Export citation

Export citation

Choose format for download:

Download Citation
  • Editors' Suggestion

Structural Phase Separation Couples to Charge-Density-Wave Formation in Kagome Metal FeGe

Boyang Zhao1, Youngjun Ahn1,*, Qinwen Deng2, Yidai Liu2, Sijie Xu4,5, Donald A. Walko3, Stephan O. Hruszkewycz1, Pengcheng Dai4,5, Liang Wu2 et al.

Haidan Wen1,3,†

  • *Contact author: youngjun.ahn@anl.gov
  • †Contact author: wen@anl.gov

Phys. Rev. Lett. 137, 146102 – Published 29 September, 2026

DOI: https://doi.org/10.1103/tqqs-s1r6

Abstract

The intertwining of charge, spin, and lattice degrees of freedom underlies the emergent properties of correlated materials. A recent prominent example is the kagome metal FeGe, which hosts a charge density wave (CDW) within a preexisting antiferromagnetic state. Although partial Ge-Ge dimerization is known to accompany CDW formation, the thermodynamic pathway through which long-range CDW order emerges remains unclear. Using temperature-dependent high-resolution x-ray diffraction measurements, we observed a robust splitting of the lattice reflection into two coexisting peaks with distinct lattice parameters in FeGe crystals exhibiting long-range CDW order at the CDW transition temperature. In addition, the long-range CDW order emerges concurrently and remains commensurate with a structural phase characterized by the smaller out-of-plane lattice parameter. Our observation provides direct evidence for a first-order structural phase transition coupled to long-range CDW order, which is absent in samples exhibiting short-range CDW order. A Landau model shows that strong charge-lattice coupling is a key factor in stabilizing the long-range CDW order. Our Letter reveals that the first-order structural phase transition is crucial for stabilizing long-range CDW order, suggesting lattice strain as a tuning parameter for controlling intertwined electronic states in kagome metals.

Physics Subject Headings (PhySH)

Authorization Required

We need you to provide your credentials before accessing this content.

Supplemental Material (Subscription Required)

References (Subscription Required)

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation