Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Featured in Physics
  • Editors' Suggestion
  • Open Access

Spectroscopy along Flerovium Decay Chains: Discovery of Ds280 and an Excited State in Cn282

A. Såmark-Roth1,*, D. M. Cox1, D. Rudolph1, L. G. Sarmiento1, B. G. Carlsson1, J. L. Egido2, P. Golubev1, J. Heery3, A. Yakushev4 et al.

S. Åberg1, H. M. Albers4, M. Albertsson1, M. Block4,5,6, H. Brand4, T. Calverley3, R. Cantemir4, R. M. Clark7, Ch. E. Düllmann4,5,6, J. Eberth8, C. Fahlander1, U. Forsberg1, J. M. Gates7, F. Giacoppo4,5, M. Götz4,5,6, S. Götz4,5,6, R.-D. Herzberg3, Y. Hrabar1, E. Jäger4, D. Judson3, J. Khuyagbaatar4,5, B. Kindler4, I. Kojouharov4, J. V. Kratz6, J. Krier4, N. Kurz4, L. Lens4,6,†, J. Ljungberg1, B. Lommel4, J. Louko9, C.-C. Meyer5,6, A. Mistry10,4, C. Mokry5,6, P. Papadakis3,‡, E. Parr4, J. L. Pore7, I. Ragnarsson1, J. Runke4,6, M. Schädel4, H. Schaffner4, B. Schausten4, D. A. Shaughnessy11, P. Thörle-Pospiech5,6, N. Trautmann6, and J. Uusitalo9

  • 1Department of Physics, Lund University, 22100 Lund, Sweden
  • 2Departamento de Física Teórica and CIAFF, Universidad Autónoma de Madrid, 28049 Madrid, Spain
  • 3Department of Physics, University of Liverpool, Liverpool L69 7ZE, United Kingdom
  • 4GSI Helmholtzzentrum für Schwerionenforschung GmbH, 64291 Darmstadt, Germany
  • 5Helmholtz Institute Mainz, 55099 Mainz, Germany
  • 6Department Chemie–Standort TRIGA, Johannes Gutenberg-Universität Mainz, 55099 Mainz, Germany
  • 7Nuclear Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
  • 8Institut für Kernphysik, Universität zu Köln, 50937 Köln, Germany
  • 9Department of Physics, University of Jyväskylä, 40014 Jyväskylä, Finland
  • 10Institut für Kernphysik, Technische Universität Darmstadt, 64289 Darmstadt, Germany
  • 11Nuclear and Chemical Sciences Division, Lawrence Livermore National Laboratory, Livermore, California 94550, USA

  • *Anton.Samark-Roth@nuclear.lu.se
  • †Present address: Institut für Physikalische Chemie und Radiochemie, Hochschule Mannheim, 68163 Mannheim, Germany.
  • ‡Present address: STFC Daresbury Laboratory, Daresbury, Warrington WA4 4AD, United Kingdom.

Phys. Rev. Lett. 126, 032503 – Published 22 January, 2021

DOI: https://doi.org/10.1103/PhysRevLett.126.032503

Abstract

A nuclear spectroscopy experiment was conducted to study α-decay chains stemming from isotopes of flerovium (element Z=114). An upgraded TASISpec decay station was placed behind the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt, Germany. The fusion-evaporation reactions Ca48+Pu242 and Ca48+Pu244 provided a total of 32 flerovium-candidate decay chains, of which two and eleven were firmly assigned to Fl286 and Fl288, respectively. A prompt coincidence between a 9.60(1)-MeV α particle event and a 0.36(1)-MeV conversion electron marked the first observation of an excited state in an even-even isotope of the heaviest man-made elements, namely Cn282. Spectroscopy of Fl288 decay chains fixed Qα=10.06(1)  MeV. In one case, a Qα=9.46(1)-MeV decay from Cn284 into Ds280 was observed, with Ds280 fissioning after only 518  μs. The impact of these findings, aggregated with existing data on decay chains of Fl286,288, on the size of an anticipated shell gap at proton number Z=114 is discussed in light of predictions from two beyond-mean-field calculations, which take into account triaxial deformation.

View figure in article

Physics Subject Headings (PhySH)

synopsis

An Octad for Darmstadtium and Excitement for Copernicium

Published 22 January, 2021

The discovery that copernicium can decay into a new isotope of darmstadtium and the observation of a previously unseen excited state of copernicium provide clues to the location of the “island of stability.”

See more in Physics

See Also

Article Text

Supplemental Material

References (61)

  1. L. Öhrström and J. Reedijk, Pure Appl. Chem. 88, 1225 (2016).
  2. Special Issue on Superheavy Elements, edited by Ch. E. Düllmann, R.-D. Herzberg, W. Nazarewicz, and Y. Oganessian, Nucl. Phys. A944, 1 (2015), https://www.sciencedirect.com/journal/nuclear-physics-a/vol/944.
  3. D. Rudolph, EPJ Web Conf. 131 (2016), https://www.epj-conferences.org/articles/epjconf/abs/2016/26/contents/contents.html.
  4. Ch. E. Düllmann, M. Schädel, A. Yakushev, A. Türler, K. Eberhardt, J. V. Kratz et al., Phys. Rev. Lett. 104, 252701 (2010).
  5. U. Forsberg, D. Rudolph, L.-L. Andersson, A. Di Nitto, Ch. E. Düllmann, C. Fahlander et al., Nucl. Phys. A953, 117 (2016).
  6. A. Türler, R. Eichler, and A. Yakushev, Nucl. Phys. A944, 640 (2015).
  7. A. Yakushev and R. Eichler, EPJ Web Conf. 131, 07003 (2016).
  8. A. Yakushev, J. M. Gates, A. Türler, M. Schädel, Ch. E. Düllmann, D. Ackermann et al., Inorg. Chem. 53, 1624 (2014).
  9. A. Yakushev, L. Lens, Ch. E. Düllmann, H. M. Albers, M. Asai, M. Block et al., Nat. Chem. (to be published).
  10. D. Rudolph, U. Forsberg, P. Golubev, L. G. Sarmiento, A. Yakushev, L.-L. Andersson et al., Phys. Rev. Lett. 111, 112502 (2013).
  11. J. M. Gates, K. E. Gregorich, O. R. Gothe, E. C. Uribe, G. K. Pang, D. L. Bleuel et al., Phys. Rev. C 92, 021301(R) (2015).
  12. L. G. Sarmiento, EPJ Web Conf. 131, 05004 (2016).
  13. D. Rudolph, L. G. Sarmiento, and U. Forsberg, AIP Conf. Proc. 1681, 030015 (2015).
  14. Yue Shi, D. E. Ward, B. G. Carlsson, J. Dobaczewski, W. Nazarewicz, I. Ragnarsson, and D. Rudolph, Phys. Rev. C 90, 014308 (2014).
  15. J. M. Gates, G. K. Pang, J. L. Pore, K. E. Gregorich, J. T. Kwarsick, G. Savard et al., Phys. Rev. Lett. 121, 222501 (2018).
  16. J. Dobaczewski, A. V. Afanasjev, M. Bender, L. M. Robledo, and Yue Shi, Nucl. Phys. A944, 388 (2015).
  17. P.-H. Heenen, J. Skalski, A. Staszczak, and D. Vretenar, Nucl. Phys. A944, 415 (2015).
  18. D. M. Cox et al., Phys. Rev. Lett. (to be published).
  19. D. M. Cox, A. Såmark-Roth, D. Rudolph, L. G. Sarmiento, C. Fahlander, U. Forsberg et al., J. Phys. Conf. Ser. 1643, 012125 (2020).
  20. A. Såmark-Roth et al., Phys. Rev. C (to be published).
  21. See Supplemental Material at http://link.aps.org/supplemental/10.1103/PhysRevLett.126.032503 for detailed results and statistical assessments concerning decay chains starting with isotopes Fl286,288.
  22. E. Jäger, H. Brand, Ch. E. Düllmann, J. Khuyagbaatar, J. Krier, M. Schädel, T. Torres, and A. Yakushev, J. Radioanal. Nucl. Chem. 299, 1073 (2014).
  23. J. Runke, Ch. E. Düllmann, K. Eberhardt, P. A. Ellison, K. E. Gregorich, S. Hoffmann et al., J. Radioanal. Rad. Nucl. Chem. 299, 1081 (2014).
  24. J. F. Ziegler, Nucl. Instrum. Methods Phys. Res., Sect. B 219–220, 1027 (2004).
  25. W. D. Myers and W. J. Swiatecki, Nucl. Phys. A601, 141 (1996).
  26. A. Semchenkov, W. Brüchle, E. Jäger, E. Schimpf, M. Schädel, C. Mühle et al., Nucl. Instrum. Methods Phys. Res., Sect. B 266, 4153 (2008).
  27. L.-L. Andersson, D. Rudolph, P. Golubev, R.-D. Herzberg, R. Hoischen, E. Merchán et al., Nucl. Instrum. Methods Phys. Res., Sect. A 622, 164 (2010).
  28. J. M. Gates, Ch. E. Düllmann, M. Schädel, A. Yakushev, A. Türler, K. Eberhardt et al., Phys. Rev. C 83, 054618 (2011).
  29. U. Forsberg, P. Golubev, L. G. Sarmiento, J. Jeppsson, D. Rudolph, L.-L. Andersson et al., Acta Phys. Pol. 43, 305 (2012).
  30. K. E. Gregorich, Nucl. Instrum. Methods Phys. Res., Sect. A 711, 47 (2013).
  31. J. Eberth, H. G. Thomas, P. v. Brentano, R. M. Lieder, H. M. Jäger, H. Kämmerling, M. Berst, D. Gutknecht, and R. Henck, Nucl. Instrum. Methods Phys. Res., Sect. A 369, 135 (1996).
  32. A. Såmark-Roth, D. M. Cox, J. Eberth, P. Golubev, D. Rudolph, L. G. Sarmiento, G. Tocabens, M. Ginsz, B. Pirard, and P. Quirin, Eur. Phys. J. A 56, 141 (2020).
  33. Yu. Ts. Oganessian, V. K. Utyonkov, Yu. V. Lobanov, F. Sh. Abdullin, A. N. Polyakov, I. V. Shirokovsky et al., Phys. Rev. C 70, 064609 (2004).
  34. S. Hofmann, D. Ackermann, S. Antalic, H. G. Burkhard, V. F. Comas, R. Dressler et al., Eur. Phys. J. A 32, 251 (2007).
  35. L. Stavsetra, K. E. Gregorich, J. Dvorak, P. A. Ellison, I. Dragojević, M. A. Garcia, and H. Nitsche, Phys. Rev. Lett. 103, 132502 (2009).
  36. P. A. Ellison, K. E. Gregorich, J. S. Berryman, D. L. Bleuel, R. M. Clark, I. Dragojević et al., Phys. Rev. Lett. 105, 182701 (2010).
  37. Yu. Ts. Oganessian, V. K. Utyonkov, Yu. V. Lobanov, F. Sh. Abdullin, A. N. Polyakov, I. V. Shirokovsky et al., Phys. Rev. C 69, 054607 (2004).
  38. Yu. Ts. Oganessian, V. K. Utyonkov, Yu. V. Lobanov, F. Sh. Abdullin, A. N. Polyakov, R. N. Sagaidak et al., Phys. Rev. C 74, 044602 (2006).
  39. Yu. Ts. Oganessian, F. Sh. Abdullin, C. Alexander, J. Binder, R. A. Boll, S. N. Dmitriev et al., Phys. Rev. Lett. 109, 162501 (2012).
  40. Yu. Ts. Oganessian, V. K. Utyonkov, Yu. V. Lobanov, F. Sh. Abdullin, A. N. Polyakov, I. V. Shirokovsky et al., in JINR, E7-2004-160 (2004), p. 128, http://www.jinr.ru/publish/Preprints/2004/160(E7-2004-160).pdf.
  41. S. Hofmann, S. Heinz, R. Mann, J. Maurer, J. Khuyagbaatar, D. Ackermann et al., Eur. Phys. J. A 48, 62 (2012).
  42. D. Kaji, K. Morita, K. Morimoto, H. Haba, M. Asai, K. Fujita et al., J. Phys. Soc. Jpn. 86, 034201 (2017).
  43. K.-H. Schmidt, Eur. Phys. J. A 8, 141 (2000).
  44. C. Qi, F. R. Xu, R. J. Liotta, R. Wyss, M. Y. Zhang, C. Asawatangtrakuldee, and D. Hu, Phys. Rev. C 80, 044326 (2009).
  45. F. P. Heßberger, EPJ Web Conf. 131, 02005 (2016).
  46. K.-H. Schmidt, C.-C. Sahm, K. Pielenz, and H.-G. Clerc, Z. Phys. A 316, 19 (1984).
  47. The suggested version B of chain 3 in Ref. [42] has serious problems with both the derived α energy, correlation time, and in particular the position of the 0.83-MeV escape event tentatively assigned to Fl288.

  48. P. Möller, A. J. Sierk, T. Ichikawa, and H. Sagawa, At. Data. Nucl. Data Sheets 109–110, 1 (2016).
  49. P. Jachimowicz, M. Kowal, and J. Skalski, Phys. Rev. C 89, 024304 (2014).
  50. E. Olsen and W. Nazarewicz, Phys. Rev. C 99, 014317 (2019).
  51. M. Warda and J. L. Egido, Phys. Rev. C 86, 014322 (2012).
  52. V. Prassa, T. Nikšić, G. A. Lalazissis, and D. Vretenar, Phys. Rev. C 86, 024317 (2012).
  53. T. R. Rodríguez and J. L. Egido, Phys. Rev. C 81, 064323 (2010).
  54. J. L. Egido and A. Jungclaus, Phys. Rev. Lett. 125, 192504 (2020).
  55. B. G. Carlsson and J. Ljungberg, Phys. Rev. Lett. (to be published).
  56. S. Ćwiok, P. H. Heenen, and W. Nazarewicz, Nature (London) 433, 705 (2005).
  57. T. Kibédi, M. B. Trzhaskovskaya, M. Gupta, and A. E. Stuchberry, At. Data. Nucl. Data Sheets 98, 313 (2012).
  58. F. P. Heßberger, S. Hoffmann, G. Münzenberg, K.-H. Schmidt, P. Armbruster, and R. Hingmann, Nucl. Instrum. Methods Phys. Res., Sect. A 274, 522 (1989).
  59. Ch. Theissen, A. Lopez-Martens, and Ch. Bonnelle, Nucl. Instrum. Methods Phys. Res., Sect. A 589, 230 (2008).
  60. A. N. Andreyev, M. Huyse, P. Van Duppen, L. Weissman, D. Ackermann, J. Gerl et al., Nature (London) 405, 430 (2000).
  61. K. Van de Vel, A. N. Andreyev, D. Ackermann, H. J. Boardman, P. Cagarda, J. Gerl et al., Phys. Rev. C 68, 054311 (2003).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation