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    High-Precision Mass Measurements of Neutron Deficient Silver Isotopes Probe the Robustness of the N=50 Shell Closure

    Zhuang Ge (葛壮)1,2,*, Mikael Reponen1,†, Tommi Eronen1, Baishan Hu (胡柏山)3,4,5, Markus Kortelainen1, Anu Kankainen1, Iain Moore1, Dmitrii Nesterenko1, Cenxi Yuan (袁岑溪)6 et al.

    Olga Beliuskina1, Laetitia Cañete1,‡, Ruben de Groote1,7, Clément Delafosse1,8, Timo Dickel2,10, Antoine de Roubin1,§, Sarina Geldhof1,9, Wouter Gins1, Jason D. Holt3,11, Marjut Hukkanen1,12, Arthur Jaries1, Ari Jokinen1, Ágota Koszorús13,14,7, Gabriella Kripkó-Koncz10, Sonja Kujanpää1, Yi Hua Lam (藍乙華)15,16, Stylianos Nikas1, Alejandro Ortiz-Cortes1,9, Heikki Penttilä1, Daniel Pitman-Weymouth1, Wolfgang Plaß2,10, Ilkka Pohjalainen1, Andrea Raggio1, Sami Rinta-Antila1, Jorge Romero1,13, Marek Stryjczyk1, Markus Vilen1,14, Ville Virtanen1, and Alexandra Zadvornaya1,∥

    • *Contact author: zhuang.z.ge@jyu.fi
    • †Contact author: mikael.h.t.reponen@jyu.fi
    • ‡Also at Northeastern University London, Devon House, 58 St Katharine’s Way, E1W 1LP, London, United Kingdom.
    • §Also at LPC Caen, Université de Caen Normandie, 14050 Caen Cedex, France.
    • ∥Present address: University of Edinburgh, Edinburgh, EH9 3FD, United Kingdom.

    Phys. Rev. Lett. 133, 132503 – Published 26 September, 2024

    DOI: https://doi.org/10.1103/PhysRevLett.133.132503

    Abstract

    High-precision mass measurements of exotic Ag95–97 isotopes close to the N=Z line have been conducted with the JYFLTRAP double Penning trap mass spectrometer, with the silver ions produced using the recently commissioned inductively heated hot cavity catcher laser ion source at the Ion Guide Isotope Separator On-Line facility. The atomic mass of Ag95 was directly determined for the first time. In addition, the atomic masses of β-decaying 2+ and 8+ states in Ag96 have been identified and measured for the first time, and the precision of the Ag97 mass has been improved. The newly measured masses, with a precision of ≈1  keV/c2, have been used to investigate the N=50 neutron shell closure, confirming it to be robust. Empirical shell-gap and pairing energies determined with the new ground-state mass data are compared with the state-of-the-art ab initio calculations with various chiral effective field theory Hamiltonians. The precise determination of the excitation energy of the Ag96m isomer in particular serves as a benchmark for ab initio predictions of nuclear properties beyond the ground state, specifically for odd-odd nuclei situated in proximity to the proton dripline below Sn100. In addition, density functional theory calculations and configuration-interaction shell-model calculations are compared with the experimental results. All theoretical approaches face challenges to reproduce the trend of nuclear ground-state properties in the silver isotopic chain across the N=50 neutron shell and toward the proton dripline.

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