity, Phys. Rev. B 102, 205136 (2020).
- J. R. Schrieffer and P. A. Wolff, Relation between the Anderson and Kondo Hamiltonians, Phys. Rev. 149, 491 (1966).
- G. Coddens, On the problem of the relation between phason elasticity and phason dynamics in quasicrystals, Eur. Phys. J. B 54, 37 (2006).
- G. D. Mahan, Many-Particle Physics (Springer Science & Business Media, New York, 2013).
- A. Altland and B. D. Simons, Condensed Matter Field Theory (Cambridge University Press, Cambridge, 2010).
- A. M. Tsvelik, Quantum Field Theory in Condensed Matter Physics (Cambridge University Press, Cambridge, 2007).
- P. Mellado, F. Muñoz, and J. Cabezas-Escares, companion paper, Sliding phasons in moiré ladders, Phys. Rev. B 113, 165152 (2026).
- P. M. Chaikin, T. C. Lubensky, and T. A. Witten, Principles of Condensed Matter Physics (Cambridge University Press, Cambridge, 1995), Vol. 10.
- S. J. Denholme, A. Yukawa, K. Tsumura, M. Nagao, R. Tamura, S. Watauchi, I. Tanaka, H. Takayanagi, and N. Miyakawa, Coexistence of superconductivity and charge-density wave in the quasi-one-dimensional material , Sci. Rep. 7, 45217 (2017).
- Z. Liu, J. Li, J. Zhang, J. Li, P. Yang, S. Zhang, G. Chen, Y. Uwatoko, H. Yang, Y. Sui, et al., Quasi-one-dimensional superconductivity in the pressurized charge-density-wave conductor , npj Quantum Mater. 6, 90 (2021).