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Electrically Tunable Picosecond-Scale Octupole Fluctuations in Chiral Antiferromagnets

Shiva T. Konakanchi1,*, Sagnik Banerjee2, Mohammad M. Rahman3, Yuta Yamane4,5, Shun Kanai4,6,7,8,9, Shunsuke Fukami4,6,7,10,11, and Pramey Upadhyaya2,†

  • 1Department of Physics and Astronomy, Purdue University, West Lafayette, Indiana 47907, USA
  • 2Elmore Family School of Electrical and Computer Engineering, Purdue University, West Lafayette, Indiana 47907, USA
  • 3Department of Chemistry and Biochemistry, University of Maryland, College Park, Maryland 20742, USA
  • 4Research Institute of Electrical Communication, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 Japan
  • 5Frontier Research Institute for Interdisciplinary Sciences, Tohoku University, Sendai 980-8578, Japan
  • 6WPI-Advanced Institute for Materials Research (WPI-AIMR), Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, Japan
  • 7Center for Science and Innovation in Spintronics, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, Japan
  • 8PRESTO, Japan Science and Technology Agency (JST), Kawaguchi 332-0012, Japan
  • 9Division for the Establishment of Frontier Sciences of Organization for Advanced Studies at Tohoku University, Tohoku University, Sendai 980-8577, Japan
  • 10Center for Innovative Integrated Electronic Systems, Tohoku University, 468-1 Aramaki Aza Aoba, Aoba-ku, Sendai 980-0845, Japan
  • 11Inamori Research Institute for Science, Kyoto 600-8411, Japan

  • *Contact author: skonakan@purdue.edu
  • †Contact author: prameyup@purdue.edu

Phys. Rev. Lett. 135, 136704 – Published 25 September, 2025

DOI: https://doi.org/10.1103/w2wj-c9jx

Abstract

We present a theory for the relaxation time of the octupole order parameter in nanoscale chiral antiferromagnets (AFMs) coupled to thermal baths and spin injection sources. Using stochastic spin dynamics simulations, we demonstrate that the octupole moment relaxes through two distinct mechanisms—escape over a barrier and precessional dephasing—as the barrier for octupole fluctuations is lowered relative to the thermal energy. Notably, the octupole moment relaxes orders of magnitude faster than the typical dipolar order parameters, reaching picosecond timescales. By combining Langer’s theory with an effective low-energy description of octupole dynamics in chiral AFMs, we derive analytical expressions for the relaxation times. We find that relaxation in chiral AFMs parallels dipole relaxation in XY magnets, with exchange fields serving the role of the dipole fields. Further, by drawing on the analogy between order parameter dynamics in XY magnets under spin injection and current-biased Josephson junctions, we propose a new scheme for electrically tuning the octupole relaxation times. Our Letter offers fundamental insights for the development of next-generation spintronic devices that harness octupole order parameters for information encoding.

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