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Third-Order Nonlinear Hall Effect in Altermagnet RuO2

R. Y. Chu1,*, L. Han1,*, Z. H. Gong2,*, X. Z. Fu3, H. Bai1, S. X. Liang1, C. Chen1, S-W. Cheong4, Y. Y. Zhang3 et al.

J. W. Liu3, Y. Y. Wang1, F. Pan1, H. Z. Lu2,5,†, and C. Song1,‡

  • *These authors contributed equally to this work.
  • †Contact author: luhz@sustech.edu.cn
  • ‡Contact author: songcheng@mail.tsinghua.edu.cn

Phys. Rev. Lett. 135, 216703 – Published 17 November, 2025

DOI: https://doi.org/10.1103/rv1n-vr4p

Abstract

Altermagnets are a novel class of magnetic materials with cutting-edge advantages. Identifying altermagnets, i.e., exploring their distinguishing fingerprints, is vital but challenging. The as-reported spontaneous anomalous Hall effect is not universally present in all altermagnets due to magnetic symmetry constraints, and the second-order nonlinear Hall effect is prohibited by spatial-inversion symmetry. Here, we report the experimental discovery of a third-order nonlinear Hall effect (TNHE) in RuO2 thin films. TNHE emerges when current is applied along [110] or [1¯10] crystal direction for RuO2(001), as the second-order currents induce a magnetization by breaking orthogonal mirror and rotation symmetries of this altermagnet. These symmetry-breaking conditions also enforce a twofold angular dependence of TNHE concerning current direction in the RuO2(001) plane. Moreover, temperature-dependent measurements and scaling law analysis reveal that TNHE is governed primarily by the third-order skew scattering mechanism. Our findings establish TNHE as a transport fingerprint of altermagnet RuO2, which can be generalized to other altermagnets such as d-wave V2X2O (X=Se or Te) and g-wave MnTe and CrSb.

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