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Emergence of a Symmetry-Broken Chern Insulator near a Moiré Kondo Breakdown
Phys. Rev. Lett. 137, 206602 – Published 13 November, 2026
DOI: https://doi.org/10.1103/szcj-44xj
Abstract
Moiré semiconductors built on angle-aligned transition metal dichalcogenide (TMD) heterobilayers provide a physical realization of the Kondo lattice model, in which one TMD layer is prepared in a Mott insulating state supporting a lattice of local magnetic moments and the other layer in a metallic state supporting itinerant carriers. The artificial Kondo lattice enables the exploration of exotic states of matter near a continuously tunable Kondo breakdown. Here we report the emergence of a symmetry-broken Chern insulator at a moiré hole filling factor in angle-aligned moiré bilayers, which realize a chiral Kondo lattice. The symmetry-broken Chern insulator, which exhibits integer quantized Hall conductance at a fractional moiré filling, breaks the translational symmetry of the lattice spontaneously; it also appears only near a magnetic-field-induced Kondo breakdown in the mixed-valence regime of the material. We further demonstrate that the magnetic field required to induce the Kondo breakdown and to stabilize the symmetry-broken Chern insulator is twist angle dependent. The results present new opportunities for exploring the subtle interplay between topology and Kondo interactions in moiré semiconductors.
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References (48)
- S. Kirchner, S. Paschen, Q. Chen, S. Wirth, D. Feng, J. D. Thompson, and Q. Si, Colloquium: Heavy-electron quantum criticality and single-particle spectroscopy, Rev. Mod. Phys. 92, 011002(C) (2020).
- S. Paschen and Q. Si, Quantum phases driven by strong correlations, Nat. Rev. Phys. 3, 9 (2021).
- G. Stewart, Heavy-fermion systems, Rev. Mod. Phys. 56, 755 (1984).
- V. Vaňo, M. Amini, S. C. Ganguli, G. Chen, J. L. Lado, S. Kezilebieke, and P. Liljeroth, Artificial heavy fermions in a van der Waals heterostructure, Nature (London) 599, 582 (2021).
- G. Li et al., Two-dimensional Fermi surfaces in Kondo insulator , Science 346, 1208 (2014).
- M. Dzero, K. Sun, V. Galitski, and P. Coleman, Topological Kondo insulators, Phys. Rev. Lett. 104, 106408 (2010).
- J. Hertz, Quantum critical phenomena, Phys. Rev. B 14, 1165 (1976).
- A. Millis, Effect of a nonzero temperature on quantum critical points in itinerant fermion systems, Phys. Rev. B 48, 7183 (1993).
- P. Gegenwart, Q. Si, and F. Steglich, Quantum criticality in heavy-fermion metals, Nat. Phys. 4, 186 (2008).
- S. Wirth and F. Steglich, Exploring heavy fermions from macroscopic to microscopic length scales, Nat. Rev. Mater. 1, 16051 (2016).
- G. Stewart, Non-Fermi-liquid behavior in d- and f-electron metals, Rev. Mod. Phys. 73, 797 (2001).
- H. Löhneysen, A. Rosch, M. Vojta, and P. Wolfle, Fermi-liquid instabilities at magnetic quantum phase transitions, Rev. Mod. Phys. 79, 1015 (2007).
- J. Mydosh and P. Oppeneer, Colloquium: Hidden order, superconductivity, and magnetism: The unsolved case of , Rev. Mod. Phys. 83, 1301(C) (2011).
- M. P. Allan, F. Massee, D. K. Morr, J. Van Dyke, A. W. Rost, A. P. Mackenzie, C. Petrovic, and J. C. Davis, Imaging Cooper pairing of heavy fermions in , Nat. Phys. 9, 468 (2013).
- L. Jiao, S. Howard, S. Ran, Z. Wang, J. Olivares Rodriguez, M. Sigrist, Z. Wang, N. P. Butch, and V. Madhavan, Chiral superconductivity in heavy-fermion metal , Nature (London) 579, 523 (2020).
- W. Simeth et al., A microscopic Kondo lattice model for the heavy fermion antiferromagnet , Nat. Commun. 14, 8239 (2023).
- A. Kumar, N. C. Hu, A. H. MacDonald, and A. C. Potter, Gate-tunable heavy fermion quantum criticality in a moiré Kondo lattice, Phys. Rev. B 106, L041116 (2022).
- W. Zhao, B. Shen, Z. Tao, Z. Han, K. Kang, K. Watanabe, T. Taniguchi, K. F. Mak, and J. Shan, Gate-tunable heavy fermions in a moiré Kondo lattice, Nature (London) 616, 61 (2023).
- W. Zhao et al., Emergence of ferromagnetism at the onset of moiré Kondo breakdown, Nat. Phys. 20, 1772 (2024).
- Y. Zhang, W. Zhao, Z. Han, K. Watanabe, T. Taniguchi, J. Shan, and K. F. Mak, Thermoelectricity of moiré heavy fermions in bilayers, Phys. Rev. Lett. 136, 186501 (2026).
- W. Zhao et al., Emergence of Chern metal in a moiré Kondo lattice, arXiv:2506.14063.
- Z. Han, Y. Xia, Z. Xia, W. Zhao, Y. Zhang, K. Watanabe, T. Taniguchi, J. Shan, and K. F. Mak, Evidence of topological Kondo insulating state in moiré bilayers, Nat. Phys. 22, 396 (2026).
- D. Guerci, J. Wang, J. Zang, J. Cano, J. H. Pixley, and A. Millis, Chiral Kondo lattice in doped bilayers, Sci. Adv. 9, eade7701 (2023).
- J. Mendez-Valderrama, S. Kim, and D. Chowdhury, Correlated topological mixed-valence insulators in moiré heterobilayers, Phys. Rev. B 110, L201105 (2024).
- F. Xie, L. Chen, and Q. Si, Kondo effect and its destruction in heterobilayer transition metal dichalcogenides, Phys. Rev. Res. 6, 013219 (2024).
- Q. Wu et al., Realization of a Kondo insulator in a multilayer moire superlattice, arXiv:2507.01329.
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/szcj-44xj for device fabrication, electrical transport measurements, additional temperature-dependence data, transport evidence of heavy Fermi physics, Kondo breakdown schematics, twist angle dependence, high-field data, and schematic phase diagram.
- Z. Han et al., Stacking-order-dependent electronic properties of MoTe2/WSe2 moiré bilayers, arXiv:2605.21233.
- T. Li et al., Quantum anomalous Hall effect from intertwined moiré bands, Nature (London) 600, 641 (2021).
- W. Zhao et al., Realization of the Haldane Chern insulator in a moiré lattice, Nat. Phys. 20, 275 (2024).
- X. Chang et al., Electric-field-tuned consecutive topological phase transitions between distinct correlated insulators in moiré heterobilayer, Phys. Rev. Lett. 136, 096503 (2026).
- L. Wang, Y. Gao, B. Wen, Z. Han, T. Taniguchi, K. Watanabe, M. Koshino, J. Hone, and C. R. Dean, Evidence for a fractional fractal quantum Hall effect in graphene superlattices, Science 350, 1231 (2015).
- E. M. Spanton, A. A. Zibrov, H. Zhou, T. Taniguchi, K. Watanabe, M. P. Zaletel, and A. F. Young, Observation of fractional Chern insulators in a van der Waals heterostructure, Science 360, 62 (2018).
- H. Polshyn et al., Topological charge density waves at half-integer filling of a moiré superlattice, Nat. Phys. 18, 42 (2021).
- Y. Saito, J. Ge, L. Rademaker, K. Watanabe, T. Taniguchi, D. A. Abanin, and A. F. Young, Hofstadter subband ferromagnetism and symmetry-broken Chern insulators in twisted bilayer graphene, Nat. Phys. 17, 478 (2021).
- Y. Xie et al., Fractional Chern insulators in magic-angle twisted bilayer graphene, Nature (London) 600, 439 (2021).
- M. He, J. Cai, Y.-H. Zhang, Y. Liu, Y. Li, T. Taniguchi, K. Watanabe, D. H. Cobden, M. Yankowitz, and X. Xu, Symmetry-broken Chern insulators in twisted double bilayer graphene, Nano Lett. 23, 11066 (2023).
- R. Su, D. Waters, B. Zhou, K. Watanabe, T. Taniguchi, Y.-H. Zhang, M. Yankowitz, and J. Folk, Moiré-driven topological electronic crystals in twisted graphene, Nature (London) 637, 1084 (2025).
- D. Waters et al., Chern insulators at integer and fractional filling in moiré pentalayer graphene, Phys. Rev. X 15, 011045 (2025).
- Z. Zhang et al., Cascade of zero-field Chern insulators in magic-angle bilayer graphene, Natl. Sci. Rev. 13, nwaf265 (2025).
- S. Kitagawa, H. Ikeda, Y. Nakai, T. Hattori, K. Ishida, Y. Kamihara, M. Hirano, and H. Hosono, Metamagnetic behavior and Kondo breakdown in heavy-fermion CeFePO, Phys. Rev. Lett. 107, 277002 (2011).
- J. Cai et al., Signatures of fractional quantum anomalous Hall states in twisted , Nature (London) 622, 63 (2023).
- Y. Zeng, Z. Xia, K. Kang, J. Zhu, P. Knüppel, C. Vaswani, K. Watanabe, T. Taniguchi, K. F. Mak, and J. Shan, Thermodynamic evidence of fractional Chern insulator in moiré , Nature (London) 622, 69 (2023).
- H. Park et al., Observation of fractionally quantized anomalous Hall effect, Nature (London) 622, 74 (2023).
- F. Xu et al., Observation of integer and fractional quantum anomalous Hall effects in twisted bilayer , Phys. Rev. X 13, 031037 (2023).
- Z. Lu, T. Han, Y. Yao, A. P. Reddy, J. Yang, J. Seo, K. Watanabe, T. Taniguchi, L. Fu, and L. Ju, Fractional quantum anomalous Hall effect in multilayer graphene, Nature (London) 626, 759 (2024).
- H. Pan, M. Xie, F. Wu, and S. Das Sarma, Topological Phases in AB-Stacked : Topological Insulators, Chern Insulators, and Topological Charge Density Waves, Phys. Rev. Lett. 129, 056804 (2022).
- https://cstr.cn/31123.02.SECUF.