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    Close Proximity to a Quantum Phase Transition in TmZn2GaO5

    Matthew Ennis1,*, Rabindranath Bag1,*, Tessa Cookmeyer2,*, Matthew B. Stone3, Alexander I. Kolesnikov3, Tao Hong3, Leon Balents2, and Sara Haravifard1,4,5,†

    • *These authors contributed equally to this work.
    • †Contact author: sara.haravifard@duke.edu

    Phys. Rev. Lett. 136, 256707 – Published 24 June, 2026

    DOI: https://doi.org/10.1103/vhv1-pz6q

    Abstract

    TmZn2GaO5 is a newly synthesized triangular lattice magnet that exhibits a unique quantum phase characterized by strong Ising anisotropy, a pseudodoublet crystal electric field ground state, and a low-energy gapped excitation at the K point. Unlike its well-known counterparts, TmMgGaO4 and YbMgGaO4, this material crystallizes in a distinct hexagonal structure, leading to a platform for investigating frustrated magnetism. Magnetic susceptibility, heat capacity, and inelastic neutron scattering measurements confirm the absence of long-range magnetic order down to 50 mK, placing TmZn2GaO5 in a distinct region of the transverse-field Ising model phase diagram. Theoretical calculations based on spin-wave theory and mean-field modeling reproduce key experimental observations, reinforcing the material’s placement in a quantum disordered or multipolar state near a quantum critical point that separates it from the low-energy phase of TmMgGaO4. These results highlight its potential for exploring quantum disordered states, anisotropic excitations, and exotic quantum phases in frustrated spin systems.

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