We theoretically propose a scheme to enhance the photon indistinguishability of spectrally mismatched single photons via Floquet-engineered optical frequency combs in cavity quantum electrodynamic systems. By periodically modulating two distinct single-photon states under a modulation frequency which is exactly equal to the spectral mismatch of two cavity modes, a pair of single-photon frequency-comb states is prepared energy-conservatively based on full unitary operations. The two states show high indistinguishability with an ideal $g_{\mathrm{HOM}}^{(2)}(0)$ down to zero due to the superposition of intensity-matched single-photon states coherently distributed across the teeth of the combs.

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• Cavity quantum electrodynamics
• Molecular spectra
• Quantum states of light
• Single photon sources
• Spectral shaping
• Quantum dots
• Jaynes-Cummings model