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    Odd-Parity Magnetism Driven by Antiferromagnetic Exchange

    Yue Yu1, Magnus B. Lyngby2, Tatsuya Shishidou1, Mercè Roig1,2, Andreas Kreisel2, Michael Weinert1, Brian M. Andersen2, and Daniel F. Agterberg1

    Phys. Rev. Lett. 135, 046701 – Published 22 July, 2025

    DOI: https://doi.org/10.1103/zk69-k6b2

    Abstract

    Realizing odd-parity, time-reversal-preserving, nonrelativistic spin splitting is a central goal for spintronics applications. We propose a group-theory-based microscopic framework to induce odd-parity spin splitting from coplanar antiferromagnetic (AFM) states without spin-orbit coupling (SOC). We develop phenomenological models for 421 conventional period-doubling AFM systems in nonsymmorphic space groups and construct minimal microscopic models for 119 of these. We find that these AFM states can attain three possible competing ground states. These ground states all break symmetries in addition to those broken by the usual AFM order. Specifically, they give rise to either odd-parity spin-splitting, nematic order, or scalar odd-parity order related to multiferroicity. Our microscopic theories reveal that the odd-parity spin-splitting energy scale is generically large and further reveal that the scalar odd-parity order gives a nonzero Berry curvature dipole without SOC. We identify 67 materials in the Magndata database for which our theory applies. We provide density-functional theory (DFT) calculations on Fe-based materials that reveal an h-wave spin splitting consistent with our symmetry arguments and apply our microscopic model to determine the nonrelativistic Edelstein response for CeNiAsO.

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