Unveiling High-Energy Ultrafast Responses Driven by Fermi-Level Gap Opening in Charge-Density Waves
Phys. Rev. Lett. 137, 206902 – Published 12 November, 2026
DOI: https://doi.org/10.1103/vz71-r52l
Abstract
Ultrafast pump-probe spectroscopy is indispensable for investigating interactions, collective excitations, and nonequilibrium dynamics in superconductors and correlated electron systems. However, how a small gap opening near the Fermi surface affects the spectral changes in the high-energy interband transition region remains elusive. To address this issue, we perform systematic studies of carrier relaxation dynamics in the prototype charge-density-wave (CDW) material . We find that the CDW gap shrinks substantially under optical pumping. This band renormalization strongly modulates interband transitions associated with the gap edge, inducing a pronounced transient reflectivity change at the corresponding probe energies. These results establish a direct link between low-energy order-parameter dynamics and high-energy spectral responses, providing a general framework for interpreting transient signals in gapped quantum materials.