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    Néel-Antiferromagnet-Proximitized Superconductivity in the NbSe2/MnPS3 Heterostructures

    Xinyi Zheng1,2,*, Ruihuan Duan3,*, Xilin Feng4,*, Desheng Wu5,6,*, Xue Yang1,2,7, Lihong Hu1,2, Lei Xu1,2, Sicheng Zhou1,2, Siyuan Zhou1,2 et al.

    Ximing Zhang1,2, Zishuo Peng1,2, Bingbing Tong1,8, Peiling Li1,2,8, Junya Feng1, Zhaozheng Lyu1,2,8, Hua Ke9, Jie Shen1,2,8, Jianlin Luo1,2,8, Fanming Qu1,2,8, Zheng Liu3,10, Kam Tuen Law4,†, Guangtong Liu1,2,8,‡, and Li Lu1,2,8,§

    • *These authors contribute equally to this work.
    • †Contact author: phlaw@ust.hk
    • ‡Contact author: gtliu@iphy.ac.cn
    • §Contact author: lilu@iphy.ac.cn

    Phys. Rev. Lett. 137, 156301 – Published 5 October, 2026

    DOI: https://doi.org/10.1103/xfg2-227f

    Abstract

    Antiferromagnet-superconductor (AFM-SC) hybrids offer a rich but largely unexplored platform for realizing spin-triplet Cooper pairing and chiral topological superconductivity, yet experimental demonstrations remain scarce. Here, we report the modification of superconductivity in NbSe2/MnPS3 heterostructures via the AFM proximity effect. The Néel order of MnPS3 effectively suppresses the Ising superconductivity of NbSe2 and induces a spatially inhomogeneous superconducting state with an inherent junction network. Leveraging this intrinsic Josephson coupling, we observe a finite phase offset in the critical-current interference pattern and a zero-field supercurrent diode effect—two independent signatures of spontaneous time-reversal symmetry breaking. Supported by theoretical modeling, we attribute these emergent phenomena to the proximity-induced stabilization of a subdominant in-plane triplet pairing channel, which is distinct from the intrinsic Ising channel of NbSe2. Our findings establish AFM-SC heterostructures as a versatile platform for exploring nonreciprocal transport and open promising avenues for superconducting spintronics.

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