Export citation

Export citation

Choose format for download:

Download Citation

    Broadband Carrier-Envelope Phase-Controlled Stimulated Ultraviolet Emission from Carbon Dioxide Ions

    Jingsong Gao1,*, Hao Liang2,*, Ming-Shian Tsai3, Ming-Chang Chen3, Hans Jakob Wörner4, and Meng Han1,†

    • *These authors contributed equally to this work.
    • †Contact author: meng9@ksu.edu

    Phys. Rev. Lett. 135, 223802 – Published 24 November, 2025

    DOI: https://doi.org/10.1103/tjwb-9wxl

    Abstract

    A coherent broadband ultraviolet light source is essential for both fundamental research and industrial applications, yet its generation remains challenging. Here, we demonstrate microjoule-level ultraviolet emission spanning 300–450 nm from carbon dioxide ions (CO2+), driven by carrier-envelope-phase (CEP)-stabilized, near-single-cycle light pulses. The radiation arises from transitions between the first excited and ground cationic states, created by strong-field ionization with near-infrared pulses, and self-seeded by either self-phase modulation (SPM) or third-harmonic (TH) generation in the ultraviolet range. Interestingly, while TH-seeded stimulated emission is unaffected by CEP, SPM-seeded ultraviolet radiation shows strong CEP dependence. This arises from a Ramsey-type interference, where the relative phase between the SPM and the strong-field-prepared ionic polarization controls the constructive or destructive interference of the superposition between two ionic states, directly modulating the ionic dipole strength. Leveraging this CEP-sensitive lasing, we demonstrate a single-shot CEP tagging technique with remarkable resolution and simplicity. Our Letter establishes a powerful method for generating and controlling broadband ultraviolet stimulated emission in molecular ions using strong, waveform-stabilized ultrashort pulses, highlighting new possibilities in strong-field ionic quantum optics.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    Supplemental Material (Subscription Required)

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation