Export citation

Export citation

Choose format for download:

Download Citation

    Room Temperature Superfluorescence from an Electron-Hole Liquid

    Naresh Aggarwal1, Ajay Kumar Poonia1, Dmitry N. Dirin2, Ihor Cherniukh3, Arijit Sinha4, Umesh V. Waghmare4, Maryna I. Bodnarchuk3, Sebastian Wüster1, Maksym V. Kovalenko2,3 et al.

    K. V. Adarsh1,*

    • *Contact author: adarsh@iiserb.ac.in

    Phys. Rev. Lett. 134, 083801 – Published 26 February, 2025

    DOI: https://doi.org/10.1103/PhysRevLett.134.083801

    Abstract

    Superfluorescence, a coherent burst of light from an excited ensemble of emitters, is a crucial quantum optical phenomenon with far-reaching implications in nanophotonics and many-body optical processes. Despite its observation in various systems, realizing superfluorescence in an electron-hole plasma (EHP) at room temperature has remained a formidable challenge, hindering the development of continuous-wave and electrically excited superfluorescence devices. Herein, we address this challenge by condensing the high-density EHP into an electron-hole liquid (EHL) at room temperature, thereby preserving quantum coherence. Using a model system of nanocrystal thin films, we demonstrate the first experimental observation of room temperature superfluorescence from an EHL. Key attributes heralding superfluorescence include a redshift of ∼94  meV from uncorrelated exciton emission, a fluence-dependent delayed growth of macroscopic coherence with abrupt radiative decay ∼1250 times faster than spontaneous emission, a distinct quadratic fluence dependence with a clear threshold, and Burnham-Chiao ringing. These findings open up exciting possibilities for developing electrically pumped colloidal nanocrystals lasers and quantum technologies operating at room temperature.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    Supplemental Material (Subscription Required)

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation