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Spectroscopy along Flerovium Decay Chains: Discovery of and an Excited State in
Phys. Rev. Lett. 126, 032503 – Published 22 January, 2021
DOI: https://doi.org/10.1103/PhysRevLett.126.032503
Abstract
A nuclear spectroscopy experiment was conducted to study -decay chains stemming from isotopes of flerovium (element ). An upgraded TASISpec decay station was placed behind the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt, Germany. The fusion-evaporation reactions and provided a total of 32 flerovium-candidate decay chains, of which two and eleven were firmly assigned to and , respectively. A prompt coincidence between a 9.60(1)-MeV particle event and a 0.36(1)-MeV conversion electron marked the first observation of an excited state in an even-even isotope of the heaviest man-made elements, namely . Spectroscopy of decay chains fixed . In one case, a -MeV decay from into was observed, with fissioning after only . The impact of these findings, aggregated with existing data on decay chains of , on the size of an anticipated shell gap at proton number is discussed in light of predictions from two beyond-mean-field calculations, which take into account triaxial deformation.
Physics Subject Headings (PhySH)
synopsis
An Octad for Darmstadtium and Excitement for Copernicium
The discovery that copernicium can decay into a new isotope of darmstadtium and the observation of a previously unseen excited state of copernicium provide clues to the location of the “island of stability.”
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See Also
Spectroscopy along flerovium decay chains. III. Details on experiment, analysis, , and spontaneous fission branches
Spectroscopy along flerovium decay chains. II. Fine structure in odd-
Article Text
Supplemental Material
References (61)
- L. Öhrström and J. Reedijk, Pure Appl. Chem. 88, 1225 (2016).
- Special Issue on Superheavy Elements, edited by Ch. E. Düllmann, R.-D. Herzberg, W. Nazarewicz, and Y. Oganessian, Nucl. Phys. A944, 1 (2015), https://www.sciencedirect.com/journal/nuclear-physics-a/vol/944.
- D. Rudolph, EPJ Web Conf. 131 (2016), https://www.epj-conferences.org/articles/epjconf/abs/2016/26/contents/contents.html.
- Ch. E. Düllmann, M. Schädel, A. Yakushev, A. Türler, K. Eberhardt, J. V. Kratz et al., Phys. Rev. Lett. 104, 252701 (2010).
- U. Forsberg, D. Rudolph, L.-L. Andersson, A. Di Nitto, Ch. E. Düllmann, C. Fahlander et al., Nucl. Phys. A953, 117 (2016).
- A. Türler, R. Eichler, and A. Yakushev, Nucl. Phys. A944, 640 (2015).
- A. Yakushev and R. Eichler, EPJ Web Conf. 131, 07003 (2016).
- A. Yakushev, J. M. Gates, A. Türler, M. Schädel, Ch. E. Düllmann, D. Ackermann et al., Inorg. Chem. 53, 1624 (2014).
- A. Yakushev, L. Lens, Ch. E. Düllmann, H. M. Albers, M. Asai, M. Block et al., Nat. Chem. (to be published).
- D. Rudolph, U. Forsberg, P. Golubev, L. G. Sarmiento, A. Yakushev, L.-L. Andersson et al., Phys. Rev. Lett. 111, 112502 (2013).
- J. M. Gates, K. E. Gregorich, O. R. Gothe, E. C. Uribe, G. K. Pang, D. L. Bleuel et al., Phys. Rev. C 92, 021301(R) (2015).
- L. G. Sarmiento, EPJ Web Conf. 131, 05004 (2016).
- D. Rudolph, L. G. Sarmiento, and U. Forsberg, AIP Conf. Proc. 1681, 030015 (2015).
- Yue Shi, D. E. Ward, B. G. Carlsson, J. Dobaczewski, W. Nazarewicz, I. Ragnarsson, and D. Rudolph, Phys. Rev. C 90, 014308 (2014).
- J. M. Gates, G. K. Pang, J. L. Pore, K. E. Gregorich, J. T. Kwarsick, G. Savard et al., Phys. Rev. Lett. 121, 222501 (2018).
- J. Dobaczewski, A. V. Afanasjev, M. Bender, L. M. Robledo, and Yue Shi, Nucl. Phys. A944, 388 (2015).
- P.-H. Heenen, J. Skalski, A. Staszczak, and D. Vretenar, Nucl. Phys. A944, 415 (2015).
- D. M. Cox et al., Phys. Rev. Lett. (to be published).
- D. M. Cox, A. Såmark-Roth, D. Rudolph, L. G. Sarmiento, C. Fahlander, U. Forsberg et al., J. Phys. Conf. Ser. 1643, 012125 (2020).
- A. Såmark-Roth et al., Phys. Rev. C (to be published).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/PhysRevLett.126.032503 for detailed results and statistical assessments concerning decay chains starting with isotopes .
- E. Jäger, H. Brand, Ch. E. Düllmann, J. Khuyagbaatar, J. Krier, M. Schädel, T. Torres, and A. Yakushev, J. Radioanal. Nucl. Chem. 299, 1073 (2014).
- J. Runke, Ch. E. Düllmann, K. Eberhardt, P. A. Ellison, K. E. Gregorich, S. Hoffmann et al., J. Radioanal. Rad. Nucl. Chem. 299, 1081 (2014).
- J. F. Ziegler, Nucl. Instrum. Methods Phys. Res., Sect. B 219–220, 1027 (2004).
- W. D. Myers and W. J. Swiatecki, Nucl. Phys. A601, 141 (1996).
- A. Semchenkov, W. Brüchle, E. Jäger, E. Schimpf, M. Schädel, C. Mühle et al., Nucl. Instrum. Methods Phys. Res., Sect. B 266, 4153 (2008).
- L.-L. Andersson, D. Rudolph, P. Golubev, R.-D. Herzberg, R. Hoischen, E. Merchán et al., Nucl. Instrum. Methods Phys. Res., Sect. A 622, 164 (2010).
- J. M. Gates, Ch. E. Düllmann, M. Schädel, A. Yakushev, A. Türler, K. Eberhardt et al., Phys. Rev. C 83, 054618 (2011).
- U. Forsberg, P. Golubev, L. G. Sarmiento, J. Jeppsson, D. Rudolph, L.-L. Andersson et al., Acta Phys. Pol. 43, 305 (2012).
- K. E. Gregorich, Nucl. Instrum. Methods Phys. Res., Sect. A 711, 47 (2013).
- J. Eberth, H. G. Thomas, P. v. Brentano, R. M. Lieder, H. M. Jäger, H. Kämmerling, M. Berst, D. Gutknecht, and R. Henck, Nucl. Instrum. Methods Phys. Res., Sect. A 369, 135 (1996).
- A. Såmark-Roth, D. M. Cox, J. Eberth, P. Golubev, D. Rudolph, L. G. Sarmiento, G. Tocabens, M. Ginsz, B. Pirard, and P. Quirin, Eur. Phys. J. A 56, 141 (2020).
- Yu. Ts. Oganessian, V. K. Utyonkov, Yu. V. Lobanov, F. Sh. Abdullin, A. N. Polyakov, I. V. Shirokovsky et al., Phys. Rev. C 70, 064609 (2004).
- S. Hofmann, D. Ackermann, S. Antalic, H. G. Burkhard, V. F. Comas, R. Dressler et al., Eur. Phys. J. A 32, 251 (2007).
- L. Stavsetra, K. E. Gregorich, J. Dvorak, P. A. Ellison, I. Dragojević, M. A. Garcia, and H. Nitsche, Phys. Rev. Lett. 103, 132502 (2009).
- P. A. Ellison, K. E. Gregorich, J. S. Berryman, D. L. Bleuel, R. M. Clark, I. Dragojević et al., Phys. Rev. Lett. 105, 182701 (2010).
- Yu. Ts. Oganessian, V. K. Utyonkov, Yu. V. Lobanov, F. Sh. Abdullin, A. N. Polyakov, I. V. Shirokovsky et al., Phys. Rev. C 69, 054607 (2004).
- Yu. Ts. Oganessian, V. K. Utyonkov, Yu. V. Lobanov, F. Sh. Abdullin, A. N. Polyakov, R. N. Sagaidak et al., Phys. Rev. C 74, 044602 (2006).
- Yu. Ts. Oganessian, F. Sh. Abdullin, C. Alexander, J. Binder, R. A. Boll, S. N. Dmitriev et al., Phys. Rev. Lett. 109, 162501 (2012).
- Yu. Ts. Oganessian, V. K. Utyonkov, Yu. V. Lobanov, F. Sh. Abdullin, A. N. Polyakov, I. V. Shirokovsky et al., in JINR, E7-2004-160 (2004), p. 128, http://www.jinr.ru/publish/Preprints/2004/160(E7-2004-160).pdf.
- S. Hofmann, S. Heinz, R. Mann, J. Maurer, J. Khuyagbaatar, D. Ackermann et al., Eur. Phys. J. A 48, 62 (2012).
- D. Kaji, K. Morita, K. Morimoto, H. Haba, M. Asai, K. Fujita et al., J. Phys. Soc. Jpn. 86, 034201 (2017).
- K.-H. Schmidt, Eur. Phys. J. A 8, 141 (2000).
- C. Qi, F. R. Xu, R. J. Liotta, R. Wyss, M. Y. Zhang, C. Asawatangtrakuldee, and D. Hu, Phys. Rev. C 80, 044326 (2009).
- F. P. Heßberger, EPJ Web Conf. 131, 02005 (2016).
- K.-H. Schmidt, C.-C. Sahm, K. Pielenz, and H.-G. Clerc, Z. Phys. A 316, 19 (1984).
The suggested version B of chain 3 in Ref. [42] has serious problems with both the derived energy, correlation time, and in particular the position of the 0.83-MeV escape event tentatively assigned to .
- P. Möller, A. J. Sierk, T. Ichikawa, and H. Sagawa, At. Data. Nucl. Data Sheets 109–110, 1 (2016).
- P. Jachimowicz, M. Kowal, and J. Skalski, Phys. Rev. C 89, 024304 (2014).
- E. Olsen and W. Nazarewicz, Phys. Rev. C 99, 014317 (2019).
- M. Warda and J. L. Egido, Phys. Rev. C 86, 014322 (2012).
- V. Prassa, T. Nikšić, G. A. Lalazissis, and D. Vretenar, Phys. Rev. C 86, 024317 (2012).
- T. R. Rodríguez and J. L. Egido, Phys. Rev. C 81, 064323 (2010).
- J. L. Egido and A. Jungclaus, Phys. Rev. Lett. 125, 192504 (2020).
- B. G. Carlsson and J. Ljungberg, Phys. Rev. Lett. (to be published).
- S. Ćwiok, P. H. Heenen, and W. Nazarewicz, Nature (London) 433, 705 (2005).
- T. Kibédi, M. B. Trzhaskovskaya, M. Gupta, and A. E. Stuchberry, At. Data. Nucl. Data Sheets 98, 313 (2012).
- F. P. Heßberger, S. Hoffmann, G. Münzenberg, K.-H. Schmidt, P. Armbruster, and R. Hingmann, Nucl. Instrum. Methods Phys. Res., Sect. A 274, 522 (1989).
- Ch. Theissen, A. Lopez-Martens, and Ch. Bonnelle, Nucl. Instrum. Methods Phys. Res., Sect. A 589, 230 (2008).
- A. N. Andreyev, M. Huyse, P. Van Duppen, L. Weissman, D. Ackermann, J. Gerl et al., Nature (London) 405, 430 (2000).
- K. Van de Vel, A. N. Andreyev, D. Ackermann, H. J. Boardman, P. Cagarda, J. Gerl et al., Phys. Rev. C 68, 054311 (2003).