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    Dominant Charge Density Order in TaTe4

    Hongtao Rong1,9,*, Qiangqiang Gu3,7,*, Xue Yang4,*, Yihao Lin2,*, Chengcheng Zhang1, Yuan Wang1, Ruixin Guo1, Zhanyang Hao1, Yongqing Cai1 et al.

    Fayuan Zhang1, Zhicheng Jiang5, Yichen Yang5, Qi Jiang5, Zhengtai Liu5, Mao Ye5, Shu Guo1, Le Wang1, Junhao Lin1, Li Lu4,6, Guangtong Liu4,6,†, Ji Feng2,6,‡, and Chaoyu Chen1,8,§

    • *These authors contributed equally to this work.
    • †Contact author: gtliu@iphy.ac.cn
    • ‡Contact author: jfeng11@pku.edu.cn
    • §Contact author: chency@sustech.edu.cn

    Phys. Rev. Lett. 133, 116403 – Published 12 September, 2024

    DOI: https://doi.org/10.1103/PhysRevLett.133.116403

    Abstract

    Electronic orders such as charge density wave (CDW) and superconductivity raise exotic physics and phenomena as evidenced in recently discovered kagome superconductors and transition metal chalcogenides. In most materials, CDW induces a weak, perturbative effect, manifested as shadow bands, minigaps, resistivity kinks, etc. Here we demonstrate a unique example—transition metal tetratellurides TaTe4, in which the CDW order dominates the electronic structure and transport properties. Using angle-resolved photoemission spectroscopy, we found that the band structure of CDW TaTe4 is characterized by small, bulk electron pockets. Density functional theory analyses reveal their CDW origin from the folding of the original, large Fermi pockets. Importantly, the CDW induced pockets result in prominent frequencies in the quantum oscillation of the magnetoresistance. Satisfactory agreements are reached between results from photoemission spectroscopy, density functional theory, and quantum oscillation, concerning the shape, size, location, and angle dependence of the CDW pockets. Our results underline transition metal tetratellurides as an outstanding example for exploring the interplay between CDW, pressure induced superconductivity, and potential topological states under strong field.

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