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    Unveiling High-Energy Ultrafast Responses Driven by Fermi-Level Gap Opening in Charge-Density Waves

    Qiong Wu1,2,*,†, Tianchen Hu2,*,‡, Junhan Huang2, Yongjie Liu3, Fei Sun4,5, Shuxiang Xu6, Li Yue7, Zijian Lin2, Xinyu Zhou2 et al.

    Tao Dong8,2 and Nan-Lin Wang8,2,7,9,§

    • *These authors contributed equally to this work.
    • †Contact author: qwu@cqu.edu.cn
    • ‡Contact author: tchu@pku.edu.cn
    • §Contact author: nlwang@sjtu.edu.cn

    Phys. Rev. Lett. 137, 206902 – Published 12 November, 2026

    DOI: https://doi.org/10.1103/vz71-r52l

    Abstract

    Ultrafast pump-probe spectroscopy is indispensable for investigating interactions, collective excitations, and nonequilibrium dynamics in superconductors and correlated electron systems. However, how a small gap opening near the Fermi surface affects the spectral changes in the high-energy interband transition region remains elusive. To address this issue, we perform systematic studies of carrier relaxation dynamics in the prototype charge-density-wave (CDW) material EuAl4. We find that the CDW gap shrinks substantially under optical pumping. This band renormalization strongly modulates interband transitions associated with the gap edge, inducing a pronounced transient reflectivity change at the corresponding probe energies. These results establish a direct link between low-energy order-parameter dynamics and high-energy spectral responses, providing a general framework for interpreting transient signals in gapped quantum materials.

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