- Accepted Paper
Magnetic order, magnons, and crystal fields in van der Waals CeSiI
Phys. Rev. Lett. - Accepted 23 October, 2026
DOI: https://doi.org/10.1103/tq6k-wy73
Phys. Rev. Lett. - Accepted 23 October, 2026
DOI: https://doi.org/10.1103/tq6k-wy73
We report neutron and X-ray absorption spectroscopy as well as resonant inelastic X-ray scattering of magnetic excitations in the new heavy-fermion van-der-Waals superconductor CeSiI. We determined effective Hamiltonians and ground states of crystal electric fields and magnons. Isotropic Heisenberg interactions on a quasi two dimensional lattice, including ferromagnetic nearest-neighbor exchange as the dominant interaction, provide an excellent account to the low-energy measured dynamics and stabilize a co-rotating spin cycloid. Our study provides the basis to model CeSiI from first principles, thereby laying the ground for microscopic understanding of heavy-fermion physics, their unconventional superconductivity, and quantum criticality.
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