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Direct Evidence for Anisotropic Magnetic Interaction in α−RuCl3 from Polarized Inelastic Neutron Scattering

Markus Braden1,*, Xiao Wang2,3,4, Alexandre Bertin1, Paul Steffens5, and Yixi Su2,†

  • *Contact author: braden@ph2.uni-koeln.de
  • †Contact author: y.su@fz-juelich.de

Phys. Rev. Lett. 134, 236702 – Published 12 June, 2025

DOI: https://doi.org/10.1103/vlzq-swfm

Abstract

Polarized neutron scattering experiments reveal anisotropy of magnetic correlations in the candidate Kitaev material α−RuCl3. The anisotropy of the inelastic response at the magnetic Bragg positions is opposite to the expectation for a simple Heisenberg model. Near the antiferromagnetic propagation vector, there are no low-energy transversal magnon modes and the response is always uniaxially polarized. These observations directly prove the fully anisotropic and bond-directional character of the magnetic interaction in α−RuCl3. However, other findings disagree with a simple or strongly dominant Kitaev component.

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