• Accepted Paper

X-ray view of ultrafast Néel vector dynamics: Direct observation of light-induced spin reorientation in TmFeO3

Somnath Jana, Ronny Knut, Dmytro Afanasiev, Niko Pontius, Christian Schüßler-Langeheine, Christian Tzschaschel, Daniel Schick, Alexey V. Kimel, Olof Karis, Clemens von Korff Schmising, and Stefan Eisebitt

Phys. Rev. Lett. - Accepted 6 November, 2026

DOI: https://doi.org/10.1103/1cbm-wc5p

Abstract

Using time-resolved x-ray magnetic linear dichroism in reflection geometry, we provide a direct, element-specific probe of the Néel vector dynamics in TmFeO3 on ultrafast timescales. Our measurements reveal that, following optical excitation, the Néel vector rotates primarily within the ac~plane, achieving near-complete reorientation within ∼20 ps. This process is driven by a phonon-induced anisotropy change with a 10 ps relaxation time, accompanied by a coherent 80 GHz oscillation of the Néel vector around the dynamically evolving potential landscape. Our study demonstrates the capability of reflection-geometry soft x-ray spectroscopy to resolve intrinsic antiferromagnetic dynamics, paving the way for investigations of a broad range of functional antiferromagnets and application-relevant thin films.

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