• Accepted Paper

Optical readout of the magnetic state using terahertz electric fields

T. G. H. Blank, C. Bauer, M. X. Na, E. A. Mashkovich, A. K. Zvezdin, A. M. Kalashnikova, and A. V. Kimel

Phys. Rev. Lett. - Accepted 11 September, 2026

DOI: https://doi.org/10.1103/rpfv-7nm6

Abstract

A single-cycle terahertz (THz) pulse applied to single-crystal holmium iron garnet Ho3Fe5O12 strongly perturbs the magneto-optical Faraday effect – an effect conventionally employed for optical readout of the magnetic state. This ultrafast perturbation sets in when cooling below the magnetization compensation temperature, where the unit cell distorts and the spins of Ho3+ form a noncollinear "double-umbrella" structure. The experimental dependencies reveal that the findings can be described as the ultrafast THz-electric-field-induced magneto-optical (TEMO) Faraday effect, caused by the resonant excitation of crystal-field-split f-f electronic transitions of Ho3+ in a noncentrosymmetric environment of oxygen ions. We demonstrate that the effect is not limited to Ho3Fe5O12, but is also present in other rare-earth iron garnets, such as Tb3Fe5O12. The effect can facilitate ultrafast optical readout of magnetic bits at a sub-100~nm spatial scale.

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