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Probing Magnetic Exchange Interactions with Helium

C. Trainer1, C. M. Yim1,2, C. Heil3, L. S. Farrar1, V. Tsurkan4,5, A. Loidl4, and P. Wahl1

  • 1SUPA, School of Physics and Astronomy, University of St Andrews, North Haugh, St Andrews KY16 9SS, United Kingdom
  • 2Tsung Dao Lee Institute & School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China
  • 3Institute of Theoretical and Computational Physics, Graz University of Technology, NAWI Graz, 8010 Graz, Austria
  • 4Center for Electronic Correlations and Magnetism, Experimental Physics V, University of Augsburg, D-86159 Augsburg, Germany
  • 5Institute of Applied Physics, MD 2028 Chisinau, Republic of Moldova

Phys. Rev. Lett. 127, 166803 – Published 12 October, 2021

DOI: https://doi.org/10.1103/PhysRevLett.127.166803

Abstract

Controlling and sensing spin polarization of electrons forms the basis of spintronics. Here, we report a study of the effect of helium on the spin polarization of the tunneling current and magnetic contrast in spin-polarized scanning tunneling microscopy (SP STM). We show that the magnetic contrast in SP STM images recorded in the presence of helium depends sensitively on the tunneling conditions. From tunneling spectra and their variation across the atomic lattice we establish that the helium can be reversibly ejected from the tunneling junction by the tunneling electrons. The energy of the tunneling electrons required to eject the helium depends on the relative spin polarization of the tip and sample, making the microscope sensitive to the magnetic exchange interactions. We show that the time-averaged spin polarization of the tunneling current is suppressed in the presence of helium and thereby demonstrate voltage control of the spin polarization of the tunneling current across the tip-sample junction.

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